4.8 Article

Holographic maps of quasiparticle interference

Journal

NATURE PHYSICS
Volume 12, Issue 11, Pages 1052-+

Publisher

NATURE PUBLISHING GROUP
DOI: 10.1038/NPHYS3829

Keywords

-

Funding

  1. Israel Science Foundation [1542/14]
  2. Harvard-MIT CUA
  3. NSF Grant [DMR-1308435]
  4. MURI-AFOSR
  5. ARO-MURI on Atomtronics
  6. ARO MURI Qusim Program
  7. M. Rossler, the Walter Haefner Foundation
  8. Humboldt Foundation
  9. Simons Foundation
  10. ETH Foundation
  11. Direct For Mathematical & Physical Scien
  12. Division Of Materials Research [1308435] Funding Source: National Science Foundation

Ask authors/readers for more resources

The analysis of Fourier-transformed scanning tunnelling microscopy images with subatomic resolution is a common tool for studying the properties of quasiparticle excitations in strongly correlated materials. Although Fourier amplitudes are generally complex valued, earlier analysis primarily focused on their absolute values. Their complex phases were often deemed random, and thus irrelevant, due to the unknown positions of the impurities in the sample. Here we show how to factor out these random phases by analysing overlaps between Fourier amplitudes that differ by reciprocal lattice vectors. The resulting holographic maps provide important and previously unknown information about the electronic structures. When applied to superconducting cuprates, our method solves a long-standing puzzle of the dichotomy between equivalent wavevectors. We show that d-waveWannier functions of the conduction band provide a natural explanation for experimental results that were interpreted as evidence for competing unconventional charge modulations. Our work opens a new pathway to identify the nature of electronic states in scanning tunnelling microscopy.

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.8
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Article Instruments & Instrumentation

In situ uniaxial pressure cell for x-ray and neutron scattering experiments

G. Simutis, A. Bollhalder, M. Zolliker, J. Kuespert, Q. Wang, D. Das, F. Van Leeuwen, O. Ivashko, O. Gutowski, J. Philippe, T. Kracht, P. Glaevecke, T. Adachi, M. Zimmermann, S. Van Petegem, H. Luetkens, Z. Guguchia, J. Chang, Y. Sassa, M. Bartkowiak, M. Janoschek

Summary: We propose an in situ uniaxial pressure device designed for small angle x-ray and neutron scattering experiments at low temperatures and high magnetic fields. The device uses a rod with an integrated transducer to transmit force to the sample, allowing forces of up to 200 N in both compressive and tensile configurations. It can be operated in a continuous-pressure mode with feedback control while the temperature is changing. The device is compatible with various instruments and cryostats through simple and exchangeable adapters, and it supports rapid sample changes with multiple sample holders.

REVIEW OF SCIENTIFIC INSTRUMENTS (2023)

Article Multidisciplinary Sciences

Tunable unconventional kagome superconductivity in charge ordered RbV3Sb5 and KV3Sb5

Z. Guguchia, C. Mielke, D. Das, R. Gupta, J. -X. Yin, H. Liu, Q. Yin, M. H. Christensen, Z. Tu, C. Gong, N. Shumiya, Md Shafayat Hossain, Ts Gamsakhurdashvili, M. Elender, Pengcheng Dai, A. Amato, Y. Shi, H. C. Lei, R. M. Fernandes, M. Z. Hasan, H. Luetkens, R. Khasanov

Summary: In this study, pressure-tuned and ultra-low temperature muon spin spectroscopy was used to uncover the unconventional nature of superconductivity in RbV3Sb5 and KV3Sb5. It was found that at ambient pressure, time-reversal symmetry breaking charge order was observed in RbV3Sb5, and the superconducting state displayed a nodal energy gap and reduced superfluid density. Applying pressure suppressed the charge-order transitions, increased the superfluid density, and progressively evolved the superconducting state from nodal to nodeless. The optimal superconductivity state was found to break time-reversal symmetry. These results offer unique insights into the nature of the pairing state and highlight the tunable nodal kagome superconductivity competing with time-reversal symmetry-breaking charge order.

