Article
Materials Science, Ceramics
Jingjing Wang, Dayu Zhou, Wei Dong, Xiaoduo Hou, Feng Liu, Nana Sun, Faizan Ali, Ziqi Li
Summary: The study demonstrates that the ferroelectric properties and crystalline structure of pure zirconia thin films are influenced by film thickness, with an increase in thickness leading to a higher m-phase fraction. Futhermore, a phase transition from orthorhombic to cubic and tetragonal phases was observed as the thickness increased.
CERAMICS INTERNATIONAL
(2021)
Article
Materials Science, Ceramics
Leonard Jacques, Veronika Kovacova, Jung In Yang, Susan Trolier-McKinstry
Summary: This study investigates the activation energies for KNN thin films with manganese doping, revealing that crystallization is nucleation-limited and can be reduced by using a seed layer.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2021)
Article
Materials Science, Ceramics
Li Zhang, Chen Zhou, Renhuai Wei, Xiaotian Kong, Xuebin Zhu
Summary: In this study, LaRh1-xNixO3 (x = 0, 0.05, 0.1) thin films were deposited by chemical solution deposition. The results showed that Ni doping can enhance the conductivity of the films, making them suitable for a wide range of applications.
CERAMICS INTERNATIONAL
(2023)
Article
Physics, Applied
Kuan-Ting Ho, Daniel Monteiro Diniz Reis, Karla Hiller
Summary: This study reveals the mechanism of resistance degradation in lead-free alternative KNN thin films, finding that the conduction mechanism is Schottky-limited and the resistance degradation is accompanied by the interfacial accumulation of additional charged defects and a reduction in Schottky barrier height. The results show that oxygen vacancies accumulate in the field-up polarity and multiple defects, potentially oxygen vacancies and holes trapped by potassium vacancies, accumulate in the field-down polarity. By measuring different film samples, it is found that the natural logarithm of leakage current is linearly proportional to the defect concentration to the power of 0.25.
APPLIED PHYSICS LETTERS
(2022)
Review
Chemistry, Multidisciplinary
Bingbing Yang, Linghua Jin, Renhuai Wei, Xianwu Tang, Ling Hu, Peng Tong, Jie Yang, Wenhai Song, Jianming Dai, Xuebin Zhu, Yuping Sun, Shujun Zhang, Xiaolin Wang, Zhenxiang Cheng
Summary: This paper summarizes the development of bismuth ferrite thin films in recent years, introduces the method and challenges of chemical solution route preparation. It also proposes an all-solution chemical-solution deposition (AS-CSD) method to prepare ferroelectric films with different orientations, and studies their growth, structure, and ferroelectric properties.
Article
Chemistry, Physical
TeJing Jiao, Caiyin You, Na Tian, Li Ma, ZongFan Duan, FuXue Yan, PengRong Ren, GaoYang Zhao
Summary: LiFe5O8/Ba0.6Sr0.4TiO3 (LFO/BST) composite films were fabricated via chemical solution deposition method, where the internal electric field could be established inside the film owing to the lithium ions' de-intercalating effect of LiFe5O8 (LFO) layer under the bias field. Thus, we successfully achieved a high dielectric tunability and low loss in the composite films.
APPLIED SURFACE SCIENCE
(2022)
Review
Chemistry, Multidisciplinary
Sucheta Sengupta, Rinki Aggarwal, Yuval Golan
Summary: Among the chemical deposition methods, chemical deposition from aqueous solution (CD) is the oldest and most studied process. It requires an intricate balance of growth parameters to produce high-quality thin films. The presence of complexing agents helps to control the morphology of the thin films.
MATERIALS CHEMISTRY FRONTIERS
(2021)
Article
Engineering, Electrical & Electronic
Li Zhang, Yanqiu Liu, Renhuai Wei, Xiaotian Kong, Ping Li, Jiangying Yu, Kai Huang, Xuebin Zhu
Summary: In this study, epitaxial La0.7Sr0.3MnO3 thin films were successfully prepared by using an ultraviolet laser-assisted annealing technique. The films exhibited a specific epitaxial relationship and showed enhanced properties with increasing laser energy density.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2022)
Review
Chemistry, Multidisciplinary
Wenqian Yao, Hongtao Liu, Jianzhe Sun, Bin Wu, Yunqi Liu
Summary: This review provides a comprehensive overview of current challenges and opportunities for chemical vapor deposition (CVD) growth, characterization, and electrical properties of graphene depending on the layer number and twist angles. Various state-of-the-art innovations using the CVD method are presented, and the underlying growth mechanisms and characterization methods are discussed.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Materials Science, Ceramics
Rong Tu, Zhen Liu, Qingfang Xu, Song Zhang, Qizhong Li, Xian Zhang, Marina L. Kosinova, Takashi Goto
Summary: Silicon nitride films were fabricated using halide laser chemical vapor deposition (LCVD) for surface protection of electronic devices. The study investigated the effects of deposition parameters on the crystallinity, microstructure, deposition rate, Vickers microhardness, nano-hardness, and electrical resistivity. The highest deposition rate was achieved at a temperature of 1573 K and pressure of 10 kPa. The hardness of the films increased with temperature and the electrical resistivity decreased.
JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
(2023)
Article
Engineering, Electrical & Electronic
Hao Wang, Jian Zhai, Wenhui Lu, Jianguo Chen, Jinrong Cheng
Summary: BF-PT thin films deposited on stainless steel substrates exhibit superior microstructure and excellent dielectric, ferroelectric properties, as well as outstanding fatigue resistance.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2021)
Article
Materials Science, Multidisciplinary
L. N. Maskaeva, E. V. Mostovshchikova, I. V. Vaganova, V. F. Markov, V. I. Voronin, A. D. Kutyavina, I. N. Miroshnikova, E. G. Vovkotrub
Summary: Films of cubic substitutional CdxPb1-xS solid solutions were synthesized using chemical bath deposition with varying cadmium acetate salt concentrations, leading to changes in crystal structure, chemical composition, morphology, and optical properties. The study also found that the concentration of cadmium acetate in the solution significantly affects the properties of the synthesized solid solution films.
Article
Engineering, Electrical & Electronic
Huan Liu, Yuanbo Gong, Hongwei Diao, Xiaojie Jia, Lei Zhao, Wenjing Wang, Wei Wang, Jun Zong
Summary: Ce-doped indium oxide (ICO) films were prepared via reactive plasma deposition, and the impact of annealing temperature and time on the electrical, optical, and structural properties of the films was investigated. The results showed that annealing treatment improved the crystallinity, grain size, transmittance, and reduced resistivity of the ICO films. Annealing at 210 degrees C in air for 50 min yielded films with a mobility of 93.3 cm²/V s, carrier concentration of 2.48 x 10²⁰/cm³, average transmittance of 86.5%, and resistivity of 2.6 x 10⁻⁴ Ω·cm. The ICO films exhibited higher carrier mobility and lower carrier concentration compared to Sn-doped In₂O₃ (ITO) films, which is favorable for enhancing the efficiency of solar cells.
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
(2023)
Article
Materials Science, Ceramics
Martina Angermann, Georg Jakopic, Christine Prietl, Thomas Griesser, Klaus Reichmann, Marco Deluca
Summary: In this study, RuO2 thin films were synthesized using water and acetic acid as solvents. The microstructure, phase purity, electrical and optical properties, as well as thermal stability of the films were characterized. The films showed metallic behavior with low resistivity and high optical absorption.
JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY
(2023)
Article
Chemistry, Multidisciplinary
Li Liu, Mariko Ueda, Toshiyuki Kawaharamura
Summary: In this research, antimony doped tin oxide thin films are grown using an environmental-friendly mist chemical vapor deposition system. The role of different solutions in supporting the film fabrication process is analyzed and studied. The experimental results show that the choice of supporting solution affects the conductivity and transmittance of the Sb:SnOx films.
Article
Materials Science, Ceramics
Yujuan Xie, Bi-Xia Wang, Neha Claire, Zuo-Guang Ye
Summary: A Bi(Zn1/2Ti1/2)O-3-PbZrO3-PbTiO3 ternary solid solution was synthesized to develop high-performance piezo-/ferroelectric materials, with the best properties found in the y = 0.15 series. This series showed improved dielectric constant, remnant polarization, Curie temperature, and coercive field, making it a promising material for high-power piezoelectric applications.
JOURNAL OF THE AMERICAN CERAMIC SOCIETY
(2022)
Article
Chemistry, Physical
Qiang Wang, Gang Niu, Ruobing Wang, Ren Luo, Zuo-Guang Ye, Jinshun Bi, Xi Li, Zhitang Song, Wei Ren, Sannian Song
Summary: This study presents significant enhancements in PCRAM electronic synapses based on materials engineering and pulse programming. The controllability of conductance is increased through carbon doping, while non-linear programmable pulse excitations lead to reliable synaptic potentiation and depression. Improved programmable pulse schemes are demonstrated, showing potential advantages in flexible programming and reliable data collection.
