4.8 Article

Observation of Coexisting Dirac Bands and Moire Flat Bands in Magic-Angle Twisted Trilayer Graphene

Journal

ADVANCED MATERIALS
Volume 34, Issue 42, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202205996

Keywords

Dirac fermions; flat bands; magic-angle twisted trilayer graphene; moire patterns

Funding

  1. National Key R&D program of China [2020YFA0309601, 2017YFA0305400]
  2. National Natural Science Foundation of China [12174257, 12074176, 62122036, 62034004, 61921005, 61974176, 12104304]
  3. Strategic Priority Research Program of the Chinese Academy of Sciences [XDB44000000]
  4. AIQ foundation
  5. International Postdoctoral Exchange Fellowship Program (Talent-Introduction Program) [YJ20200126]
  6. China Postdoctoral Science Foundation [2021M692131]
  7. ShanghaiTech University

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Magic-angle twisted trilayer graphene (MATTG) has shown rich and unique properties, including superconductivity and distinct band structure. Experimental measurements reveal the coexistence of different bands in MATTG, which is crucial for further understanding its unconventional superconductivity.
Moire superlattices that consist of two or more layers of 2D materials stacked together with a small twist angle have emerged as a tunable platform to realize various correlated and topological phases, such as Mott insulators, unconventional superconductivity, and quantum anomalous Hall effect. Recently, magic-angle twisted trilayer graphene (MATTG) has shown both robust superconductivity similar to magic-angle twisted bilayer graphene and other unique properties, including the Pauli-limit violating and re-entrant superconductivity. These rich properties are deeply rooted in its electronic structure under the influence of distinct moire potential and mirror symmetry. Here, combining nanometer-scale spatially resolved angle-resolved photoemission spectroscopy and scanning tunneling microscopy/spectroscopy, the as-yet unexplored band structure of MATTG near charge neutrality is systematically measured. These measurements reveal the coexistence of the distinct dispersive Dirac band with the emergent moire flat band, showing nice agreement with the theoretical calculations. These results serve as a stepstone for further understanding of the unconventional superconductivity in MATTG.

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