4.8 Article

Stable and Salt-Resistant Janus Evaporator Based on Cellulose Composite Aerogels from Waste Cotton Fabric

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 14, Issue 36, Pages 41114-41121

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c12750

Keywords

solar steam generation; waste cotton fabric; Janus evaporator; cellulose aerogel; desalination

Funding

  1. National Natural Science Foundation of China [51973027, 61902357, 52003044]
  2. Fundamental Research Funds for the Central Universities [2232020A-08, 2232020D-12]
  3. International Cooperation Fund of Science and Technology Commission of Shanghai Municipality [21130750100]
  4. Chang Jiang Scholars Program
  5. Innovation Program of Shanghai Municipal Education Commission [2019-01-07-00-03-E00023]
  6. Shang-hai Sailing Program [19YF1400700]
  7. Young Elite Scientists Sponsorship Program by CAST
  8. DHU Distinguished Young Professor Program
  9. Graduate Student Innovation Fund of Donghua University [CUSF-DH-D-2022039]

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This study reports on a dual-sided solar evaporator made with cellulose composite aerogels, which shows potential for seawater desalination and wastewater purification.
Solar steam generation has been considered a promising approach for using renewable solar energy to produce clean water from seawater and wastewater. It shows great potential for alleviating water shortages. However, salt accumulation and system longevity are challenges which impede the widespread use of evaporators. Tins paper reports a stable Janus evaporator with thickness controllable hydrophilic and hydrophobic layers based on cellulose composite aerogels, which were extracted from waste cotton fabric by a two-step freeze-drying process. The obtained glutaraldehyde cross-linked carbon nanotubes/cellulose Janus aerogel exhibited an attractive solar steam generation rate of 1.81 kg.m(-2).h(-1) and a light-to-vapor efficiency of up to 92.5% in 1 sun illumination. Moreover, the Janus solar steam generator could pledge stable and sustainable solar-driven water evaporation performance within a 10 h test, showing a high salt-resistant property in simulated seawater. In addition, the developed solar evaporator also had a good purification effect on dye wastewater. These findings suggest its potential ability for seawater desalination and wastewater purification.

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