JOURNAL OF MATERIOMICS
(2022)
Article
Chemistry, Multidisciplinary
Guohua Dong, Yue Hu, Changqing Guo, Haijun Wu, Haixia Liu, Ruobo Peng, Dan Xian, Qi Mao, Yongqi Dong, Yanan Zhao, Bin Peng, Zhiguang Wang, Zhongqiang Hu, Junwei Zhang, Xueyun Wang, Jiawang Hong, Zhenlin Luo, Wei Ren, Zuo-Guang Ye, Zhuangde Jiang, Ziyao Zhou, Houbing Huang, Yong Peng, Ming Liu
Summary: This study presents a method for preparing self-assembled, epitaxial, ferroelectric nanosprings and demonstrates their super-scalability and full recovery capability.
ADVANCED MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Zenghui Liu, Hua Wu, Jian Zhuang, Gang Niu, Nan Zhang, Wei Ren, Zuo-Guang Ye
Summary: Bismuth-based piezo-/ferroelectric single crystals (BPSCs) show promising potential for high-temperature electromechanical applications due to their excellent piezoelectric performance and high Curie temperature. Recent research has focused on materials design, crystal growth, physical properties, crystal chemistry, and complex domain structures of BPSCs, providing a positive outlook for future applications.
Article
Acoustics
Zibo Jiang, Chenxue Hou, Chunlong Fei, Zhaoxi Li, Zuo-Guang Ye
Summary: This study investigates the relationship between composition segregation and ultrasonic transducer performance in lead magnesium niobate-lead titanate (PMN-PT) single crystals. The results show that changes in crystal composition significantly affect the piezoelectric coefficient and relative permittivity, but have minimal impact on the transducer bandwidth and center frequency. By using crystals of different compositions, similar transducer performance can be achieved, reducing material costs.
IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL
(2022)
Article
Multidisciplinary Sciences
Liyan Dai, Jinyan Zhao, Jingrui Li, Bohan Chen, Shijie Zhai, Zhongying Xue, Zengfeng Di, Boyuan Feng, Yanxiao Sun, Yunyun Luo, Ming Ma, Jie Zhang, Sunan Ding, Libo Zhao, Zhuangde Jiang, Wenbo Luo, Yi Quan, Jutta Schwarzkopf, Thomas Schroeder, Zuo-Guang Ye, Ya-Hong Xie, Wei Ren, Gang Niu
Summary: In this study, the remote epitaxy of BaTiO3 on germanium using a graphene intermediate layer was demonstrated, resulting in a highly heterogeneous epitaxial system. Graphene played an important role in surface passivation. The transferred BTO3-delta films possessed enhanced flexoelectric properties.
NATURE COMMUNICATIONS
(2022)
Article
Materials Science, Multidisciplinary
Ruikang Wang, Tianyi Yan, Chao Li, Wei Ren, Gang Niu, Zhuang-De Jiang, Chenying Wang, Ming Liu, Zuo-Guang Ye, Yijun Zhang
Summary: This study investigated the microstructure and solid-state reaction of Al2O3/ZnO nanolaminates using atomic layer deposition and post-annealing. The results show that the growth temperature and post-annealing temperature not only affect the crystallinity and preferred orientation of the nanocomposites, but also influence the interfacial diffusion and counter-diffusion of atoms, thereby affecting the solid-state reaction.
MATERIALS CHEMISTRY AND PHYSICS
(2022)
Article
Physics, Applied
Hao Yang, Jinyan Zhao, Wei Ren, Zuo-Guang Ye, K. B. Vinayakumar, Rosana A. Dias, Rui M. R. Pinto, Jian Zhuang, Nan Zhang
Summary: A sodium bismuth titanate-based thin film was prepared using the sol-gel spin coating method, which showed low dielectric loss and high remnant polarization. The film exhibited stable piezoelectric response at higher temperatures, and the fabricated piezoelectric device demonstrated a large macro-scale strain value.
