Journal
BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY
Volume 14, Issue -, Pages 1546-1553Publisher
BEILSTEIN-INSTITUT
DOI: 10.3762/bjoc.14.131
Keywords
amidation; C-H activation; cobalt; ferrocene; mechanochemistry
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Funding
- DFG
- CSC
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Versatile C-H amidations of synthetically useful ferrocenes were accomplished by weakly-coordinating thiocarbonyl-assisted cobalt catalysis. Thus, carboxylates enabled ferrocene C-H nitrogenations with dioxazolones, featuring ample substrate scope and robust functional group tolerance. Mechanistic studies provided strong support for a facile organometallic C-H activation manifold.
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