Article
Environmental Sciences
Jeison Manuel Arroyave, Marcelo Avena, Wenfeng Tan, Mingxia Wang
Summary: This article investigates the adsorption-desorption kinetics of phosphate on goethite using ATR-FTIR spectroscopy, providing new insights and experimental methods for understanding the behavior of pollutants with phosphonic or phosphinic moieties in the environment.
Article
Engineering, Environmental
Vanessa F. D. Martins, Carlos Miguel, Jonathan C. Goncalves, Alirio E. Rodrigues, Luis M. Madeira
Summary: This study developed and implemented a one-dimensional heterogeneous dynamic fixed-bed model for CO2 capture at high temperatures. The model successfully predicted the equilibrium and kinetics of CO2 adsorption on a K-promoted hydrotalcite. The model considered two different adsorption sites and incorporated a change in activation energy to explain the observed capacity loss. The model was validated under wet conditions, making it more robust for process optimization and industrial design.
CHEMICAL ENGINEERING JOURNAL
(2022)
Article
Chemistry, Multidisciplinary
Lisi Liang, Jiayu Mi, Linbo Li, Xihong He, Wenlong Guo
Summary: The Al-La hybrid gel, constructed using a novel acid-catalyzed sol-gel formation process, showed high fluoride ion adsorption efficiency and capacity. Systematic investigations on the properties, optimal adsorption conditions, synthetic principle, and adsorption mechanism of the material confirmed its excellent adsorption performance.
Article
Chemistry, Multidisciplinary
Abdulrahman Abu-Nada, Ahmed Abdala, Gordon McKay
Summary: Graphene oxide (GO) was successfully synthesized and characterized in this study, showing excellent adsorption capability for removing Sr (II) from aqueous solutions. The adsorption equilibrium and kinetic results were in agreement with the Langmuir isotherm model and the pseudo-second-order kinetic model. The maximum strontium adsorption capacity reached 131.4 mg/g, suggesting potential applications in wastewater treatment.
Article
Electrochemistry
Tamas Pajkossy
Summary: A theory is proposed to analyze voltammograms and dynamic electrochemical impedance spectroscopy (dEIS) measurements of diffusion-hindered adsorption processes. The theory allows for the calculation of adsorption kinetics and isotherm parameters from a set of voltammograms taken at different scan-rates. The theory also includes the analysis of high frequency impedance spectra measured during potential scans. The presented theory synthesizes previous theories on diffusion-controlled charge transfer and adsorption, and supports the determination of rate coefficients as a function of electrode potential using fast dEIS measurements.
ELECTROCHIMICA ACTA
(2023)
Article
Biochemistry & Molecular Biology
Nikolay S. Chirkov, Shi-Yow Lin, Alexander Michailov, Reinhard Miller, Boris A. Noskov
Summary: The interactions between DNA and lysozyme in the surface layer were studied using various experimental methods. Unlike the case with a monolayer of cationic synthetic polyelectrolyte, no continuous network of DNA/lysozyme complexes was formed. The weaker interactions between lysozyme and DNA led to the formation of more disordered aggregates at high lysozyme concentrations in the surface layer.
INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES
(2022)
Article
Chemistry, Physical
Paola S. Pauletto, Sabrina F. Lutke, Guilherme L. Dotto, Nina Paula G. Salau
Summary: The study investigates the simultaneous adsorption of paracetamol and nimesulide using activated carbon, revealing a displacement phenomenon where nimesulide molecules replace active sites previously occupied by paracetamol. The higher affinity between AC and nimesulide is attributed to the more hydrophobic nature of nimesulide. The thermodynamic analysis suggests exothermic, favorable, and spontaneous adsorption with low adsorption energies supporting physisorption.
JOURNAL OF MOLECULAR LIQUIDS
(2021)
Article
Chemistry, Multidisciplinary
Jiang Li, Joakim Halldin Stenlid, Thomas Ludwig, Philomena Schlexer Lamoureux, Frank Abild-Pedersen
Summary: Accurate theoretical simulation of electrochemical activation barriers is crucial for understanding electrocatalysis. By developing an analytical approach based on charge conservation and decoupled potential energy surfaces, we successfully simulated the Pt-catalyzed alkaline hydrogen evolution reaction with consideration of solvent thermal fluctuations, showing the significant impact of water-metal distances on charge transfer barriers.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2021)
Article
Chemistry, Applied
Yan-Hua Fan, Ya-Xin Li, Wen-Jie Zhu, Yan Bai, Dong-Bin Dang
Summary: In this study, the adsorption performances of four 3D polyoxometalate-based metal-organic frameworks (POMOFs) on organic dyes were systematically studied. The results showed that these compounds exhibited highly sensitive selective adsorption behavior towards the cationic dye methylene blue. The study provides a new idea for the adsorption and separation of cationic dyes in wastewater by constructing materials with a large amount of charge on the surface.
