4.8 Article

Enhanced Thermo-optical Response by Means of Anapole Excitation

Journal

JOURNAL OF PHYSICAL CHEMISTRY LETTERS
Volume 13, Issue 26, Pages 6230-6235

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.2c00870

Keywords

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Funding

  1. Spanish national project INMUNOTERMO [PGC2018-096649-B-I]
  2. UK Leverhulme Turst [RPG-2018-384]
  3. Ministry of Science of Spain for his FPI grant
  4. Ramon y Cajal Fellowship [RYC-2016-20831]

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This study proposes a spectrally tunable anapole nanoheater based on a dielectric anapole resonator. It can control the light-matter interaction and shift the thermal response from the shortwave infrared range to the near-infrared range.
ABSTRACT: High refractive index (HRI) dielectric nanostructures offer a versatile platform to control the light-matter interaction at the nanoscale as they can easily support electric and magnetic modes with low losses. An additional property that makes them extraordinary is that they can support low radiative modes, so-called anapole modes. In this work, we propose a spectrally tunable anapole nanoheater based on the use of a dielectric anapole resonator. We show that a gold ring nanostructure, a priori nonresonant, can be turned into a resonant unit by just filling its hole with an HRI material supporting anapole modes, resulting in a more efficient nanoheater able to amplify the photothermal response of the bare nanoring. As proof of concept, we perform a detailed study of the thermoplasmonic response of a gold nanoring used as heating source and a silicon disk, designed to support anapole modes, located in its center acting as an anapolar resonator. Furthermore, we utilize the anapole excitation to easily shift the thermal response of these structures from the shortwave infrared range to the nearinfrared range.

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