Article
Engineering, Environmental
Zhenyu Chen, Xiaojun Luo, Yuan Zeng, Shufei Tan, Jie Guo, Zhenming Xu
Summary: The study found that the mass concentration of PM10 was higher but the number concentration was lower in the manual dismantling workshop compared to the thermal dismantling workshop. The gaseous phase PBDE concentration was higher in the manual dismantling workshop while the particulate phase PBDE concentration was higher in the thermal dismantling workshop. The size distribution of particles was similar between the two workshops, but there were significant differences in the distribution of particle-bound PBDE.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Public, Environmental & Occupational Health
Ming-Jun Hu, Jin-Liang Zhu, Qian Zhang, Jia-Liu He, Wan-Jun Yang, Zhen-Yu Zhu, Jia-Hu Hao, Fen Huang
Summary: Exposure to PBDEs and metals among rural adult residents along the Yangtze River in China may influence thyroid function, with some PBDE congeners and metals showing associations with thyroid hormones. However, there was no statistically significant association observed between PBDEs, metals, and thyroid-stimulating hormone. Bayesian Kernel Machine Regression analysis suggested similar trends in the relationship between PBDEs, metals mixtures, and thyroid hormones. Additional studies are needed to confirm these findings and identify potential mechanisms.
INTERNATIONAL JOURNAL OF HYGIENE AND ENVIRONMENTAL HEALTH
(2021)
Article
Environmental Sciences
Aalekhya Reddam, Andreas Sjodin, Whitney Cowell, Richard Jones, Shuang Wang, Frederica Perera, Julie B. Herbstman, Allison Kupsco
Summary: This study found associations between exposure to polybrominated diphenyl ethers (PBDEs) and birth outcomes in a cohort of Dominican and African American newborns, mainly affecting birth weight and length.
ENVIRONMENTAL RESEARCH
(2023)
Review
Biochemistry & Molecular Biology
Jinsong Xue, Qingqing Xiao, Min Zhang, Dan Li, Xiaofei Wang
Summary: Polybrominated diphenyl ethers (PBDEs) are widely used flame retardants found in various materials. They have been detected in soil, air, water, dust, and animal tissues, and are associated with a range of toxic effects on different organ systems. Understanding the mechanisms and potential toxicity of PBDEs is important for developing effective prevention strategies.
INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
(2023)
Article
Biochemistry & Molecular Biology
Chinemerem Ruth Ohoro, Abiodun Olagoke Adeniji, Lucy Semerjian, Anthony Ifeanyi Okoh, Omobola Oluranti Okoh
Summary: This study investigated the concentrations, potential sources, and compositional profile of PBDEs in the surface water and sediment of Nahoon Estuary in South Africa. The study found that the concentrations of PBDEs varied with the seasons and the most contaminated site was NH1, which was attributed to stormwater runoff from a creek. BDE-17 was the dominant PBDE congener detected. Although there was no correlation between the congeners and organic carbon and organic matter, the human health risk assessment indicated a low eco-toxicological risk. Constant monitoring is recommended to ensure the safety of the estuary.
Article
Environmental Sciences
Naomi Azar, Linda Booij, Gina Muckle, Tye E. Arbuckle, Jean R. Seguin, Elizabeth Asztalos, William D. Fraser, Bruce P. Lanphear, Maryse F. Bouchard
Summary: The study found that prenatal exposure to background levels of PBDEs, especially BDE-47, was associated with lower IQ scores in boys, but not in girls. This suggests that exposure to PBDEs during early development may have a sex-dependent and detrimental effect on a child's neurodevelopmental trajectory.
ENVIRONMENT INTERNATIONAL
(2021)
Article
Environmental Sciences
Mantong Jin, Shunfei Zhang, Jiaqi He, Zhuhao Lu, Shanshan Zhou, Nanxi Ye
Summary: The study investigated PBDE contamination in the microenvironment of family automobiles in Hangzhou City, China. Decabromodiphenyl ether (BDE-209) was found to be the major component, primarily sourced from volatile polyurethanes in seat covers and foot pads. Infants and toddlers were most exposed to PBDEs, with BDE-47 and -99 posing the primary health risks.
SCIENCE OF THE TOTAL ENVIRONMENT
(2021)
Article
Engineering, Environmental
Bingbing Sun, Jing Liu, Yu-Qi Zhang, Kenneth M. Y. Leungb, Eddy Y. Zeng
Summary: This study found that PBDEs in microplastics can leach upon ingestion, but the leaching kinetics of inherent contaminants from ingested microplastics are poorly understood. Although the bioaccumulation of PBDEs in fish oil can be accelerated in the gastrointestinal tract, the steady-state concentrations of PBDEs in cod tissue lipid through ingestion of microplastics were found to be below the lower end of the global PBDE concentration, suggesting that ingestion of microplastics by organisms remains a negligible pathway.