Article
Chemistry, Physical
Richika Ganjoo, Chandrabhan Verma, Ashish Kumar, M. A. Quraishi
Summary: The most effective corrosion inhibitors are organic compounds, especially heterocyclic ones, with polar functional groups, nonbonding electrons, and multiple bonds. Dyes efficiently bind to metal surfaces through their electron-rich spots, known as adsorption centers, and have excellent anticorrosive properties. This review work focuses on the interfacial adsorption of dye molecules and how it negatively affects metallic corrosion, using the Langmuir isotherm model to block the active sites.
ADVANCES IN COLLOID AND INTERFACE SCIENCE
(2023)
Article
Environmental Sciences
Masahiro Umehara, Yoshiaki Kumamoto, Kenta Mukai, Akira Isogai
Summary: The adsorption isotherms, kinetics, and thermodynamics of fluoride ions (F-) on FeOOH powders in water were studied. The results showed that FeOOH/TOCN powder is an excellent and efficient F- adsorbent in water. The adsorption of F- on FeOOH initially formed a monolayer through physical adsorption, and the adsorption kinetics followed the pseudo-second-order model. The thermodynamic analysis indicated that the adsorption process was spontaneous in water.
ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
(2023)
Article
Engineering, Chemical
Stephen T. Castonguay, Pratanu Roy, Yunwei Sun, Sylvie Aubry, Brandon Foley, Elizabeth A. Glascoe, Hom N. Sharma
Summary: A sorption and diffusion model is developed to simulate complex sorption processes in multi-material systems. The model uses a mobile-immobile decomposition of the vapor concentration, with different modes representing mobile and immobilization processes. It can simulate five types of sorption and incorporate additional dynamics compared to thermodynamic equilibrium-based models. The model is solved using finite element method and backward Euler method, with four different materials parameterized and demonstrated in examples.
CHEMICAL ENGINEERING SCIENCE
(2023)
Article
Physics, Fluids & Plasmas
Hiroki Yamamoto, Shingo Ichiki, Daichi Yanagisawa, Katsuhiro Nishinari
Summary: This paper proposes a two-lane model with interactions between the lanes and investigates both bidirectional and unidirectional flows. Theoretical expressions for the global density of the system in the steady state are obtained through mean-field analyses, and it is found that the (2 x 2)-cluster mean-field analysis approximates the simulation results well. The phenomena are explained qualitatively through a simple analysis of correlations. These findings provide informative suggestions for actual traffic systems.
Article
Engineering, Chemical
Pratanu Roy, Stephen T. Castonguay, Jennifer M. Knipe, Yunwei Sun, Elizabeth A. Glascoe, Hom N. Sharma
Summary: This work explores the modeling and characterization of diffusive moisture transport coupled with kinetic Langmuir adsorption in a multi-material system. The finite volume method with an implicit Euler time-stepping scheme is used to solve the coupled unsteady diffusion-sorption equations. A level set framework with a smoothed Heaviside function is employed to handle moisture concentration and flux conditions at material interfaces, allowing for the simulation of complex 3D shapes.
CHEMICAL ENGINEERING SCIENCE
(2022)
Article
Engineering, Environmental
S. Aguirre-Contreras, R. Leyva-Ramos, R. Ocampo-Perez, C. G. Aguilar-Madera, J. V. Flores-Cano, N. A. Medellin-Castillo
Summary: The mathematical modeling of the dynamic adsorption of 8-Hydroxyquinoline on activated carbon in batch and fixed-bed adsorbers is described in this study. The model considers mass transport phenomena and includes axial dispersion, convective transport, intraparticle diffusion mechanisms, and adsorption on the active site. A methodology based on adsorption equilibrium and rate studies is proposed to solve the model, without considering fitting the mass transport parameters for breakthrough curve prediction, which is an important advancement in fixed-bed column design. The equilibrium results show that 8-HQ adsorbs onto activated carbon through dispersive and hydrophobic interactions, with a mass adsorbed of 454 mg g-1. The kinetic study reveals that achieving equilibrium is faster under turbulent stirring regime, and intraparticle transport is governed by surface diffusion. By using information obtained from the batch regime, the packed bed behavior can be interpreted and predicted in a wide range of operational conditions with an error of 10.6% in breakthrough point prediction.
