Journal
CHEMICAL ENGINEERING JOURNAL
Volume 350, Issue -, Pages 248-256Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2018.05.182
Keywords
rGO/ZnS-MoS(2)catalyst; Visible-light photocatalytic activity; Industrial wastewater treatment; COD removal
Categories
Funding
- Natural Science Foundation of China [51741806, 51178213, 51238002]
- National Science Fund for Excellent Young Scholars [51422807]
- Department of Education Fund of Jiangxi Province [GJJ150742]
- Natural Science Foundation of Jiangxi Province [20161BAB206117]
- Science Fund for Excellent Young Scholars of Jiangxi Province [20122BAB213014]
- Open fund by Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle [ES201780294]
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ZnS-MoS2 solid solution anchored on reduced graphene oxide sheet (rGO/ZnS-MoS2) was explored as novel visible-light-driven photocatalysts, and synthesized by solvent thermal method. The light absorption intensity of rGO/ZnS-MoS2 was greatly strengthened, and rGO/ZnS-MoS2 possess modulated continuous band gaps from 3.47 to 3.56 eV by changing the Zn/Mo ratios and rGO content. Their photocatalytic activities for 2-nitrophenol degradation are dependent on the chemical composition, and the optimal 11% rGO/ZnS-MoS2 possessed the highest photocatalytic performance, which could be attributed to the most efficient charge separation, the largest specific area, and its optimized band structure. Moreover, 11% rGO/ZnS-MoS2 can effectively treat real industrial effluent with 74.05% COD removal, and maintain long-term stability without obvious decline after five use cycle.
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