JOURNAL OF HAZARDOUS MATERIALS
(2021)
Article
Engineering, Environmental
Qiang Xie, Ronglan Yu, Duan Gui, Yuping Wu
Summary: This study analyzed PBDE bioaccumulation patterns in Indo-Pacific humpback dolphin samples from the Pearl River Estuary. The results showed that PBDE levels in these samples were the highest to date, with adult males and calves having the highest levels. The study also found a positive relationship between PBDE concentrations in calves and annual calf stranding death rates, suggesting that maternal exposure to PBDEs may contribute to the high death rates in calves.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Article
Environmental Sciences
Chunnian Da, Ruwei Wang, Qing Huang, Jinyu Mao, Lijin Xie, Chao Xue, Long Zhang
Summary: This study investigated the temporal changes of PBDEs in the sediment cores from the Anhui Province section of Yangtze River, China. It found that the dramatic increase of BDE-209 and n-ary sumation Br-3-Br-9-BDEs concentrations from 1990-2008 was consistent with the booming production and consumption of household appliances and electronics, while the recent declines may be associated with the decreasing use of legacy commercial PBDE mixtures.
BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY
(2021)
Article
Environmental Sciences
Ruixue Guo, Yumeng Qi, Beibei Li, Nannan Wu, Jie Tian, Zunyao Wang, Ruijuan Qu
Summary: This study systematically investigates the degradation kinetics and mechanisms of two common PBDEs congeners on biomass under sunlight irradiation conditions. It reveals the highest photodegradation rate on specific types of biomass and highlights the involvement of hydroxyl H in lignin from biomass in the formation of primary products.
Article
Environmental Sciences
Binxu Liu, Ningning Song, Tao Jiang, Juan Wu, Lei Zhang, Wei Ge, Chao Chai
Summary: The study investigated the distribution, congener patterns, possible sources, and ecological risks of polybrominated diphenyl ethers (PBDEs) in the surface sediments of 20 fishing ports along the coast of Bohai Sea. The results showed that BDE-209 was the dominant congener and high concentrations of PBDEs were found near Liaohe River, Haihe River, manufacturing plants of BFRs near Laizhou Bay, and tipping areas of marine garbage.
MARINE POLLUTION BULLETIN
(2021)
Article
Environmental Sciences
Shifra Yonis, Sanober Kahkashan, Dave Adelman, Rainer Lohmann
Summary: Hydrophobic organic contaminants (HOCs) are indicators of human activities that can negatively impact water quality. This study used polyethylene passive samplers to determine concentrations and gradients of polycyclic aromatic hydrocarbons (PAHs) and organochlorinated pesticides (OCPs) in Narragansett Bay. The results showed that PAHs deposited in the water column, while OCPs reached equilibrium.
MARINE POLLUTION BULLETIN
(2023)
Article
Marine & Freshwater Biology
Hongyu Li, Yunxue Li, Bushra Maryam, Zhiyong Ji, Jun Sun, Xianhua Liu
Summary: The combined toxicity of microplastics and polybrominated diphenyl ethers (PBDEs) poses a significant threat to aquaculture and food safety, affecting the health and gene expression of farmed fishes.
AQUATIC TOXICOLOGY
(2022)
Article
Biochemistry & Molecular Biology
Lai-Xin Liu, Ru-Rong Gu, Yang Jin, Xue-Qin Chen, Xu-Wen Li, Yue-Ming Zheng, Zhao-Bing Gao, Yue-Wei Guo
Summary: Natural polybrominated diphenyl ethers have various biological activities. In this study, five polybrominated diphenyl ether natural products and 30 new derivatives were synthesized and their activities were studied, which may contribute to the discovery of new marine polybrominated diphenyl ether derived drugs.