JOURNAL OF WATER PROCESS ENGINEERING
(2023)
Article
Nanoscience & Nanotechnology
Shahinur Acter, Mark Louis P. Vidallon, Simon Crawford, Rico F. Tabor, Boon Mian Teo
Summary: The study found that the size of polydopamine bowl-shaped mesoporous nanoparticles significantly affects their cellular internalization efficiency, and the size of nanoparticles also regulates the pathways of cellular internalization.
ACS APPLIED NANO MATERIALS
(2021)
Article
Chemistry, Physical
Johan Larsson, Ashley P. Williams, Marie Wahlgren, Lionel Porcar, Stefan Ulvenlund, Tommy Nylander, Rico F. Tabor, Adrian Sanchez-Fernandez
Summary: Recent studies have demonstrated that the rheological properties of systems formed by the self-assembly of long tail sugar-based surfactants into worm-like micelles can be tuned by subtle modifications of the surfactant monomer's molecular characteristics. The anomeric configuration of the surfactant was found to induce significant changes in nanostructure and rheology, with shear-thinning behavior relating to the re-arrangement of worm-like micelles. These findings provide a detailed mechanism by which sugar-based surfactants control the rheology of the fluid, offering potential for future studies in this area.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Physical
Mark Louis P. Vidallon, Luke W. Giles, Matthew J. Pottage, Calum S. G. Butler, Simon A. Crawford, Alexis Bishop, Rico F. Tabor, Liliana de Campo, Boon Mian Teo
Summary: The study utilized neutron scattering techniques to observe the phase transition of polydopamine-shelled perfluorocarbon emulsion droplets into microbubbles upon heating, showing that the transition temperatures are higher than the boiling points of pure liquid perfluorocarbons. Analysis and model fitting of neutron scattering data allowed monitoring of droplet size distributions at different temperatures, providing valuable insights into the transformation of these emulsion droplet systems.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Alexandra Semenova, Mark Louis P. Vidallon, Bart Follink, Paul L. Brown, Rico F. Tabor
Summary: A novel procedure for the synthesis of polyethylenimine (PEI)-silica nanocomposite particles with high adsorption capacities has been developed based on an emulsion templating concept. The resulting composite showed exceptional chelating properties for charged species and demonstrated great potential in various industries. By modulating emulsification conditions, the production of smaller particles was achieved, further enhancing the binding capacities for copper ions.
Article
Chemistry, Physical
Thomas M. McCoy, Alexander J. Armstrong, Jackson E. Moore, Stephen A. Holt, Rico F. Tabor, Alexander F. Routh
Summary: This study investigates the spontaneous adsorption of graphene oxide (GO) sheets at the air-water interface using X-ray reflectivity (XRR) measurements. It is found that GO sheets do not spontaneously adsorb at the air-water interface, but can be driven to the surface when incorporated with surfactant molecules at optimal ratios. However, excessive surfactant can inhibit GO surface adsorption.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2022)
Article
Chemistry, Physical
Zhenzhen Lu, Luke W. Giles, Boon M. Teo, Rico F. Tabor
Summary: In this study, Au NPs were successfully synthesized using a sustainable method with carbon dots serving as both reducing agent and stabilizer. The reduction mechanism of Au3+ was investigated by studying the effects of different functional groups in the carbon dots, leading to the observation of various morphologies of Au NPs.
