4.8 Article

Energy generation from airborne noise: Improving electrical outputs of single-layer polyvinylidene difluoride nanofiber membranes by incorporating a small number of nylon-6 nanofibers

Journal

NANO ENERGY
Volume 90, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.nanoen.2021.106618

Keywords

Energy harvesting; Airborne noise; Polyvinylidene difluoride; Nylon-6; Acoustoelectric; Charge transport

Funding

  1. Australian Research Council [DP 210100838]
  2. Natural Science Foundation of Shandong Province [ZR2020ME062]
  3. Jiangsu New Vison Advanced Functional Fiber Innovation Center open fund (China)
  4. State Key laboratory for biofibers and Ecotextiles of Qingdao University (China) open fund

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This research presents a novel approach to improve the electrical output of a noise-related energy harvester by incorporating a small number of nylon-6 nanofibers into the PVDF fibrous matrix, significantly enhancing the acoustoelectric conversion and electrical outputs. The addition of nylon-6 nanofibers can increase the voltage and current outputs by 2.7 times and 2.6 times, respectively, compared to a pure PVDF nanofiber counterpart, with a broader bandwidth range.
Considerable research has been devoted to generating electricity from airborne noise. However, it is still a challenge to develop high-efficiency, large-output energy harvesters for this purpose. Herein, we present a novel approach to improve the electrical output of a noise-related energy harvester, made of single-layer poly-vinylidene difluoride (PVDF) nanofiber membrane, simply by incorporating a small number of nylon-6 nanofibers into the PVDF fibrous matrix. The addition of just 4.3 wt% nylon-6 nanofibers profoundly improves the acoustoelectric conversion. In an airborne noise environment (e.g., 230 Hz 118 dB SPL), the device (working area 12 cm(2)) can generate peak electrical outputs as high as 201.4 V and 17.6 mu A (power density 1.30 W/m(2)). The voltage and current outputs are 2.7 times and 2.6 times higher, respectively, compared to the pure PVDF nanofiber counterpart. The nylon-6/PVDF device also showed broader bandwidth, covering a frequency range of 230-800 Hz. The nylon-6 nanofibers were found to play dual roles in noise harvesting: 1) a tribo component to cause an endogenous triboelectric effect with PVDF nanofibers, and 2) a dopant to form macro dipoles, thus improving the charge transport from a dielectric layer to the external electrodes, which significantly increases the electrical outputs. Incorporating high polarity dopant may form a novel approach to improve the electrical outputs of acoustoelectric nanofibers.

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