Review
Engineering, Environmental
Xin Wang, Xiantong Yu, Jun Song, Weichun Huang, Yuanjiang Xiang, Xiaoyu Dai, Han Zhang
Summary: Antimonene, as an emerging 2D material discovered in 2015, has gained popularity for its unique optical and electronic properties. Theoretical and experimental studies have shown its remarkable semiconducting properties, making it promising for practical applications in various fields. Recent research has focused on its applications in nanophotonics, such as photodetectors, solar cells, photocatalysis, cancer therapy, and surface plasmon resonance sensors, indicating its potential for wider applications.
CHEMICAL ENGINEERING JOURNAL
(2021)
Review
Chemistry, Multidisciplinary
Xuchen Zheng, Siao Chen, Jinze Li, Han Wu, Chao Zhang, Danyan Zhang, Xi Chen, Yang Gao, Feng He, Lan Hui, Huibiao Liu, Tonggang Jiu, Ning Wang, Guoxing Li, Jialiang Xu, Yurui Xue, Changshui Huang, Chunying Chen, Yanbing Guo, Tong-Bu Lu, Dan Wang, Lanqun Mao, Jin Zhang, Yue Zhang, Lifeng Chi, Wanlin Guo, Xian-He Bu, Hongjie Zhang, Liming Dai, Yuliang Zhao, Yuliang Li
Summary: Graphdiyne (GDY), a two-dimensional all-carbon network with sp/sp(2)-hybridized structure, has shown great potential for innovation and development in various fields. GDY has attracted extensive attention from scientists due to its controlled growth, chemical and physical properties, and mechanisms that differ from traditional carbon materials. It has become one of the frontiers of chemistry and materials science and has generated numerous research achievements in the fundamental and applied study of carbon materials. The applications of GDY in catalysis, energy storage, photoelectronic, biomedicine, environmental science, life science, detectors, and material separation are comprehensively introduced in this review.
Article
Materials Science, Multidisciplinary
Qingyan Pan, Xinsheng Chen, Hao Li, Siqi Chen, Xuhan Zheng, Hui Liu, Bo Li, Yingjie Zhao
Summary: We report a crystalline two-dimensional benzotrithiophene-based graphdiyne material with good crystallinity and unique pore structure, showing semiconductor characteristics and high conductivity.
Review
Nanoscience & Nanotechnology
Xuezhi Ma, Nathan Youngblood, Xiaoze Liu, Yan Cheng, Preston Cunha, Kaushik Kudtarkar, Xiaomu Wang, Shoufeng Lan
Summary: This article discusses the method of changing the optical properties of 2D materials by engineering the photonic environment, emphasizing the importance of the interaction between the environment and the materials for efficiency. By modifying dielectric and metallic environments, the light-matter interaction of 2D materials can be effectively shaped.
Article
Nanoscience & Nanotechnology
Runhao Huang, Zhenhui Kou, Raul D. Rodriguez, Xusheng Wang, Yang Hou, Tao Wang, Tao Zhang
Summary: The two-dimensional layered carbon allotrope graphdiyne (GDY) is a promising material for solar energy utilization. However, the complex synthesis method and limited activity of metal-free materials hinder its practical applications. In this study, a silver-metalated GDY (Ag-GDY) photocatalyst was successfully synthesized using a facile and scalable wet-chemistry strategy. Ag-GDY exhibited excellent performance in the light-driven decomposition of antibiotics.
ACS APPLIED NANO MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Nan Gao, Hui Zeng, Xiaofang Wang, Yue Zhang, Shuai Zhang, Ruwen Cui, Meining Zhang, Lanqun Mao
Summary: Graphdiyne (GDY), a 2D carbon allotrope, demonstrates a new character in electrochemiluminescence (ECL) investigation with strong emission and potential for emerging applications in imaging and light-emitting devices.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Nanoscience & Nanotechnology
T. P. Rasmussen, P. A. D. Goncalves, Sanshui Xiao, Sebastian Hofferberth, N. Asger Mortensen, Joel D. Cox
Summary: By bending 2D materials into parabolic shapes to form waveguides, the field confinement associated with graphene plasmons can be significantly increased, leading to the formation of plasmonic waveguides. In 2D parabolic waveguides, the high field confinement of channel polaritons can enhance the spontaneous emission rate of quantum emitters near the parabolic vertex.
