Strong and Tough Supramolecular Covalent Adaptable Networks with Room‐Temperature Closed‐Loop Recyclability

Anti‐freezing Hydrogel Electrolyte with Ternary Hydrogen Bonding for High Performance zinc‐ion Batteries

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Closing the “One Monomer–Two Polymers–One Monomer” Loop via Orthogonal (De)polymerization of a Lactone/Olefin Hybrid

(2022) Changxia Shi et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Designed from Biobased Materials for Recycling: Imine‐Based Covalent Adaptable Networks

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Hydrogen‐Bonding Affords Sustainable Plastics with Ultrahigh Robustness and Water‐Assisted Arbitrarily Shape Engineering

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Redesigned Hybrid Nylons with Optical Clarity and Chemical Recyclability

(2022) Robin M. Cywar et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Mechanically Robust Supramolecular Plastics with Energy-Saving and Highly Efficient Closed-Loop Recyclability

(2022) Xingyuan Lu et al.   MACROMOLECULES

A Chemically Recyclable Crosslinked Polymer Network Enabled by Orthogonal Dynamic Covalent Chemistry

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Sustainable polyesters via direct functionalization of lignocellulosic sugars

(2022) Lorenz P. Manker et al.   Nature Chemistry

Circularity in mixed-plastic chemical recycling enabled by variable rates of polydiketoenamine hydrolysis

(2022) Jeremy Demarteau et al.   Science Advances

Closed‐Loop Recycling of Poly(Imine‐Carbonate) Derived from Plastic Waste and Bio‐based Resources

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Circularly Recyclable Polymers Featuring Topochemically Weakened Carbon–Carbon Bonds

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Mechano-responsive hydrogen-bonding array of thermoplastic polyurethane elastomer captures both strength and self-healing

(2021) Youngho Eom et al.   Nature Communications

Closed-loop recycling of polyethylene-like materials

(2021) Manuel Häußler et al.   NATURE

Hybrid monomer design for unifying conflicting polymerizability, recyclability, and performance properties

(2021) Changxia Shi et al.   Chem

Healable and Recyclable Elastomers with Record‐High Mechanical Robustness, Unprecedented Crack Tolerance, and Superhigh Elastic Restorability

(2021) Zequan Li et al.   ADVANCED MATERIALS

O‐to‐S Substitution Enables Dovetailing Conflicting Cyclizability, Polymerizability, and Recyclability: Dithiolactone vs. Dilactone

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Fast Reprocessing of Acetal Covalent Adaptable Networks with High Performance Enabled by Neighboring Group Participation

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Olefin metathesis-based chemically recyclable polymers enabled by fused-ring monomers

(2021) Devavrat Sathe et al.   Nature Chemistry

Chemically recyclable thermoplastics from reversible-deactivation polymerization of cyclic acetals

(2021) Brooks A. Abel et al.   SCIENCE

The global threat from plastic pollution

(2021) Matthew MacLeod et al.   SCIENCE

Biobased High-Performance Aromatic–Aliphatic Polyesters with Complete Recyclability

(2021) Yi-Min Tu et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Design principles for intrinsically circular polymers with tunable properties

(2021) Changxia Shi et al.   Chem

Reshapeable, rehealable and recyclable sensor fabricated by direct ink writing of conductive composites based on covalent adaptable network polymers

(2021) Xu He et al.   International Journal of Extreme Manufacturing

Network Design to Control Polyimine Vitrimer Properties: Physical Versus Chemical Approach

(2020) Raymond Hajj et al.   MACROMOLECULES

Chemical recycling to monomer for an ideal, circular polymer economy

(2020) Geoffrey W. Coates et al.   Nature Reviews Materials

Remalleable, Healable, and Highly Sustainable Supramolecular Polymeric Materials Combining Superhigh Strength and Ultrahigh Toughness

(2020) Wenwen Niu et al.   ACS Applied Materials & Interfaces

Tough and Multi‐Recyclable Cross‐Linked Supramolecular Polyureas via Incorporating Noncovalent Bonds into Main‐Chains

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Resilient yet entirely degradable gelatin-based biogels for soft robots and electronics

(2020) Melanie Baumgartner et al.   NATURE MATERIALS

Catalyst-Free Metathesis of Cyclic Acetals and Spirocyclic Acetal Covalent Adaptable Networks

(2020) Shuangjian Yu et al.   ACS Macro Letters

Geminal Dimethyl Substitution Enables Controlled Polymerization of Penicillamine-Derived β-Thiolactones and Reversed Depolymerization

(2020) Wei Xiong et al.   Chem

Flexible Self‐Repairing Materials for Wearable Sensing Applications: Elastomers and Hydrogels

(2020) Shaonan Li et al.   MACROMOLECULAR RAPID COMMUNICATIONS

Acylsemicarbazide Moieties with Dynamic Reversibility and Multiple Hydrogen Bonding for Transparent, High Modulus, and Malleable Polymers

(2020) Daihua Fu et al.   MACROMOLECULES

Predicted growth in plastic waste exceeds efforts to mitigate plastic pollution

(2020) Stephanie B. Borrelle et al.   SCIENCE

100th Anniversary of Macromolecular Science Viewpoint: Toward Catalytic Chemical Recycling of Waste (and Future) Plastics

(2020) Joshua C. Worch et al.   ACS Macro Letters

Degradable and Fully Recyclable Dynamic Thermoset Elastomer for 3D‐Printed Wearable Electronics

(2020) Yifan Guo et al.   ADVANCED FUNCTIONAL MATERIALS

Proteinaceous Fibers with Outstanding Mechanical Properties Manipulated by Supramolecular Interactions

