Journal
ORGANIC LETTERS
Volume 19, Issue 24, Pages 6658-6661Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.7b03386
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Funding
- National Natural Science Foundation of China (NSFC) [21532010, 21372242, 21472214, 21421091, 21702109]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDB20030100]
- 1000-Talent Youth Plan of China
- European Community (FP7-PEOPLE-IIF) [912364]
- NSFC
- Research Grants Council of Hong Kong Joint Research Scheme [21361162001]
- Chinese Academy of Sciences, Nankai University
- Technology Commission of Shanghai Municipality
- Croucher Foundation of Hong Kong
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An asymmetric [3 + 2] cycloaddition reaction of vinyl epoxides with alpha,beta-unsaturated ketones, the single activated electron-deficient alkenes, has been achieved under Pd-catalysis in excellent diastereo- and enantioselectivity. The utilities of the protocol are demonstrated by transformation of the products into other useful chiral molecules. Density functional theory calculations rationalize the stereocontrol of the reaction.
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