Review
Materials Science, Multidisciplinary
Ting Zhang, Yu-jing Wang, Ling-min Shi, Li-min Shi, Shou-ning Chai, Chi He
Summary: This review provides an introduction to the special physicochemical properties and main synthesis methods of Graphdiyne. It summarizes the theoretical and experimental studies on non-metal/metal atom doping and chemical group modification and discusses the challenges in its development.
NEW CARBON MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Jiaheng Hou, Lishui Sun, Qingyan Pan, Yingjie Zhao
Summary: Graphdiyne (GDY) is an exclusive carbon allotrope with a distinctive 2D structure, which has attracted great interest due to its excellent electronic properties. The porous nature and high specific surface area of GDY make it highly promising for various applications. However, the synthesis of GDY still faces many obstacles, and developing new synthesis methods for high-quality GDY is crucial. Therefore, this overview categorizes the reported synthesis techniques into three distinct approaches and provides valuable references for addressing the persistent challenges in GDY synthesis. In addition, an outlook sheds light on future research of GDY materials.
Review
Chemistry, Multidisciplinary
Naihua Miao, Zhimei Sun
Summary: Magnetic materials have long been a focus in materials physics and chemistry, with 2D magnets emerging as a promising family with atomically thin thickness for future applications in spintronic devices. Recent advancements in theory, simulations, and experiments have made notable progress in understanding and utilizing 2D magnets, particularly in van der Waals materials and heterojunctions. The discussion of possible directions for future investigation is expected to inspire increased interest in the development and applications of 2D magnets and spintronic devices.
WILEY INTERDISCIPLINARY REVIEWS-COMPUTATIONAL MOLECULAR SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Lan Hui, Yurui Xue, Yuxin Liu, Yuliang Li
Summary: The unique nanostructure of GDY provides active sites for hydrogen adsorption and facilitates the electron-transfer process, making it a superior metal-free efficient HER electrocatalyst with long-term durability compared to Pt/C.
Article
Nanoscience & Nanotechnology
Yihua Lu, Yunduo Yu, Xi Zhu, Min Wang
Summary: The study shows that B6C6N6-1 and B6C6N6-2 are stable 2D BCN structures with good thermal stability and mechanical stability, making them suitable for semiconductor and mechanical applications.
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES
(2021)
Article
Chemistry, Physical
Xiaoling Zhan, Huifang Kang, Feng Qian, Lanqing Xu, Yongping Zheng, Zhigao Huang
Summary: In this paper, cobalt-doped graphdiyne nanosheets were successfully synthesized by introducing transition metal cobalt into the alkynyl unit of graphdiyne using a bottom-up liquid-liquid interface synthesis method. The obtained nanosheets showed obvious room temperature ferromagnetism. Density function theory results indicated that cobalt-doped graphdiyne is a half-metallic material with a kagome lattice, and the embedded cobalt atoms are the source of magnetic moment. The special kagome structure exhibited flat band ferromagnetism, consistent with the experimental observations. The successful synthesis of cobalt-doped graphdiyne not only promotes the study of graphdiyne's magnetism, but also provides a new route for the experimental synthesis of kagome lattice materials.
JOURNAL OF ALLOYS AND COMPOUNDS
(2023)
Review
Chemistry, Multidisciplinary
Mengke Wang, Junmei Pu, Yi Hu, You Zi, Zheng-Guang Wu, Weichun Huang
Summary: Graphdiyne (GDY) is a promising material with rich chemical bonds, highly pi-conjugated structure, uniformly distributed pores, large surface area, and high inhomogeneity of charge distribution. This review highlights the synthetic strategies and surface/interface engineering methods for optimizing the nanostructures of GDY. The functionalization of GDY and its applications in various fields are comprehensively discussed.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Review
Chemistry, Multidisciplinary
Shuya Zhao, Zhaoyang Chen, Huimin Liu, Lu Qi, Zhiqiang Zheng, Xiaoyu Luan, Yaqi Gao, Runyu Liu, Jiayu Yan, Fanle Bu, Yurui Xue, Yuliang Li
Summary: Graphdiyne, a two-dimensional carbon material with both sp and sp2 hybridization, possesses unique properties such as alkyne-rich structures, large π conjugated system, uniform pores, specific unevenly-distributed surface charge, and incomplete charge transfer. These properties make it highly promising for practical applications in catalysis, energy conversion and storage, intelligent devices, life science, and photoelectric fields. Graphdiyne has become one of the hottest research frontiers in chemistry and materials science, leading to original and innovative results in fundamental and applied carbon materials research. Recent advancements have been made in the development of graphdiyne-based multiscale catalysts for nitrogen fixation and ammonia synthesis at room temperatures and ambient pressures. This review provides an updated synthesis of such catalysts and their applications in ammonia synthesis, highlighting the unique features of graphdiyne and discussing future challenges and perspectives.
