Journal
ISRAEL JOURNAL OF CHEMISTRY
Volume 58, Issue 1-2, Pages 45-51Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ijch.201700088
Keywords
Iridium; ruthenium; enantioselective catalysis; carbonyl addition; hydrogen transfer
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Stereo- and site-selective methods for the byproduct-free modification of unprotected organic compounds that occur through the addition or redistribution of hydrogen are natural endpoints in the advancement of methods for efficient chemical synthesis. Progress toward this goal requires a departure from reactants that embody non-native structural elements, including stoichiometric organometallic reagents, directing/protecting groups and chiral auxiliaries. In this perspective, we highlight how hydrogen-mediated C-C bond formations developed in our laboratory have enabled progress toward ideal chemical syntheses of this type.
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