Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2017, Issue 21, Pages 3049-3054Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201700505
Keywords
Fluorinated compounds; Fluorine; C-H functionalization; Nitrogen heterocycles; Homogeneous catalysis; Alkenylation; Copper; Palladium
Categories
Funding
- INSA Rouen, Rouen University
- Centre National de la Recherche Scientifique (CNRS)
- EFRD
- Labex SynOrg [ANR-11-LABX-0029]
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The copper- and palladium/copper-catalyzed direct C-H fluoroalkenylation of pyridine N-oxides and related heterocycles using various gem-bromofluoroalkenes as electrophiles is reported. The dimetallic palladium/copper process proved to be more efficient than copper catalysis, giving access to various relevant 2-fluoroalkenylated azines.
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