NATURE COMMUNICATIONS (2023)

Article Chemistry, Physical

Partitioning the Two-Leg Spin Ladder in Ba2Cu1-xZnxTeO6: From Magnetic Order through Spin-Freezing to Paramagnetism

Charlotte Pughe, Otto H. J. Mustonen, Alexandra S. Gibbs, Stephen Lee, Rhea Stewart, Ben Gade, Chennan Wang, Hubertus Luetkens, Anna Foster, Fiona C. Coomer, Hidenori Takagi, Edmund J. Cussen

Summary: Ba2CuTeO6 is a material with a two-leg spin ladder structure of Cu2+ cations, which can be chemically tuned by substituting non-magnetic Zn2+ at the Cu2+ site. The substitution partitions the spin ladders into clusters, leading to a transition from long-range order to spin-freezing as the Zn2+ substitution increases. This provides a well-controlled tuning of the magnetic disorder and a model system for studying defects and segmentation in low-dimensional quantum magnets.

CHEMISTRY OF MATERIALS (2023)

Article Chemistry, Inorganic & Nuclear

A Trinuclear High-Spin Iron(III) Complex with a Geometrically Frustrated Spin Ground State Featuring Negligible Magnetic Anisotropy and Antisymmetric Exchange

Benjamin Kintzel, Michael Boehme, Daniel Plaul, Helmar Goerls, Nicolas Yeche, Felix Seewald, Hans -Henning Klauss, Andrei A. Zvyagin, Erik Kampert, Thomas Herrmannsdoerfer, Gwendolyne Pascua, Christopher Baines, Hubertus Luetkens, Winfried Plass

Summary: The trinuclear high-spin iron(III) complex [Fe3Cl3(saltag(Br))(py)(6)]ClO4 was synthesized and characterized. Magnetic measurements showed antiferromagnetic exchange between the iron(III) ions, resulting in a geometrically spin-frustrated ground state. High-field magnetization and muon-spin relaxation experiments confirmed the isotropic nature of the magnetic exchange and the absence of significant intermolecular interactions. The complex is considered an ideal candidate for studying spin-electric effects.

INORGANIC CHEMISTRY (2023)

Article Multidisciplinary Sciences

Nodeless electron pairing in CsV3Sb5-derived kagome superconductors

Yigui Zhong, Jinjin Liu, Xianxin Wu, Zurab Guguchia, J. -x. Yin, Akifumi Mine, Yongkai Li, Sahand Najafzadeh, Debarchan Das, Charles Mielke, Rustem Khasanov, Hubertus Luetkens, Takeshi Suzuki, Kecheng Liu, Xinloong Han, Takeshi Kondo, Jiangping Hu, Shik Shin, Zhiwei Wang, Xun Shi, Yugui Yao, Kozo Okazaki

Summary: The newly discovered kagome superconductors offer a promising platform to explore the interplay between band topology, electronic order, and lattice geometry. However, the nature of the superconducting ground state and the electron pairing symmetry in this system is still not well understood. In this study, we directly observed a nodeless and nearly isotropic superconducting gap in the momentum space of two different kagome superconductors using high-resolution and low-temperature angle-resolved photoemission spectroscopy. The unique properties of the superconducting gap are independent of charge order in the normal state. This comprehensive characterization provides essential information about the electron pairing symmetry in kagome superconductors and advances our understanding of superconductivity and intertwined electronic orders in quantum materials.

NATURE (2023)

Article Instruments & Instrumentation

GermanIum array for non-destructive testing (GIANT) setup for muon-induced x-ray emission (MIXE) at the Paul Scherrer Institute

Lars Gerchow, Sayani Biswas, Gianluca Janka, Carlos Vigo, Andreas Knecht, Stergiani Marina Vogiatzi, Narongrit Ritjoho, Thomas Prokscha, Hubertus Luetkens, Alex Amato

Summary: The pioneering work on Muon-induced x-ray emission (MIXE) technique was conducted at the Paul Scherrer Institute (PSI) in the 1980s for non-destructive assessment of elemental compositions. In recent years, this method has been improved and adopted at many muon facilities worldwide. The GermanIum Array for Non-destructive Testing (GIANT) setup at PSI is a dedicated MIXE spectrometer that offers excellent performance and has been used for various applications such as archaeological research and collaboration with the industry.

