Journal
ORGANIC LETTERS
Volume 18, Issue 24, Pages 6256-6259Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b03017
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Funding
- University of York
- Leverhulme Trust [ECF-2015-013]
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A series of high-yielding silver(I)-catalyzed cyclization reactions of pyridine-, isoquinoline-, and pyrazineynones are described. The operationally simple and mild reaction conditions are a significant improvement over previously reported thermal cyclizations. The quinolizinone products were also used in a novel dearomatization strategy to prepare 0.53 g of the alkaloid lasubine II in five steps and 36% overall yield.
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