Article
Computer Science, Artificial Intelligence
Weichun Huang, Yixue Yang, Xiaohui Huang, Zhiying Peng, Liyan Xiong
Summary: In recent years, a new fine-grained task called emotion-cause pair extraction (ECPE) has been proposed in sentiment analysis field, aiming to extract all emotions and their causes from a document. However, existing methods often ignore the relationship between emotion clauses and cause clauses. To address this, we propose an end-to-end framework that uses interactive attention and fusion mechanism to learn the relationship between emotions and causes, achieving better results than state-of-the-art baselines.
APPLIED INTELLIGENCE
(2023)
Article
Computer Science, Information Systems
Liyan Xiong, Hu Yi, Xiaohui Huang, Weichun Huang
Summary: This paper proposes an efficient network model for counting crowds in crowded scenes. The model achieves accurate counting of crowds with varying densities and scales through multi-scale contextual feature fusion and spatial channel attention mechanism. Experimental results show that the model outperforms many state-of-the-art methods in counting performance and generated density maps.
MULTIMEDIA TOOLS AND APPLICATIONS
(2023)
Article
Nanoscience & Nanotechnology
Jun Zhu, Hongyan Chen, You Zi, Mengke Wang, Weichun Huang
Summary: This study successfully synthesized uniform zero-dimensional bismuth quantum dots of different sizes and applied them in photoelectrochemical photodetection. The results showed that the fabricated bismuth quantum dot-based electrode exhibited suitable photoresponse and excellent photodetection performance. By optimizing the size, the best photoelectrochemical photoresponse behavior can be achieved.
Article
Materials Science, Multidisciplinary
Tianzhong Li, Jinyong Wang, Tongkai Chen, Swelm Wageh, Ahmed A. Al-Ghamdi, Jiangtian Yu, Zhongjian Xie, Han Zhang
Summary: In this study, a drug formulation based on lactic acid bacteria (LAB) was developed to produce reactive oxygen species (ROS) in tumors and induce host immunity. The LAB were modified with zeolitic imidazolate framework-67 (ZIF-67) and effectively delivered into tumor cells, leading to the generation of ROS upon light exposure. The bacterial hybrid induced tumor shrinkage through photodynamic therapy and stimulated inflammation to attract immune cells for cancer elimination.
SCIENCE CHINA-MATERIALS
(2023)
Article
Engineering, Biomedical
Xin Liu, Hongyi Qu, Lingwei Meng, Cong Wang, Qiuliang Wang
Summary: This paper proposes a new control method to solve the defects of traditional artificial heart pumps. By designing a sliding mode controller and a feedback adjustment mechanism, blood pulsatility is improved. The method also prevents regurgitation and suction phenomena through optimization of controller parameters.
JOURNAL OF MEDICAL AND BIOLOGICAL ENGINEERING
(2023)
Article
Physics, Applied
Shunzhong Chen, Lei Wang, Zili Zhang, Yaohui Wang, Hui Wang, Junsheng Cheng, Yinming Dai, Qiuliang Wang
Summary: The Institute of Electrical Engineering, Chinese Academy of Sciences has successfully developed a whole-body magnetic resonance imaging (MRI) superconducting magnet with a diameter of 800 mm and a magnetic field of 9.4 T in 2021. This study provides a systematic analysis and simulation of the real quench protection performance. Four successful quench protections during the energization process demonstrate the feasibility of the 'in-out-in' quench protection protocol for this superconducting magnet. The flexibility of the protocol to fit different MRI magnet designs is also confirmed by adjusting the quench trigger sequence through changing the heater thickness. The study validates the accuracy of the quench protection simulation method and code and discusses the limitations and reference value of the current quench protection for other MRI magnets.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2023)
Review
Chemistry, Multidisciplinary
Xiaobing Yan, Ying Zhao, Gang Cao, Xiaoyu Li, Chao Gao, Luan Liu, Shakeel Ahmed, Faizah Altaf, Hui Tan, Xiaopeng Ma, Zhongjian Xie, Han Zhang
Summary: In the past few decades, 2D layer materials have gained attention in materials science due to their unique structure and optoelectronic properties. However, limitations in material types and large-scale synthesis have restricted their application in the field. To overcome these limitations, the combination of organic molecular materials and 2D materials enables the synthesis of 2D organic materials with excellent optical and electrical properties, as well as the free design and large-scale synthesis of 2D materials. Furthermore, 2D organic materials show promising potential in developing sensors, biomedicine, and electronics, making them an important area of research.
