Journal
ORGANIC LETTERS
Volume 20, Issue 1, Pages 32-35Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03251
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- National Natural Science Foundation of China (NNSFC) [21672049]
- Hefei University of Technology
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An asymmetric dehydrogenative Diets Alder reaction of 2-methyl-3-phenylmethylindoles and alpha,beta-unsaturated aldehydes has been established. The successful in situ generation of the indole ortho-quinodimethane intermediate and the iminium activation of enals are the keys to success, providing various tetrahydrocarbazole derivatives with up to >99% ee.
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