Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 17, Pages 6501-6510Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201500122
Keywords
alcohols; heterogeneous catalysis; magnetic properties; oxidation; palladium
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Funding
- China Scholarship Council (CSC) of the People's Republic of China
- Ministere de la Recherche et de la Technologie (MRT)
- University of Bordeaux
- University of Toulouse 3
- Centre National de la Recherche Scientifique (CNRS)
- L'Oreal
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High efficiency and selectivity, easy magnetic recovery and recycling, and use of air as the oxidant at atmospheric pressure are major objectives for oxidation catalysis in terms of sustainable and green processes. A tris(triazolyl) ligand, so far only used in copper-catalyzed alkyne azide cycloadditions, was found to be extremely efficient in SiO2/-Fe2O3-immobilized palladium complexes. It was characterized by inductively coupled plasma (ICP) analysis, transmission electron microscopy (TEM), scanning transmission electron microscopy (STEM), energy-dispersive X-ray spectroscopy (EDX), and X-ray photoelectron spectra (XPS) and found to fulfill the combined conditions for the selective oxidation of alcohols to aldehydes and ketones.
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