REVIEW OF SCIENTIFIC INSTRUMENTS (2023)

Article Humanities, Multidisciplinary

The non-destructive investigation of a late antique knob bow fibula (Bugelknopffibel) from Kaiseraugst/CH using Muon Induced X-ray Emission (MIXE)

Sayani Biswas, Isabel Megatli-Niebel, Lilian Raselli, Ronald Simke, Thomas Elias Cocolios, Nilesh Deokar, Matthias Elender, Lars Gerchow, Herbert Hess, Rustem Khasanov, Andreas Knecht, Hubertus Luetkens, Kazuhiko Ninomiya, Angela Papa, Thomas Prokscha, Peter Reiter, Akira Sato, Nathal Severijns, Toni Shiroka, Michael Seidlitz, Stergiani Marina Vogiatzi, Chennan Wang, Frederik Wauters, Nigel Warr, Alex Amato

Summary: A knob bow fibula of the Leutkirch type was excavated in 2018 in Switzerland and analyzed for its elemental composition. The fibula was made of bronze and consisted of two workpieces, with one being cast bronze and the other being forged bronze. The main elements in the fibula were copper, zinc, tin, and lead.

HERITAGE SCIENCE (2023)

Article Chemistry, Multidisciplinary

The pairing symmetry in quasi-one-dimensional superconductor Rb2Mo3As3

Ziga Gosar, Tina Arh, Kevin Jaksetic, Andrej Zorko, Wenhao Liu, Hanlin Wu, Chennan Wang, Hubertus Luetkens, Bing Lv, Denis Arcon

Summary: Quasi-one-dimensional electron systems exhibit instability towards long-range ordered phases at low temperatures. In this study, muon spin rotation and relaxation (& mu;SR) were used to investigate the superconducting state in Rb2Mo3As3, which has one of the highest critical temperatures Tc = 10.4 K among quasi-one-dimensional superconductors. The results show stronger damping below Tc due to the formation of a vortex lattice. Comparison of different models suggests that the s-wave scenario provides the best fit, but with an anomalously small superconducting gap ⠁0/Tc ratio of 2 ⠁0/kBTc = 2.74(1). However, the nodal p-wave or d-wave scenarios cannot be ruled out based on slightly worse fits, yielding more realistic ratios of 2 ⠁0/kBTc = 3.50(2) and 2 ⠁0/kBTc = 4.08(1), respectively.

JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS (2023)

Review Materials Science, Multidisciplinary

Unconventional charge order and superconductivity in kagome-lattice systems as seen by muon-spin rotation

Z. Guguchia, R. Khasanov, H. Luetkens

Summary: Kagome lattices are intriguing and rich platforms for studying the intertwining of topology, electron correlation, and magnetism. In this review, recent experimental progress on superconductivity and magnetic fingerprints of charge order in kagome-lattice systems is discussed. The systems include AV(3)Sb(5), LaRu3Si2, and CeRu2, which exhibit unique properties such as time-reversal symmetry-breaking charge ordered state, unconventional superconductivity, and rare nodeless magnetic kagome superconductivity.

NPJ QUANTUM MATERIALS (2023)

Article Materials Science, Multidisciplinary

Neutron diffraction, muon-spin rotation, and high magnetic field investigation of the multiferroic antiferromagnetic quantum spin-chain system CuCrO4

J. M. Law, H. Luetkens, G. Pascua, Th. Hansen, R. Glaum, Z. -s. Wang, J. Wosnitza, R. K. Kremer

Summary: We investigated the long-range magnetic ordering in the linear-chain spin S = 1/2 compound CuCrO4 using powder neutron diffraction and muon-spin rotation measurements. Both methods confirmed the presence of incommensurate long-range antiferromagnetic ordering below 8.5(3) K. The magnetic structure was determined based on neutron powder diffraction patterns, with a propagation vector iota = (0, 0, 0.546(1)). The Cu moments form a helicoidal spiral with an easy plane coinciding with the equatorial planes of the Jahn-Teller elongated CuO6 octahedra. The multiferroic phase was found to extend up to similar to 25 T, beyond which a new phase appeared. The magnetic moment is expected to fully saturate at fields much higher than 60 T.

PHYSICAL REVIEW B (2023)

Proceedings Paper Physics, Applied

An experimental procedure to determine quantitative muon Knight shifts

Fabian Hotz, Tina Arh, Zurab Guguchia, Debarchan Das, Chennan Wang, Matjaz Gomilsek, Andrej Zorko, Hubertus Luetkens

Summary: Muon Knight-shift measurements are challenging due to the lack of a direct method for measuring the applied external magnetic field. We propose a solution to this problem and suggest a suitable sample mounting and correcting scheme. This allows us to accurately determine the Knight-shift values even in extreme sample environments where separate measurements of the magnetic field are not feasible or practical using NMR or additional mu SR.

