4.7 Article

Enhanced thermoelectric performance of Bi2Te3 by carbon nanotubes and silicate aerogel co-doping toward ocean energy harvesting

Journal

MATERIALS TODAY SUSTAINABILITY
Volume 23, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.mtsust.2023.100476

Keywords

Thermoelectric materials; Doping; Preparation process; Thermoelectric properties; Hybrid energy harvesting

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In this study, a doped-modified thermoelectric generator (TEG) film was proposed and applied to an ocean energy harvesting prototype. The performance of a Bi2Te3-based thermoelectric material was improved by doping it with carbon nanotubes (CNTs) for high electrical conductivity and silica aerogel for low thermal conductivity. A performance-optimized, flexible thermoelectric film was fabricated using electron printing technology. When combined with a triboelectric nanogenerator (TENG) and electromagnetic generator (EMG), the hybrid energy harvesting prototype demonstrated a high output voltage and power density in simulated marine environmental experiments.
In this work, we propose a doped-modified thermoelectric generator (TEG) film and apply it to an ocean energy harvesting prototype that primarily utilizes ocean thermal energy. Firstly, A new Bi2Te3-based thermoelectric material with improved performance was synthesized by doping Bi2Te3 with Carbon nanotubes (CNTs) for their high electrical conductivity and Silica aerogel for their low thermal con-ductivity. Subsequently, a performance-optimized, flexible thermoelectric film was fabricated using electron printing technology. By combining the flexible thermoelectric film with a Triboelectric nano -generator (TENG) and Electromagnetic generator (EMG), a hybrid energy harvesting prototype was developed that can harvest marine renewable energy. The prototype demonstrates a relatively high output voltage of 61 V and an output power of 81.2 mW, corresponding to a power density of 8.1 W/m3 in simulated marine environmental experiments. This ocean-oriented hybrid energy prototype based on co-doped thermoelectric materials unveils new possibilities for self-powered devices in the field of ocean energy harvesting. & COPY; 2023 Elsevier Ltd. All rights reserved.

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