Journal
ORGANIC LETTERS
Volume 18, Issue 13, Pages 3186-3189Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b01398
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Funding
- Austrian Science Fund (FWF) [P28866-N34]
- X-ray center of the Vienna University of Technology
- Austrian Science Fund (FWF) [P 28866] Funding Source: researchfish
- Austrian Science Fund (FWF) [P28866] Funding Source: Austrian Science Fund (FWF)
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Air-stable, thermally robust, and well-defined cationic Ni(II) PNP pincer complexes based on the 2,4-diaminotriazine scaffold are described. These complexes are active catalysts for the Suzuki-Miyaura cross-coupling of a wide range of aryl, heteroaryl (including benzoxazole, thiazole, pyridine, pyrimidine, thiazole), primary and secondary alkyl halides, and pseudohalides with different organoboronate reagents giving excellent to good isolated yields. Neutral deprotonated complexes seem to play a key role in the catalytic process.
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