BIOORGANIC CHEMISTRY
(2022)
Article
Engineering, Environmental
Juliane Gluge, Rachel London, Ian T. Cousins, Jamie DeWitt, Gretta Goldenman, Dorte Herzke, Rainer Lohmann, Mark Miller, Carla A. Ng, Sharyle Patton, Xenia Trier, Zhanyun Wang, Martin Scheringer
Summary: The study reveals that there are diverse uses of per- and polyfluoroalkyl substances (PFAS), with limited information on alternatives. PFAS in consumer products can be easily replaced, while their uses in industrial processes require thorough evaluation. It is necessary to enhance coordination among stakeholders to ensure a transparent and coordinated phase-out of PFAS.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2022)
Article
Environmental Sciences
Maya E. Morales-McDevitt, Matthew Dunn, Ahsan Habib, Simon Vojta, Jitka Becanova, Rainer Lohmann
Summary: Textile waste emissions in Bangladesh could have significant impact on human and ecosystem health, but there is limited information on PFAS. A study found that fluorotelomer alcohols (FTOHs) were detected in air and water at almost all sites in Dhaka.
ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY
(2022)
Article
Oceanography
Mengyang Liu, Minggang Cai, Mengshan Duan, Meng Chen, Rainer Lohmann, Yan Lin, Junhua Liang, Hongwei Ke, Kai Zhang
Summary: The role of oceanic transport in the fate of semivolatile organic compounds in the Arctic Ocean is still unclear. Samples collected from the North Atlantic Ocean and the Arctic Ocean showed different concentrations and sources of PAHs. The Norwegian Atlantic Current and the East Greenland Current were identified as important pathways for the transport of PAHs to the Arctic Ocean.
JOURNAL OF GEOPHYSICAL RESEARCH-OCEANS
(2022)
Article
Environmental Sciences
Christine Gardiner, Anna Robuck, Jitka Becanova, Mark Cantwell, Sarit Kaserzon, David Katz, Jochen Mueller, Rainer Lohmann
Summary: Per- and polyfluoroalkyl substances (PFAS) have become a growing global concern due to their widespread presence, bioaccumulation, and adverse effects. In this study, a novel integrative passive sampler, a microporous polyethylene tube, was tested and sampling rates (R-s) for nine PFAS in surface waters were derived. The results demonstrated the potential use of passive samplers as measurement and assessment tools for PFAS in dynamic aquatic environments.
ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY
(2022)
Article
Engineering, Environmental
Heidi M. Pickard, Bridger J. Ruyle, Colin P. Thackray, Adela Chovancova, Clifton Dassuncao, Jitka Becanova, Simon Vojta, Rainer Lohmann, Elsie M. Sunderland
Summary: Per- and polyfluoroalkyl substances (PFAS) are anthropogenic chemicals widely used in modern commerce. This study focused on the bioaccumulation of PFAS precursors in recreational fish species collected from surface waters in New Hampshire. The results showed that many precursors have a higher bioaccumulation potential than their terminal PFAS, highlighting the need to consider these precursors in risk evaluations.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2022)
Article
Geosciences, Multidisciplinary
Ita Wulandari, Samuel Katz, Roger Patrick Kelly, Rebecca S. Robinson, Rainer Lohmann
Summary: The occurrence, trends, and sources of soot black carbon (BC) in coastal sediments were investigated using sediment cores from the US East Coast and Florida Straits. The study found that BC fluxes were similar at both sites and accounted for a significant percentage of total organic carbon (OC). Carbon stable isotope values indicated marine origin for OC and terrestrial origin for BC, with different sources observed between North Carolina and Florida Strait based on radiocarbon values and polycyclic aromatic hydrocarbon ratios.
GEOPHYSICAL RESEARCH LETTERS
(2023)
Article
Geosciences, Multidisciplinary
Lihong Zhang, Yuxin Ma, Simon Vojta, Maya Morales-McDevitt, Mario Hoppmann, Thomas Soltwedel, Jane Kirk, Amila De Silva, Derek Muir, Rainer Lohmann
Summary: Polycyclic aromatic hydrocarbons (PAHs) are continuously released from multiple sources and can be transported over long distances. This study investigated the presence, transport, and fate of PAHs in remote and deep oceans. Deploying passive samplers in different regions, including the High Arctic and high-emission areas, it was found that dissolved PAHs had higher concentrations in the high-emission areas. The study also found that PAHs were exported from the Arctic Ocean to the North Atlantic through the Fram Strait and the Davis Strait.
GEOPHYSICAL RESEARCH LETTERS
(2023)
Article
Chemistry, Analytical
Muhammad Sohail, Syed AliMusstjab Akber Shah Eqani, Shazia Ilyas, Habib Bokhari, Nadeem Ali, Joel E. Podgorski, Shafi Muhammad, Dave Adelman, Rainer Lohmann
Summary: This study provides new data on the distribution and sources of persistent organic pollutants (POPs) in the ambient air and surface soil along the Indus floodplain in Pakistan. The levels of DDTs and PCBs were found to be higher in both air and soil samples, with higher concentrations in the wet mountain zone. The air-soil exchange of DDTs and PCBs generally showed volatilization, except in a few samples from the frozen mountain zone and wet mountain zone. These findings suggest that long range regional atmospheric transport plays a role in the accumulation of POPs in colder areas of Pakistan.
ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS
(2023)
Article
Engineering, Environmental
Rainer Lohmann, Branislav Vrana, Derek Muir, Foppe Smedes, Jaromir Sobotka, Eddy Y. Zeng, Lian-Jun Bao, Ian J. Allan, Peleg Astrahan, Ricardo O. Barra, Terry Bidleman, Evgen Dykyi, Nicolas Estoppey, Gilberto Fillmann, Naomi Greenwood, Paul A. Helm, Liisa Jantunen, Sarit Kaserzon, J. Vinicio Macias, Keith A. Maruya, Francisco Molina, Brent Newman, Raimon M. Prats, Manolis Tsapakis, Mats Tysklind, Barend L. van Drooge, Cameron J. Veal, Charles S. Wong
Summary: Passive samplers are effective in monitoring the distribution and trends of organic pollutants in aquatic systems. The results show that certain pollutants are more concentrated in northern latitudes/Arctic Ocean, while others tend to reach equilibrium across sampling sites. Additionally, the concentrations of some pollutants are closely related to their production and use, indicating limited global transport.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Article
Engineering, Environmental
Larry B. Barber, Heidi M. Pickard, David A. Alvarez, Jitka Becanova, Steffanie H. Keefe, Denis R. LeBlanc, Rainer Lohmann, Jeffery A. Steevens, Alan M. Vajda
Summary: Aqueous film-forming foams used during fire training at Joint Base Cape Cod caused significant PFAS groundwater contamination. The potential for PFAS bioconcentration from contaminated groundwater exposure was assessed through laboratory experiments using fish, mussels, POCIS, and PETS. The study found species- and compound-specific differences in bioconcentration factors and linear and bilinear uptake patterns for PFAS.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Letter
Environmental Sciences
Matthew Dunn, Jitka Becanova, Jarod Snook, Rainer Lohmann
Article
Environmental Sciences
Jarod Snook, Jitka Becanova, Simon Vojta, Rainer Lohmann
Summary: Characterizing sorbent affinity for a target compound is an essential step in the process of capturing aquatic contaminants, but there is currently no standardized method to measure the sorbent-water distribution coefficient, leading to significant variations in experimental setup and performance. This study systematically tested variations in experimental design and proposed a reference procedure and general guidelines for batch experiments with different compounds and sorbents. Well-constrained K (sw) values for 23 PFAS and two sorbents were also reported.
Article
Engineering, Environmental
Rainer Lohmann, Branislav Vrana, Derek Muir, Foppe Smedes, Jaromir Sobotka, Eddy Y. Zeng, Lian-Jun Bao, Ian J. Allan, Peleg Astrahan, Ricardo O. Barra, Terry Bidleman, Evgen Dykyi, Nicolas Estoppey, Gilberto Fillmann, Naomi Greenwood, Paul A. Helm, Liisa Jantunen, Sarit Kaserzon, J. Vinicio Macias, Keith A. Maruya, Francisco Molina, Brent Newman, Raimon M. Prats, Manolis Tsapakis, Mats Tysklind, Barend L. van Drooge, Cameron J. Veal, Charles S. Wong
Summary: Persistent organic pollutants (POPs) are a global concern, but information on their trends in water has been missing. Passive samplers have emerged as an attractive alternative for monitoring POPs. Deployments of passive samplers at globally distributed sites showed variations in POPs concentrations, with some compounds displaying higher concentrations in specific regions. These results contribute to our understanding of the global distribution and transport of organic pollutants in aquatic systems.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2023)
Article
Environmental Sciences
Matthew Dunn, Jitka Becanova, Jarod Snook, Bridger Ruyle, Rainer Lohmann
Article
Engineering, Environmental
Heidi M. Pickard, Bridger J. Ruyle, Colin P. Thackray, Adela Chovancova, Clifton Dassuncao, Jitka Becanova, Simon Vojta, Rainer Lohmann, Elsie M. Sunderland
Summary: This study identified and quantified PFAS in recreational fish species collected from surface waters in New Hampshire, US. The results showed that many PFAS precursors have higher bioaccumulation potential than their terminal products. This study emphasized the need for risk evaluations to consider other bioaccumulative PFAS, including perfluoroalkyl sulfonamide precursors.
ENVIRONMENTAL SCIENCE & TECHNOLOGY
(2022)