Journal
CHEMICAL PHYSICS LETTERS
Volume 637, Issue -, Pages 58-62Publisher
ELSEVIER
DOI: 10.1016/j.cplett.2015.07.046
Keywords
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Funding
- JPSJ [23244063, 26287060]
- Grants-in-Aid for Scientific Research [26287060, 26287061, 23244063, 26400324] Funding Source: KAKEN
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Femtosecond luminescence of 1-, 2-, and 6-8-layer graphenes as well as graphite (n = infinity) is studied in the near- to mid-infrared region, using a luminescence up-conversion method. The luminescence decay profiles show non-exponential behaviors within several picoseconds. Compared to graphite, 1- and 2-layer graphenes exhibit a remarkable reduction of lifetime at 0.3 eV. A two-temperature model that considers an effective Fermi energy successfully reproduces the decay profiles. On the basis of the Fermi energy (0.2 eV) of 1-layer graphene obtained from the photoemission experiment, we ascribe the layer number dependence of lifetime to the effective Fermi energy difference. (C) 2015 Elsevier B.V. All rights reserved.
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