APPLIED PHYSICS LETTERS
(2022)
Review
Materials Science, Multidisciplinary
Zenghui Liu, Hua Wu, Yi Yuan, Hongyan Wan, Zeng Luo, Pan Gao, Jian Zhuang, Jie Zhang, Nan Zhang, Jingrui Li, Yage Zhan, Wei Ren, Zuo-Guang Ye
Summary: This article reviews the recent progress in bismuth-based piezo-/ferroelectric perovskite materials, including material synthesis, doping effects, and chemical modifications. It also presents the developments of these materials for high-temperature electromechanical transduction applications and proposes possible solutions to existing issues.
CURRENT OPINION IN SOLID STATE & MATERIALS SCIENCE
(2022)
Article
Chemistry, Physical
Zhe Wang, Jinyan Zhao, Nan Zhang, Wei Ren, Kun Zheng, Yi Quan, Jian Zhuang, Yijun Zhang, Luyue Jiang, Lingyan Wang, Gang Niu, Ming Liu, Zhuangde Jiang, Yulong Zhao, Zuo-Guang Ye
Summary: Lead-free bismuth sodium titanate (BNT) ceramics with a composition of x = 3.5 demonstrate a large strain response of 0.61%. The coexistence of ferroelectric and relaxor domain structures, along with the substitution of antiferroelectric NN, contribute to the enhanced strain response. This study provides new insights into the interplay between mesoscopic domains and macroscopic electrical properties in BNT-based piezoceramics.
JOURNAL OF MATERIOMICS
(2023)
Article
Materials Science, Multidisciplinary
Kai Liu, Fafu Liu, Wu Zhang, Zhanming Dou, Weigang Ma, Chanatip Samart, Naohisa Takesue, Hua Tan, Pengyuan Fan, Zuo-Guang Ye, Haibo Zhang
Summary: (Na1/2Bi1/2)TiO3-based piezoelectric multilayer actuators (MLAs) have attracted attention as a replacement for lead-based piezoelectric devices due to environmental concerns. In this study, a grain orientation engineering approach was used to prepare a textured NBT-based MLA with high strain output and effective co-firing. The textured MLA achieved a high texturing degree and significantly higher strain performance compared to the non-textured counterpart. The effects of grain orientation engineering on mechanical properties and fracture behavior were analyzed.
Article
Chemistry, Physical
Vidhi Chauhan, Bi-Xia Wang, Zuo-Guang Ye
Summary: In this study, high-quality PbHfO3 ceramics were prepared via solid-state synthesis and its characteristics were investigated. It was found that PbHfO3 exhibited orthorhombic structure with antiparallel alignment of Pb2+ ions along the [001] directions. The polarization-electric field (P-E) relation of PbHfO3 at room temperature and in the intermediate phase temperature range were measured. The results showed that PbHfO3 had a high recoverable energy-storage density and efficiency at both room temperature and intermediate phase temperature.
Article
Materials Science, Multidisciplinary
Yanxing Zhang, Jiale Zhang, Nan Zhang, Laijun Liu, Alexei A. Bokov, Zuo-Guang Ye, Dawei Wang
Summary: This study reveals a hierarchical ordering in lead-based relaxor ferroelectric perovskites, enriching our understanding of the complex nature of the chemical ordering in these materials.
Article
Materials Science, Multidisciplinary
Zhen Wang, Zheyi An, Jian Zhuang, Fei Li, Wei Ren, Zuo-Guang Ye, Nan Zhang
Summary: In this study, neutron atomic pair distribution function (PDF) analysis was used to investigate the local-structural features of relaxor-ferroelectric materials at low temperatures. The results revealed that the existence of polar nanoregions (PNRs) is characterized by strong displacement correlation rather than structural symmetry. This finding provides a better understanding of the high-performance piezoelectric properties of these materials.
JOURNAL OF MATERIALS CHEMISTRY C
(2022)
Article
Materials Science, Multidisciplinary
Zenghui Liu, Zhixuan Guo, Hongyan Wan, Yi Yuan, Hao Yang, Hua Wu, Wei Ren, Zuo-Guang Ye
Summary: Lead zirconate (PZ)-based antiferroelectric (AFE) materials have limitations due to their ultrahigh critical electric field (EF). To overcome this, a bismuth-based perovskite, Bi(Zn2/3Nb1/3)O-3 (BZN), was introduced to PZ to form the PZ-BZN solid solution. Single crystals of this system were grown and investigated, revealing improved energy storage performance and a better understanding of the domain structure and origin of the intermediate (IM) phase in PZ-based AFE materials.
JOURNAL OF MATERIALS CHEMISTRY C
(2022)