15TH INTERNATIONAL CONFERENCE ON MUON SPIN ROTATION, RELAXATION AND RESONANCE (2023)

Article Materials Science, Multidisciplinary

Neutron scattering sum rules, symmetric exchanges, and helicoidal magnetism in MnSb2O6

E. Chan, H. Lane, J. Pasztorova, M. Songvilay, R. D. Johnson, R. Downie, J-W. G. Bos, J. A. Rodriguez-Rivera, S. -W. Cheong, R. A. Ewings, N. Qureshi, C. Stock

Summary: MnSb2O6 is a noncentrosymmetric crystal with magnetic properties. It exhibits a tilted helicoidal magnetic structure at temperatures below 12K. However, this tilted structure is not favored over the pure cycloidal structure.

PHYSICAL REVIEW B (2023)

Article Materials Science, Multidisciplinary

Magnetic structure and crystal field states of Pr2Pd3Ge5: ?SR and neutron scattering investigations

V. K. Anand, D. T. Adroja, C. Ritter, Debarchan Das, Harikrishnan S. Nair, A. Bhattacharyya, Leandro Liborio, Simone Sturniolo, F. L. Pratt, Duc Le, G. Andre, Hubertus Luetkens, A. D. Hillier, Z. Hossain

Summary: We present results of muon spin relaxation (mu SR), neutron powder diffraction (NPD), and inelastic neutron scattering (INS) investigations on polycrystalline Pr2Pd3Ge5. The polycrystalline compound exhibits two antiferromagnetic transitions, which were confirmed by heat capacity measurements. Magnetic Bragg peaks were observed in the magnetically ordered state, and the magnetic structure was determined to be a canted antiferromagnetic structure of ordered Pr3+ moments. In the paramagnetic state, crystal electric field (CEF) excitations were observed through INS, and a CEF level scheme was derived through analysis.

PHYSICAL REVIEW B (2023)

Article Materials Science, Multidisciplinary

Coexistence of random singlets and disordered Kitaev spin liquid in H3LiIr2O6

Chanhyeon Lee, Suheon Lee, Youngsu Choi, C. Wang, H. Luetkens, T. Shiroka, Zeehoon Jang, Young-Gui Yoon, Kwang-Yong Choi

Summary: We used various measurements, including magnetic susceptibility, muon-spin relaxation, and nuclear magnetic resonance, to study the spin dynamics of the quantum spin liquid candidate H3LiIr2O6. We identified two characteristic temperatures, Tg = 110 K and T* = 26 K, through analysis of the relaxation rates. Below Tg, there were distinct components of slower relaxation rate governed by gapped excitations and faster relaxation rate related to gapless excitations. We observed divergent magnetic susceptibility, power-law dependence of relaxation rate on temperature, and weakly activated behavior, indicating the coexistence of a disordered spin-liquid state and spin singlets with distributed gaps.

PHYSICAL REVIEW B (2023)

Article Materials Science, Multidisciplinary

?SR measurements on Sr2RuO4 under (110) uniaxial stress

Vadim Grinenko, Rajib Sarkar, Shreenanda Ghosh, Debarchan Das, Zurab Guguchia, Hubertus Luetkens, Ilya Shipulin, Aline Ramires, Naoki Kikugawa, Yoshiteru Maeno, Kousuke Ishida, Clifford W. Hicks, Hans-Henning Klauss

Summary: Muon spin rotation/relaxation (μSR) and polar Kerr effect measurements provide evidence for a time-reversal symmetry breaking (TRSB) superconducting state in Sr2RuO4. However, the absence of a cusp in the superconducting transition temperature (Tc) vs stress and the absence of a resolvable specific heat anomaly at TRSB transition temperature (TTRSB) under uniaxial stress challenge a hypothesis of TRSB superconductivity. Recent μSR studies under pressure and with disorder indicate that the splitting between Tc and TTRSB occurs only when the structural tetragonal symmetry is broken. To further test such behavior, we measured Tc through susceptibility measurements and TTRSB through μSR, under uniaxial stress applied along a (110) lattice direction. We have obtained preliminary evidence for suppression of TTRSB below Tc, at a rate much higher than the suppression rate of Tc.

PHYSICAL REVIEW B (2023)

No Data Available