Article
Engineering, Environmental
Chenyang Xing, Zihao Li, Shaohui Zhang, Jian Bang, Zhongjian Xie, Han Zhang, Zhengchun Peng
Summary: In order to address global freshwater scarcities, innovative materials are needed for the development of solar-powered interfacial desalination and purification technologies. This study utilizes polymeric phase inversion to develop PVA-based foam hydrogels with high porosity, compressibility, and rapid water transport. These materials also exhibit low water evaporation enthalpies and achieve high evaporation rates and energy efficiency under 1 sun irradiation.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Chemistry, Physical
Xiaohan Duan, Zhihao Liu, Zhongjian Xie, Ayesha Khan Tareen, Karim Khan, Bin Zhang, Han Zhang
Summary: Currently, numerous monoelemental two-dimensional materials, called Xenes, have been extensively studied and have shown great potential for applications in photoelectric and biomedicine fields. These materials have unique structural characteristics and excellent properties, including high optical response capability and large specific surface area. In particular, Xenes have diverse utilization as biosensors for nucleic acid sequencing, bioactive detection, and cancer diagnosis.
Review
Chemistry, Multidisciplinary
Karim Khan, Ayesha Khan Tareen, Muhammad Iqbal, Zhang Ye, Zhongjian Xie, Asif Mahmood, Nasir Mahmood, Han Zhang
Summary: MXenes are a novel and extensive class of 2D materials family, which consist of early transition metals based 2D carbides, nitrides and carbonitrides nanomaterials. MXenes possess distinctive surface chemistry, graphene like shape, metallic conductivity, high hydrophilicity, outstanding mechanical and thermal properties, redox capacity and are affordable with mass-produced nature, making them of tremendous scientific and technological significance.
Review
Chemistry, Multidisciplinary
You Zi, Yi Hu, Junmei Pu, Mengke Wang, Weichun Huang
Summary: With the rapid consumption of nonrenewable energy, solar energy is considered to be a promising solution to meet future energy requirements and mitigate environmental issues. The photoelectrochemical (PEC) device, which utilizes semiconductor nanostructure-based photocatalysts, is believed to be an energy-efficient and environmentally friendly way to utilize solar energy. This review provides a comprehensive summary of the recent progress in interface engineering of semiconductor nanostructures for PEC applications, as well as the challenges and future directions in the field of next-generation PEC devices.
Article
Physics, Applied
Wanshuo Sun, Yaohui Wang, Zili Zhang, Xiaolong Zhang, Lei Wang, Junsheng Cheng, Hongli Suo, Qiuliang Wang
Summary: In this study, a NbTi-Bi2223 hybrid low-resistive joint fabricated by the superconducting solder method was systematically investigated. The joint resistance and current capability under different applied magnetic fields were measured, and the resistance exhibited a near-linear relationship with the applied field. Beyond the superconducting properties, the allowed mechanical criteria for the Bi2223 tape in the joint were also briefly studied. A 1.3 GHz NMR design with a NbTi-Bi2223 hybrid low-resistive joint was shown as an application demonstration based on the above two properties. The attempt to obtain a lower resistance value by extending the joint length was unsuccessful, and the main source of resistance in NbTi-Bi2223 was studied. We aim to present an engineering-feasible NbTi-Bi2223 hybrid low-resistive joint to help improve the development of GHZ NMR.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2023)
Review
Chemistry, Multidisciplinary
Hongyan Chen, Mengke Wang, Weichun Huang
Summary: PbO, as a new emerging 2D material, has unique optical and electronic properties, making it promising for a wide range of applications in nanophotonics. This minireview summarizes the synthesis of PbO nanostructures and discusses the recent progress in optoelectronics/photonics applications based on PbO nanostructures, as well as the current challenges and future opportunities in this research area.
