4.8 Article

Precise Tuning of Skyrmion Density in a Controllable Manner by Ion Irradiation

Journal

ACS APPLIED MATERIALS & INTERFACES
Volume 14, Issue 29, Pages 34011-34019

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsami.2c07268

Keywords

density of skyrmions; Ga+ irradiation; magnetic patterning; disorders; spintronic devices; TEM with Lorentz mode

Funding

  1. National Natural Science Foundation of China [51771085, 51571104, 51801087, 52071146, 12104197, 91962212]
  2. Science and Technology Project of Gansu Province, China [21JR7RA494, 21JR7RA492, 21JR7RA491]
  3. Fundamental Research Funds for the Central Universities [lzujbky-2020-58]
  4. Open Project of Key Laboratory for Magnetism and Magnetic Materials of the Ministry of Education, Lanzhou University [LZUMMM2021010]
  5. Special Funding for Open and Shared Large-Scale Instruments and Equipment of Lanzhou University [LZU-GXJJ-2020-011]

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In this study, a sharp increase in the density of magnetic skyrmions in specific positions of magnetic multilayer films was achieved through ion irradiation. Scanning transmission electron microscopy and micromagnetic simulation results showed that the density of skyrmions could be increased five times with a certain irradiation dose, and the magnetic field required to create skyrmions was also reduced. This research is of great significance for the practical application of magnetic skyrmions.
Magnetic skyrmions are topologically protected spin textures that were found to be promising candidates for next-generation spintronic devices owing to their small size and unique current-induced dynamics. Increasing skyrmions density at designated locations in a controllable manner is a prerequisite to further improve the recording density of magnetic memory devices and relevant spintronics. Here, we demonstrate that a sharp increase in skyrmion density in magnetic multilayer films can be purposefully realized at a site-specific position by ion irradiation, which has industrial applicability. The Cs-scanning transmission electron microscopy and micromagnetic simulation results indicate that the skyrmions density can be sharply increased five times after applying an exposure with an irradiation dose of 1.5 x 10(14) Ga+/cm(2), and the magnetic field required to create skyrmions is also reduced. The intrinsic physical mechanism of increasing skyrmion density is found to mainly originate from the formation of disorders through Ga+ irradiation, which can induce a decrease in the nucleation energy barrier of skyrmions. We further show that the artificial skyrmion patterns with tunable density can be intentionally written at specific sites by using a Ga(+ )ion beam. This work should contribute a significant step toward eventually realizing the practical recording application of magnetic skyrmions.

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