Journal
ACS APPLIED MATERIALS & INTERFACES
Volume -, Issue -, Pages -Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c16681
Keywords
origami metamaterials; triboelectric materials; mechanoelectrical multistability; sensing; energy harvesting
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This study reports origami tribo-metamaterials that use origami-enabled, tubular metamaterials to trigger triboelectric pairs for mechanoelectrical multistability. The octagonal origami unit with a triboelectric pair of fluorinated ethylene propylene-paper achieved a peak open-circuit voltage of 206.4V, a short-circuit current of 4.66 mu A, a transferred charge of 0.38 mu C, and a maximum instantaneous output power density of 0.96 mu W/cm2.
The emerging mechanical functional metamaterials reported with promising mechanoelectrical characteristics bring increasing attention to structurally functional materials. It is essential to deploy mechanical metamaterials in energy materials for effective triggering and controllable mechanoelectrical response. This study reports origami tribo-metamaterials (OTMs) that design triboelectric materials in the origami-enabled, tubular metamaterials. The octagonal, hexagonal, and conical origami units are deployed as the metamaterial substrates to trigger the triboelectric pairs for mechanoelectrical multistability. For the octagonal OTM configuration with the triboelectric pair of fluorinated ethylene propylene-paper, the peak open-circuit voltage, short-circuit current, and transferred charge are obtained as 206.4 V, 4.66 mu A, and 0.38 mu C, respectively, and the maximum instantaneous output power density is 0.96 mu W/cm2 with the load resistance of 20 M omega. The OTM takes advantage of the origami metamaterials to obtain the multistable force-displacement response as effective stimuli for the triboelectric materials, which leads to tunable mechanoelectrical performance for speed and weight sensing and energy harvesting. The proposed OTM not only offers a strategy to structurally design energy materials to achieve desirable mechanoelectrical response, but also provides a guideline for the applications of mechanical functional metamaterials in practice.
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