Article
Physics, Applied
Zili Zhang, Sikan Chen, Lei Wang, Hui Liu, Yan Liu, Yue Zhao, Hongli Suo, Qiuliang Wang
Summary: This paper presents a novel two-step procedure for measuring the critical current properties as a function of tensile stress. The proposed method eliminates the negative effect of the voltage tap used during the tensile procedure, allowing the determination of the actual irreversible degradation stress. The results show that the critical current value does not degrade until the stress reaches the 'inflection area' in the tensile curve. A feasible composite-material tensile model is established to explain this phenomenon. Fatigue measurements and EBSD experiments confirm the proposed model.
SUPERCONDUCTOR SCIENCE & TECHNOLOGY
(2023)
Article
Engineering, Environmental
Xinping Zhang, Yuxin Guo, Xiaoyang Liu, Shun-Yu Wu, Ya-Xuan Zhu, Shao-Zhe Wang, Qiu-Yi Duan, Ke-Fei Xu, Zi-Heng Li, Xiao-Yu Zhu, Guang-Yu Pan, Fu-Gen Wu
Summary: This study develops a nanotrigger HCFT for simultaneous photodynamic therapy and light-triggered ferroptosis therapy. The nanotrigger can relieve tumor hypoxia, induce enhanced photodynamic reaction, and facilitate the continuation of Fenton reaction, ultimately leading to lethal ferroptosis in tumor cells.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Olumide Bolarinwa Ayodele, Toyin Daniel Shittu, Olayinka S. Togunwa, Dan Yu, Zhen-Yu Tian
Summary: This study focused on the semihydrogenation of acetylene in an ethylene-rich stream using two alloyed Pt catalysts PtCu and PtCo. The PtCu catalyst showed higher activity and ethylene yield compared to PtCo due to its higher unoccupied Pt d-orbital density. This indicates that alloying Pt with Cu is more promising for industrial relevant SHA catalyst.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Guowei Chen, Wen-Cheng Chen, Yaozu Su, Ruicheng Wang, Jia-Ming Jin, Hui Liang, Bingxue Tan, Dehua Hu, Shaomin Ji, Hao-Li Zhang, Yanping Huo, Yuguang Ma
Summary: This study proposes an intramolecular dual-locking design for organic luminescent materials, achieving high luminescence efficiency and performance for deep-blue organic light-emitting diodes. The material also exhibits unique mechanochromic luminescence behavior and strong fatigue resistance.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Joren van Stee, Gregory Hermans, Jinu Joseph John, Koen Binnemans, Tom Van Gerven
Summary: This work presents a continuous solvent extraction method for the separation of cobalt and nickel in a millifluidic system using Cyphos IL 101 (C101) as the extractant. The optimal conditions for extraction performance and solvent properties were determined by investigating the effects of channel length, flow rate, and temperature. The performance of a developed manifold structure was compared to a single-channel system, and excellent separation results were achieved. The continuous separation process using the manifold structure resulted in high purity cobalt and nickel products.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Yan Xu, Jingai Jiang, Xinyi Lv, Hui Li, Dongliang Yang, Wenjun Wang, Yanling Hu, Longcai Liu, Xiaochen Dong, Yu Cai
Summary: A programmed gas release nanoparticle was developed to address the challenges in treating diabetic infected wounds. It effectively removes drug-resistant pathogens and remodels the wound microenvironment using NO and H2S. The nanoparticle can eliminate bacteria and promote wound healing through antibacterial and anti-inflammatory effects.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Tong Xia, Zhilin Xi, Lianquan Suo, Chen Wang
Summary: This study investigated a highly efficient coal dust suppressant with low initial viscosity and high adhesion-solidification properties. The results demonstrated that the dust suppressant formed a network of multiple hydrogen bonding cross-linking and achieved effective adhesion and solidification of coal dust through various chemical reactions.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Jinzhi Cai, Zhenshan Li
Summary: A density functional theory-based rate equation was developed to predict the gas-solid reaction kinetics of CaO carbonation with CO2 in calcium looping. The negative activation energy of CaO carbonation close to equilibrium was accurately predicted through experimental validation.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Jianxiong Chen, Fuhao Ren, Ningning Yin, Jie Mao