COLLOID AND INTERFACE SCIENCE COMMUNICATIONS
(2022)
Article
Chemistry, Physical
Geosmin A. A. Turpin, Rico F. F. Tabor, Michaela M. H. Wawryk
Summary: In this study, poly(dimethylsiloxane) (PDMS) was treated with a combination of air-plasma (P), strain (S), and relaxation (R) to create diverse surface structures. It was found that the surface chemistry directed water more strongly than the physical structures.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2022)
Article
Chemistry, Multidisciplinary
Kilian Shani Fraysse, Shane P. Meaney, Will P. Gates, Daniel P. Langley, Rico F. Tabor, Paul R. Stoddart, George W. Greene
Summary: In this study, a new phenomenon of enhancing the dissolution rate of fused silica was discovered by conducting atomic force microscopy experiments. By pressing a second, dissimilar surface against the silica and oscillating the contact pressure in deionized water, the dissolution rate was enhanced by more than 5 orders of magnitude. This enhancement was only observed at asymmetric material interfaces and exhibited characteristics consistent with the electrochemical pressure solution mechanism.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Physical
Shahinur Acter, Nazneen Jahan, Mark Louis P. Vidallon, Boon Mian Teo, Rico F. Tabor
Summary: This study explores a new approach for targeted cancer treatment by combining chemo- and photothermal therapy using bio-derived polydopamine (PDA) mesoporous nanobowls, which possess exceptional biocompatibility. The results demonstrate that loading the anticancer drug doxorubicin (DOX) into the nanobowls and treating with near-infrared (NIR) illumination significantly enhances pharmaceutical cytotoxicity to cancer cells compared to free DOX. Additionally, combining the DOX loaded nanobowls with photothermal treatment results in nearly 100% cell death. This research highlights the potential of PDA mesoporous nanobowls as a scaffold for combined chemo- and photothermal therapy, offering new opportunities for treating advanced cancer.
PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION
(2022)
Article
Acoustics
Mark Louis P. Vidallon, Ekaterina Salimova, Simon A. Crawford, Boon Mian Teo, Rico F. Tabor, Alexis I. Bishop
Summary: This study optimized the process parameters for ultrasound-assisted fabrication of polydopamine-shelled perfluorocarbon emulsion droplets. The results showed that emulsion droplets with bimodal size distributions exhibited significant photoacoustic signal enhancement. The performance of these droplets in mimicked tissue media was evaluated, demonstrating that the bimodal droplets can enhance the photoacoustic signal up to five folds. Furthermore, using enhanced photoacoustic images, the maximal tissue imaging depths were explored for the droplets, indicating potential applications in theranostics and other imaging modalities.
ULTRASONICS SONOCHEMISTRY
(2022)
Review
Acoustics
Mark louis p. Vidallon, Boon mian Teo, Alexis i. Bishop, Rico f. Tabor
Summary: Ultrasound has important applications in diagnostic imaging, and new colloidal systems are being developed to address issues with commercial ultrasound contrast agents and expand their utility in targeted drug delivery and multimodal imaging. These systems, fabricated from or modified with biologically derived materials, show potential for biomedical applications, particularly imaging-guided treatments. This review article discusses recent developments, challenges, limitations, and future directions of colloids with ultrasound contrast enhancement.
ULTRASOUND IN MEDICINE AND BIOLOGY
(2022)
Article
Chemistry, Multidisciplinary
Calum S. G. Butler, Luke W. Giles, Anna V. Sokolova, Liliana de Campo, Rico F. Tabor, Kellie L. Tuck
Summary: Azobenzene-containing surfactants have been widely studied for their use in generating photoresponsive systems. This research focuses on tail substituted azo-surfactants to understand how surfactant structure can be tailored for specific applications. The study reveals the significant influence of tail group structure and intermolecular pi-pi interactions on the behavior of azo-surfactants.
Article
Multidisciplinary Sciences
Amelia C. Y. Liu, Espen D. Bojesen, Rico F. Tabor, Stephen T. Mudie, Alessio Zaccone, Peter Harrowell, Timothy C. Petersen
Summary: This study reveals a strong correlation between the centrosymmetry of nearest-neighbor polyhedra and the local mechanical stability in glasses. By examining the distribution of local stability and centrosymmetry, the underlying relationship between particle-level structure and larger-scale behavior is uncovered, demonstrating the significance of local structural transformations in predicting stability.
Article
Chemistry, Physical
Mark Louis P. Vidallon, Luke W. Giles, Simon Crawford, Alexis Bishop, Rico F. Tabor, Liliana de Campo, Boon Mian Teo
Summary: This study utilized small- and ultra-small-angle neutron scattering techniques to observe the in situ phase transition of polydopamine-stabilised perfluorohexane emulsion droplets into microbubbles during heating. Results indicated that the phase transition temperature of PDA/PFH emulsion droplets is significantly higher than the bulk boiling point of pure liquid PFH. Analysis and model fitting of the scattering data provided insights into droplet sizes and interfacial properties at different temperatures, revealing the transformation process of these polydisperse emulsion droplet systems.
