Journal
ADVANCED MATERIALS INTERFACES
Volume 4, Issue 22, Pages -Publisher
WILEY
DOI: 10.1002/admi.201700380
Keywords
breath sensor; dendronized gold nanoparticles; nanofibrous membrane paper; sweat sensor; tunable nanocomposite interfaces
Funding
- SUNY Network of Excellence in Materials and Advanced Manufacturing
- National Science Foundation [IIP 1640669]
- Direct For Mathematical & Physical Scien
- Division Of Materials Research [1409507] Funding Source: National Science Foundation
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The development of wearable breath or sweat sensor arrays for human performance monitoring is increasingly important for providing personalized health information under various environmental conditions. A major challenge is the lack of sensing elements responsive uniquely to moisture-dominated breathing and sweating processes, which is critical for differentiating other chemical or biological species from the moisture-dominated environment. Here a novel class of nanofibrous paper chemiresistors decorated with dendronized nanoparticles that exhibit structurally tunable and negative-going responses to human breathing and sweating is reported. The nanocomposite device features flexible membrane-type scaffold derived from multilayered nanofibrous paper as a biocompatible matrix and dendronized gold nanoparticles with tunable sizes and shapes to enable structural diversity and molecular sensitivity. Key elements of novelty include the immobilization of poly(ether-ester) dendrons with oligoethylene glycol spacers on gold nanoparticles and the combination of hydrogen bonding and van der Waals interactions between partially interpenetrating dendrons, leading to tunable and unique response characteristics to breathing and sweating processes. The results demonstrate the first example of nanofibrous paper chemiresistors decorated with dendronized nanoparticles as a promising new strategy toward constructing sensing interfaces for wearable breath and sweat sensors.
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