4.6 Article

Improving the luminescence enhancement of hybrid Au nanoparticle-monolayer MoS2 by focusing radially-polarized beams

Journal

OPTICS EXPRESS
Volume 24, Issue 24, Pages 27554-27562

Publisher

Optica Publishing Group
DOI: 10.1364/OE.24.027554

Keywords

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Funding

  1. National Key R & D Program of China [2016YFA0301700]
  2. Strategic Priority Research Program of the CAS [XDB01030000]
  3. Innovation Funds from the Chinese Academy of Sciences [60921091]
  4. Open Fund of the State Key Laboratory on Integrated Optoelectronics [IOSKL2015KF12]
  5. National Natural Science Foundation of China [11304301, 11374289, 11575172, 61306150, 61590932, 91421303]
  6. Fundamental Research Funds for the Central Universities

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Monolayer transition-metal dichalcogenides (TMDs) have grown as fantastic building blocks for optoelectronic applications, owing to their direct band gap, transparency, and mechanical flexibility. Since the luminescence of monolayer TMDs suffers from low light absorption and emission, surface plasmons, which confine light at subwavelength and enhance the local electric field, are utilized to boost both excitation and emission fields of TMDs, enabling strong light-matter interaction at the nano-scale. Meanwhile, radially-polarized beams (RPBs) as new and attractive excitation source have found many applications in surface plasmon polaritons, optical tweezer and so on. Here, by using RPBs, we demonstrate the photoluminescence (PL) enhancement of monolayer molybdenum disulfide (MoS2) hybridized with 210 nm-diameter gold nanoparticle (AuNP) is improved by about 1.37-fold compared with linearly-polarized beams (LPBs). Besides, the PL enhancement with RPBs depends on the size of AuNP as well. With 210nm-diameter AuNP, the PL enhancement is more than 1.5-fold higher than that with 60nm-diameter AuNP. This study highlights that RPBs are superior to LPBs for tuning the near-field system response and shows that RPBs drive a valuable avenue to further study the emerging two-dimentional materials. (C) 2016 Optical Society of America

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