Journal
FRONTIERS IN CHEMISTRY
Volume 9, Issue -, Pages -Publisher
FRONTIERS MEDIA SA
DOI: 10.3389/fchem.2021.753741
Keywords
polyphenylenesulfone; reduced graphene oxide; titanium dioxide; photodegradation; self-cleaning
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The novel reduced graphene oxide/TiO2-polyphenylenesulfone (rGO/TiO2-PPSU) hybrid ultrafiltration membrane exhibits efficient visible-light-driven photocatalytic degradation of organic pollutants and superior antifouling properties. Compared to membranes prepared with graphene oxide and TiO2 separately, the rGO/TiO2-PPSU membrane showed significantly improved photodegradation of phenazopyridine hydrochloride solution under UV and visible light.
Nanosized titanium oxide (TiO2)-based photocatalysts have exhibited great potential for the degradation of organic contaminants, while their weak absorption of visible light limits the photocatalytic efficiency. Herein, a novel reduced graphene oxide/TiO2-polyphenylenesulfone (rGO/TiO2-PPSU) hybrid ultrafiltration membrane has been successfully prepared via a non-solvent induced phase-separation method, in which the synergistic coupling between the rGO and TiO2 could endowed the fabricated membranes with visible-light-driven efficient photocatalytically degradation of organic pollutants and outstanding photocatalytic and antifouling properties. Compared with the PPSU membranes prepared with Graphene oxide and TiO2, respectively, the rGO/TiO2-PPSU membrane demonstrated significant photodegradation towards phenazopyridine hydrochloride (PhP) solution under ultraviolet light (improved about 71 and 43%) and visible light (improved about 153 and 103%). The permeability and flux recovery rates of the membrane indicated that the high flux of the rGO/TiO2-PPSU membrane can be greatly restored after fouling, due to the improved self-cleaning properties under visible light static irradiation. With the properties of high performance of photocatalytic degradation and good self-cleaning ability, the rGO/TiO2-PPSU membrane would have great potential in water treatment.
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