Journal
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
Volume 100, Issue 12, Pages 5723-5730Publisher
WILEY
DOI: 10.1111/jace.15088
Keywords
nanocomposites; thermoelectric properties; tin; tin compounds; zinc oxide
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Funding
- National Natural Science Foundation of China [51572098, 51632006]
- National Basic Research Program of China [2013CB632500]
- Natural Science Foundation of Hubei province [2015CFB432]
- Open Fund of State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology [2016-KF-5]
- Graduates' Innovation Fund, Huazhong University of Science and Technology [5003110006]
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In this work, the thermoelectric properties of SnTe have been regulated synergistically by introduction of n-type ZnO nanoinclusions. On one hand, the excessive holes in SnTe matrix were compensated properly by n-type ZnO, and the Seebeck coefficient has been improved greatly due to the carrier energy filtering effect by a large quantity of ZnO-SnTe hetero-junction interface barriers; On the other hand, the thermal conductivity gets reduced by the enhanced phonon scattering from multiscale hierarchical architectures. Consequently, a maximum ZT of similar to 0.9 at 873K has been obtained in the 0.8 wt% sample, which enhances by 112% in comparison with the nanoinclusion-free sample.
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