Journal
ORGANIC LETTERS
Volume 19, Issue 24, Pages 6530-6533Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03236
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- CSIR, New Delhi [02(0184)/14/EMR-II]
- UGC, New Delhi
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The first catalytic enantioselective total synthesis of (-)-podophyllotoxin is accomplished by a challenging organocatalytic cross-aldol Heck cyclization and distal stereocontrolled transfer hydrogenation in five steps from three aldehydes. Reversal of selectivity in hydrogenation led to the syntheses of other stereoisomers from the common precursor.
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