Journal
ACS CATALYSIS
Volume 6, Issue 7, Pages 4699-4709Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.6b01227
Keywords
multimetallic complexes; rare earth metals; asymmetric catalysis; cooperative catalysis; C-C bond formation
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Professor Masakatsu Shibasaki's distinguished scientific accomplishments in the field of asymmetric catalysis are compiled here with particular emphasis on multimetallic cooperative catalysis. In 1992, he discovered revolutionary multimetallic chiral complexes composed of a rare earth metal, alkaline metals, and 1,1'-binaphthyl-2-binaphthols (BINOLs) that promoted a number of enantioselective reactions in a highly efficient and stereoselective manner. This finding resulted in chiral multimetallic catalysts that have significantly advanced the field of enantioselective catalysis.
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