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2021)
Article
Chemistry, Analytical
Michael J. Hertaeg, Rico F. Tabor, Heather McLiesh, Gil Garnier
Summary: Paper-based diagnostics are becoming more popular in low-cost, point of care analytical techniques, but large scale testing facilities still rely on traditional methods like gel column agglutination. The novel paper-based blood typing method presented here is rapid, scalable, and able to deliver test results in under ten seconds, making it potentially the fastest blood typing test suitable for large scale automation. This method has the potential to significantly reduce the time and cost of blood typing tests, and could lead to the development of a new high throughput and fully automatable system.
Article
Chemistry, Physical
Panpan Zhang, Xu Wang, Yangyang Yang, Haifeng Yang, Chunsheng Lu, Mingru Su, Yu Zhou, Aichun Dou, Xiaowei Li, Xiaochuan Hou, Yunjian Liu
Summary: In this study, the influence of transition metal doping on the electronic and mechanical properties and electrochemical performance of 2HMoS2/NC was investigated using Cobalt (Co) as an example. Co doping was found to effectively improve the electronic conductivity and active site areas of 2H-MoS2/NC at different positions, optimizing the adsorption and diffusion capability of potassium ions. Furthermore, the study revealed the optimal roles of different types of nitrogen atoms in kinetic adsorption, diffusion, and interfacial stability of potassium ions. These findings provide guidance for the experimental design of high rate 2H-MoS2/NC electrode materials and the optimal design of other functional composite materials.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zeeshan Ajmal, Mahmood Ul Haq, Shahid Zaman, M. K. Al-Muhanna, Anuj Kumar, Mohammed M. Fadhali, Siwar Ben Hadj Hassine, Muhammas Qasim, K. F. Alshammari, Ghulam Abbas Ashraf, Abdul Qadeer, Adil Murtaza, Sulaiman Al-Sulaimi, Huaqiang Zeng
Summary: This study presents a novel heterojunction structure (SrTiO3/CN-TAL10.0) for enhanced photocatalytic water splitting (PWS). The incorporation of thiophenedicarboxaldehyde (TAL) through copolymerization significantly improves the photocatalytic activity of carbon nitride (CN) while maintaining its photostability performance. The optimized composition allows efficient isolation of photoinduced charge carriers and enhanced charge transport, resulting in a remarkable increase in overall photocatalytic efficiency.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Angela Arnosa-Prieto, Patricia Diaz-Rodriguez, Manuel A. Gonzalez-Gomez, Pelayo Garcia-Acevedo, Lisandra de Castro-Alves, Yolanda Pineiro, Jose Rivas
Summary: Macrophages can exhibit different phenotypes depending on the microenvironment and the characteristics of magnetic iron oxide nanoparticles (MNPs). This study demonstrates that the concentration and morphology of MNPs can influence the polarization of macrophages. The findings have implications for therapeutics targeting tissue regeneration and tumor progression.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yu Fang, Cheng-Ye Zhu, Hao-Cheng Yang, Chao Zhang, Zhi-Kang Xu
Summary: This study demonstrates the advantages of vacuum-assisted interfacial polymerization (VAIP) in fabricating polyimide nanofiltration membranes. By using vacuum filtration, aqueous solutions of PIP can be evenly distributed on different microfiltration substrates, leading to the fabrication of uniform and ultra-thin polyamide layers with excellent performance. The membranes exhibit high rejection rates and water permeance, as well as satisfactory long-term stability.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Isaac J. Gresham, Edwin C. Johnson, Hayden Robertson, Joshua D. Willott, Grant B. Webber, Erica J. Wanless, Andrew R. J. Nelson, Stuart W. Prescott
Summary: Understanding the interactions between polymers and surfactants is crucial for optimizing commercial systems. This study tested the behavior of polymer-surfactant systems, revealing that they do not behave like polyelectrolytes in the presence of salt. Additionally, the structure of polymer-surfactant complexes under confinement differs from that of polyelectrolytes.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yunxiao Xie, Cui Liu, Jie Zhang, Yan Li, Bin Li, Shilin Liu
Summary: This study aimed to improve the microstructure and rheological properties of W/W Pickering emulsions by crosslinking sodium alginate at the water-water interface, thereby enhancing the activity of encapsulated probiotics in simulated gastrointestinal digestion.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Sang Ho Lee, Yige Sun, Patrick S. Grant
