Journal
ORGANOMETALLICS
Volume 35, Issue 11, Pages 1876-1884Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.organomet.6b00238
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Funding
- NSFC [21572155, 21372175]
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Unsymmetrical biaryls were synthesized by oxidative coupling reactions, between aromatic primary alcohols and arylboronic acids through the C-C bond cleavage of the primary alcohols chelated With a rhodium catalyst. The desired unsymmetrical biaryl products were obtained in good to excellent yields under the optimized reaction conditions. A wide variety of functionalities are compatible with the reaction under the optimized conditions. This new coupling strategy provides a favorable method to construct valuable biaryl compounds from aromatic primary alcohols which are cheap; environmentally friendly, and easily accessible substrates.
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