(2020) Jing Sun et al.   CCS Chemistry

Recyclable 3D Printing of Polyimine-Based Covalent Adaptable Network Polymers

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Integrating Sacrificial Bonds into Dynamic Covalent Networks toward Mechanically Robust and Malleable Elastomers

(2019) Yingjun Liu et al.   ACS Macro Letters

Closed-loop recycling of plastics enabled by dynamic covalent diketoenamine bonds

(2019) Peter R. Christensen et al.   Nature Chemistry

Internal Catalysis in Covalent Adaptable Networks: Phthalate Monoester Transesterification As a Versatile Dynamic Cross-Linking Chemistry

(2019) Maarten Delahaye et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Poly(oxime–ester) Vitrimers with Catalyst-Free Bond Exchange

(2019) Changfei He et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Adaptable Crosslinks in Polymeric Materials: Resolving the Intersection of Thermoplastics and Thermosets

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Mutually-complementary structure design towards highly stretchable elastomers with robust strength and autonomous self-healing property

(2019) Bo Wu et al.   POLYMER

Photopolymerized Triazole-Based Glassy Polymer Networks with Superior Tensile Toughness

(2018) Han Byul Song et al.   ADVANCED FUNCTIONAL MATERIALS

Recyclable, Strong, and Highly Malleable Thermosets Based on Boroxine Networks

(2018) William A. Ogden et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Reprocessable Acid-Degradable Polycarbonate Vitrimers

(2018) Rachel L. Snyder et al.   MACROMOLECULES

A synthetic polymer system with repeatable chemical recyclability

(2018) Jian-Bo Zhu et al.   SCIENCE

Brønsted-Acid-Catalyzed Exchange in Polyester Dynamic Covalent Networks

(2018) Jeffrey L. Self et al.   ACS Macro Letters

Rehealable, fully recyclable, and malleable electronic skin enabled by dynamic covalent thermoset nanocomposite

(2018) Zhanan Zou et al.   Science Advances

Colorless, Transparent, Robust, and Fast Scratch-Self-Healing Elastomers via a Phase-Locked Dynamic Bonds Design

(2018) Yue Lai et al.   ADVANCED MATERIALS

Towards Dynamic but Supertough Healable Polymers through Biomimetic Hierarchical Hydrogen-Bonding Interactions

(2018) Yan Song et al.   ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

An integrated self-healable electronic skin system fabricated via dynamic reconstruction of a nanostructured conducting network

(2018) Donghee Son et al.   Nature Nanotechnology

Robust, Fire-Safe, Monomer-Recovery, Highly Malleable Thermosets from Renewable Bioresources

(2018) Sheng Wang et al.   MACROMOLECULES

Recyclable and Malleable Epoxy Thermoset Bearing Aromatic Imine Bonds

(2018) Shou Zhao et al.   MACROMOLECULES

Toward Infinitely Recyclable Plastics Derived from Renewable Cyclic Esters

(2018) Xiaoyan Tang et al.   Chem

Chemically recyclable polymers: a circular economy approach to sustainability

(2017) Miao Hong et al.   GREEN CHEMISTRY

Oxime-Based and Catalyst-Free Dynamic Covalent Polyurethanes

(2017) Wen-Xing Liu et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Silyl Ether as a Robust and Thermally Stable Dynamic Covalent Motif for Malleable Polymer Design

(2017) Yoshio Nishimura et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Effect of Sterics and Degree of Cross-Linking on the Mechanical Properties of Dynamic Poly(alkylurea–urethane) Networks

(2017) Longhe Zhang et al.   MACROMOLECULES

50th Anniversary Perspective: There Is a Great Future in Sustainable Polymers

(2017) Deborah K. Schneiderman et al.   MACROMOLECULES

Rehealable imide–imine hybrid polymers with full recyclability

(2017) Xingfeng Lei et al.   Journal of Materials Chemistry A

Production, use, and fate of all plastics ever made

(2017) Roland Geyer et al.   Science Advances

Chemical recycling of waste plastics for new materials production

(2017) AliReza Rahimi et al.   Nature Reviews Chemistry

Repairable Woven Carbon Fiber Composites with Full Recyclability Enabled by Malleable Polyimine Networks

(2016) Philip Taynton et al.   ADVANCED MATERIALS

Sustainable polymers from renewable resources

(2016) Yunqing Zhu et al.   NATURE

Mechanically Activated, Catalyst-Free Polyhydroxyurethane Vitrimers

(2015) David J. Fortman et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Enhancing Mechanical Performance of a Covalent Self-Healing Material by Sacrificial Noncovalent Bonds

(2015) James A. Neal et al.   JOURNAL OF THE AMERICAN CHEMICAL SOCIETY

Completely recyclable biopolymers with linear and cyclic topologies via ring-opening polymerization of γ-butyrolactone

(2015) Miao Hong et al.   Nature Chemistry

Plastic waste inputs from land into the ocean

(2015) J. R. Jambeck et al.   SCIENCE

Heat- or Water-Driven Malleability in a Highly Recyclable Covalent Network Polymer

(2014) Philip Taynton et al.   ADVANCED MATERIALS

Recyclable, Strong Thermosets and Organogels via Paraformaldehyde Condensation with Diamines

(2014) J. M. Garcia et al.   SCIENCE

Silica-Like Malleable Materials from Permanent Organic Networks

(2011) D. Montarnal et al.   SCIENCE

Covalent Adaptable Networks (CANs): A Unique Paradigm in Cross-Linked Polymers

(2010) Christopher J. Kloxin et al.   MACROMOLECULES