Journal
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
Volume 476, Issue -, Pages 48-56Publisher
ELSEVIER
DOI: 10.1016/j.colsurfa.2015.03.021
Keywords
Polyelectrolytes; Multilayer coatings; 430SS; Corrosion; Self-healing; EIS
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Funding
- PAPD [50831004]
- Natural Science Foundation of Jiangsu Province [2012729]
- Innovation Fund of Jiangsu Province [BY2013072-06]
- National Natural Science Foundation of China [51171078, 11004098, 11374136]
- State Key Program for Basic Research of China [2010CB631004]
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We report the design and fabrication of smart polydiallyldimethylammonium chloride (PDDA)/polyacrylic acid (PAA) multilayer coatings with enhanced stimuli responsive self-healing and anti-corrosion ability for 430 stainless steel (SS). The multilayer coatings were prepared by layer-by-layer (LBL) technique, which allows a fine control over layer numbers (n) and coating thickness. The dependence of anti-corrosion and self-healing properties on layer number was investigated in 3% NaCl solution. The involved self-healing is attributed to the stimuli responsive swelling and electrostatic repairing of the polyelectrolyte multilayers (PEMu) in the vicinity of the scratches. The enhanced corrosion resistance ability is mainly due to the multilayer structure and the self-healing behavior that lengthens and hinders the diffusion pathway of corrosive species. (C) 2015 Elsevier B.V. All rights reserved.
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