Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 3, Issue 2, Pages 259-267Publisher
CHINESE CHEMICAL SOC
DOI: 10.1039/c5qo00381d
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Funding
- National Natural Science Foundation of China [21222203, 21372231, 21133011]
- Chinese Academy of Sciences
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Palladium-catalysed cross-coupling of aminals with N-sulfonyl hydrazones has been established via C-N bond activation under base-free conditions, in which one C-C bond and one C-S bond were simultaneously generated. It was successfully applied in the construction of a variety of aminomethyl substituted allylic sulfones. Preliminary mechanistic studies indicated that the unique electrophilic cyclopalladated complex was involved in the catalytic cycle.
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