Summary: This research developed an effective approach to enhance the charging rates of lithium ion batteries (LIBs) by strategically incorporating carbon nanotube (CNT) conductivity boosters into Li4Ti5O12 (LTO) electrodes. Multi-layer architectures comprising CNT-rich and CNT-free LTO electrode layers were manufactured using a layer-by-layer spray coating method to promote charge transfer kinetics of high mass loading electrodes. The best performing multi-layer was paired with a spray-coated LiFePO4 (LFP) positive electrode, resulting in attractive power performance that outperformed conventional LTO || LFP combinations.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jingwei Liang, Shaobin Li, Fengbo Li, Li Zhang, Yufeng Jiang, Huiyuan Ma, Kun Cheng, Liang Qing
Summary: A molybdenum-regulated self-supporting electrode material with rich vacancy defects has been successfully synthesized and shows exceptional catalytic activities and stability for electrocatalytic overall water splitting. This study provides a new perspective for the design and synthesis of non-precious metal bifunctional electrocatalysts.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Jonas Blahnik, Jennifer Schuster, Rainer Mueller, Eva Mueller, Werner Kunz
Summary: This study investigates the relationship between the morphology of PMMA monopolymers and PMMA-PHEMA copolymers with the expected nature of surfactant-free microemulsions (SFMEs) before polymerization. It is found that previously mesostructured, surfactant-free mixtures can produce porous polymers of different morphologies, while unstructured, oil-rich regions lead to solid, transparent polymers without nanostructured morphologies. Additionally, a surfactant-based reference system shows similar phase behavior and polymer morphologies as the comparable surfactant-free system, indicating the importance of the hydrotropic behavior of HEMA in this system.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Zheng-Fen Pu, Wen-Zhi She, Rong Sheng Li, Qiu-Lin Wen, Bi-Chao Wu, Chun-Hua Li, Jian Ling, Qiue Cao
Summary: This study synthesized two framework-isomeric covalent organic frameworks (COFs) and discovered that the light scattering signal of COFs can be used for the analytical detection of lead ions. By controlling synthesis conditions and introducing regulators, the morphology of COFs could be controlled and framework-isomeric COFs could be precisely synthesized.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Yuchen Weng, Ying Hong, Jingyu Deng, Sicheng Cao, Li-Juan Fan
Summary: This paper reports the preparation of dynamic color-changing fluorescent polymer nanoparticles (PNPs) by constructing a fluorescence resonance energy transfer (FRET) pair. The PNPs show excellent anti-counterfeiting effects and reproducibility. The study demonstrates a promising encryption strategy that can achieve multiple outputs with simple operation.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Guodong Liu, Zijian Wang, Jianing Wang, Hanbin Liu, Zhijian Li
Summary: This study investigates the combination of multicolor switchable polyaniline (PANI) electrode and 1-methyl-4,4'-bipyridyl iodide (MBI), which demonstrates superior optical properties in visible and near-infrared light modulation, as well as excellent electrochemical performances. This combination can be used to develop novel electrochromic devices for applications in smart packaging, smart labels, and flexible smart windows.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Huying Yan, Yang Guo, Xingzhi Bai, Jiawei Qi, Haipeng Lu
Summary: By modifying Ti3C2Tx through heterogeneous interface engineering, optimized impedance matching is achieved, leading to enhanced electromagnetic wave absorption performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Kehu Zhang, Yang Zhou, Silvia Moreno, Simona Schwarz, Susanne Boye, Brigitte Voit, Dietmar Appelhans
Summary: This article presents an advanced crosslinking strategy to fabricate clustered polymersomes using host-guest interactions. By controlling the input of crosslinker and environmental conditions, reversible aggregation and disassembly of these polymersomes can be achieved. The size and structure of these clustered polymersomes can be regulated and visualized through a fluorescent enzymatic cascade reaction.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)
Article
Chemistry, Physical
Junjie Xu, Weixiong Huang, Ruiling Li, Li Li, Jinjin Ma, Jiaou Qi, Haiyan Ma, Min Ruan, Lilin Lu
Summary: In this study, a potassium doped palladium catalyst was developed for acetylene hydrogenation, showing excellent catalytic performance and durability. The doping of potassium effectively weakened the adsorption of ethylene, improved ethylene selectivity, and lowered the barriers of hydrogen activation and transfer reactions.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2024)