Summary: This study presents an economically efficient and easily implementable surface modification approach to enhance the high-temperature electrical insulation and energy storage performance of polymer dielectrics. The self-assembly of high-insulation-performance boron nitride nanosheets (BNNS) on the film surface through electrostatic interactions effectively impedes charge injection from electrodes while promoting charge dissipation and heat transfer.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Zijian Li, Zhaohui Yang, Shao Wang, Hongxia Luo, Zhimin Xue, Zhenghui Liu, Tiancheng Mu
Summary: This study reports a strategy for upgrading polyester plastics into value-added chemicals using electrocatalytic methods. By inducing the targeted transfer of *OH species, polyethylene terephthalate was successfully upgraded into potassium diformate with high purity. This work not only develops an excellent electrocatalyst, but also provides guidance for the design of medium entropy metal oxides.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Navneet Singh Shekhawat, Surendra Kumar Patra, Ashok Kumar Patra, Bamaprasad Bag
Summary: This study primarily focuses on developing a sulphur dyeing process at room temperature using bacterial Lysate, which is environmentally friendly, energy and cost effective, and sustainable. The process shows promising improvements in dye uptake and fastness properties.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Dengjia Shen, Hongyang Ma, Madani Khan, Benjamin S. Hsiao
Summary: This study developed cationic PVC nanofibrous membranes with high filtration and adsorption capability for the removal of bacteria and hexavalent chromium ions from wastewater. The membranes demonstrated remarkable performance in terms of filtration efficiency and maximum adsorption capacity. Additionally, modified nanofibrous membranes were produced using recycled materials and showed excellent retention rates in dynamic adsorption processes.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Xiaoyan Wang, Zhikun Wang, Ben Jia, Chunling Li, Shuangqing Sun, Songqing Hu
Summary: Inspired by photosystem II, self-supported Fe-doped NiCoP nanowire arrays modified with carboxylate were constructed to boost industrial-level overall water splitting by employing the concerted proton-coupled electron transfer mechanism. The introduction of Fe and carboxyl ligand led to improved catalytic activity for HER and OER, and NCFCP@NF exhibited long-term durability for overall water splitting.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Pengyao Yu, Ge Yang, Yongming Chai, Lubomira Tosheva, Chunzheng Wang, Heqing Jiang, Chenguang Liu, Hailing Guo
Summary: Thin LTA zeolite membranes were prepared through secondary growth of nano LTA seeds in a highly reactive gel, resulting in membranes with superior permeability and selectivity in gas separation applications.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Baiqin Zhou, Huiping Li, Ziyu Wang, Hui Huang, Yujun Wang, Ruichun Yang, Ranran Huo, Xiaoyan Xu, Ting Zhou, Xiaochen Dong
Summary: The use of machine learning to predict the performance of specific adsorbents in phosphate adsorption shows great promise in saving time and revealing underlying mechanisms. However, the small size of the dataset and insufficient detailed information limits the model training process and the accuracy of results. To address this, the study employs a fuzzing strategy that replaces detailed numeric information with descriptive text messages on the physiochemical properties of adsorbents. This strategy allows the recovery of discarded samples with limited information, leading to accurate prediction of adsorption amount, capacity, and kinetics. The study also finds that phosphate uptake by adsorbents is generally through physisorption, with some involvement of chemisorption. The framework established in this study provides a practical approach for quickly predicting phosphate adsorption performance in urgent scenarios, using easily accessible information.
CHEMICAL ENGINEERING JOURNAL
(2024)
Article
Engineering, Environmental
Paula Alejandra Lamprea Pineda, Joren Bruneel, Kristof Demeestere, Lisa Deraedt, Tex Goetschalckx, Herman Van Langenhove, Christophe Walgraeve
Summary: This study evaluates the use of four esterified fatty acids and three vegetable oils as absorption liquids for hydrophobic VOCs. The experimental results show that isopropyl myristate is the most efficient liquid for absorbing the target VOCs.
CHEMICAL ENGINEERING JOURNAL
(2024)