Article
Chemistry, Multidisciplinary
Zedong Zhang, Jiexin Zhu, Shenghua Chen, Wenming Sun, Dingsheng Wang
Summary: Downsizing the active center of the main group element gallium to the atomic level enables efficient CO2 reduction with high selectivity and stability.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Physical
Yun Yang, Shixi Liu, Gang Fu
Summary: The electrochemical CO2 reduction reaction (CO2RR) over transition metal and α-In2Se3 monolayer catalysts was investigated using density functional theory (DFT) and an effective screening medium method-reference interaction site model (ESM-RISM). Relationships between oxygen-bound intermediates with *O and carbon-bound intermediates with *CHO were constructed based on scaling relationships between the adsorption free energies of intermediates. The results indicate that *OCHO intermediates are more favorable for the first hydrogenation of CO2 on M@In2Se3 catalysts, and the adsorption energy of oxygen-bound species determines the catalytic performance of M@In2Se3. The Co@In2Se3 catalyst was predicted to be the most promising catalyst with a low limiting potential of -0.385 V, and the M@In2Se3 catalysts hold great potential for highly efficient CO2RR. This work provides a fundamental understanding for the rational design of ferroelectric single-atom catalysts for highly efficient electrocatalytic CO2 reduction.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2023)
Review
Chemistry, Applied
Qian Sun, Chen Jia, Yong Zhao, Chuan Zhao
Summary: This review summarizes the fabrication, application, and characterization methods of single-atom catalysts (SACs) and molecular catalysts for CO2 electroreduction. Strategies for overcoming the issues of particle agglomeration, low metal loading, and difficulty in large-scale production of SACs, as well as the moderate activity, selectivity, and stability of molecular catalysts, are highlighted. Future directions for the development of SACs and molecular catalysts are pointed out.
CHINESE JOURNAL OF CATALYSIS
(2022)
Review
Chemistry, Multidisciplinary
Jinxian Wang, Danni Deng, Qiumei Wu, Mengjie Liu, Yuchao Wang, Jiabi Jiang, Xinran Zheng, Huanran Zheng, Yu Bai, Yingbi Chen, Xiang Xiong, Yongpeng Lei
Summary: This review summarizes the recent progress of atomically dispersed (AD) copper catalysts as a chemically tunable platform for electrochemical CO2 reduction (ECO2R). It discusses the dynamic evolution, catalytic performance, and mechanism of these catalysts, as well as the prospects and challenges in the field. The review aims to contribute to the rational design of AD copper catalysts with enhanced performance for ECO2R.
Article
Chemistry, Physical
Paige Brimley, Hussain Almajed, Yousef Alsunni, Abdulaziz W. Alherz, Zachary J. L. Bare, Wilson A. Smith, Charles B. Musgrave
Summary: This study uses Grand Canonical Density Functional Theory (GC-DFT) to model the electrochemical CO2 reduction process over metal-and nitrogen-doped graphene catalysts (MNCs) and includes the effects of the applied potential. The results predict effective catalysis of CO2R by Sc, Ti, Co, Cu, and Zn-N4Cs at moderate to large reducing potentials. The GC-DFT-computed density of states analysis demonstrates the critical role of adsorbed *CO2- anion in CO2R activation.
Article
Chemistry, Physical
Paige Brimley, Hussain Almajed, Yousef Alsunni, Abdulaziz W. Alherz, Zachary J. L. Bare, Wilson A. Smith, Charles B. Musgrave
Summary: In this study, electrochemical CO2 reduction (CO2R) over metal-and nitrogen-doped graphene catalysts (MNCs) was modeled using grand canonical density functional theory (GC-DFT), explicitly including the effects of the applied potential. The results predict that certain MNCs effectively catalyze CO2R at moderate to large reducing potentials, with ZnN4C identified as a promising electrocatalyst across a range of potentials. Thermodynamic analysis reveals insights into the pH independence of CO production and the rate-determining step of CO2R over specific catalysts.
Review
Engineering, Environmental
Yingjie Liu, Sha Bai, Qian Li, Zhaohui Wu, Tianyang Shen, Jinfeng Chu, Yu-Fei Song
Summary: This review summarizes the latest developments in single atom materials for CO2 electroreduction, including the application of dual atom catalysts and single atom-cooperating with nanoparticles materials. The article reviews the fine structure of these materials and their relationship with performance, as well as advanced spectroscopic methods for characterization and monitoring of the transformation process. In addition, it discusses the current unresolved issues and future prospects for CO2 electroreduction.
CHEMICAL ENGINEERING JOURNAL
(2023)
Review
Chemistry, Multidisciplinary
Jiexin Zhu, Lei Lv, Shahid Zaman, Xingbao Chen, Yuhang Dai, Shenghua Chen, Guanjie He, Dingsheng Wang, Liqiang Mai
Summary: This review summarizes the current research progress and future application prospects of electrochemical CO2 methanation on single-site catalysts (SSCs). It discusses the CO2 methanation mechanism, primary activity descriptors, coordination structure and design of SSCs, and several in situ characterization methods for tracking the structural changes in SSCs. This review provides insights into the further exploitation of SSCs for selective CO2 methanation and inspires the rational design of SSCs in electrochemical CO2 methanation research.
ENERGY & ENVIRONMENTAL SCIENCE
(2023)
Review
Materials Science, Multidisciplinary
Jian-Bin Liu, Hai-Sheng Gong, Gong-Lan Ye, Hui-Long Fei
Summary: This review summarizes the recent advances in graphene oxide-derived single-atom catalysts (GO-SACs) for sustainable electrochemical energy conversion, including their preparation strategies, electrochemical applications, and future prospects.
Article
Chemistry, Physical
Xinyu Li, Haobo Li, Zhen Zhang, Javen Qinfeng Shi, Yan Jiao, Shi-Zhang Qiao
Summary: In this study, a class of triple-atom A2B catalysts, with two A metal atoms and one B metal atom embedded in nitrogen-doped graphene plane, were designed and evaluated for electrochemical CO2 reduction. The results showed that these catalysts can selectively produce valuable hydrocarbon products while maintaining high reactivity, and six potential CRR catalysts were proposed.
Review
Materials Science, Multidisciplinary
Xiaojiao Li, Xiaohu Yu, Qi Yu
Summary: This article reviews the recent progress of Cu-based single-atom catalysts (SACs) in CO2 reduction reaction (CO2 RR), discussing the regulatory strategies for the interaction of the active site with key reaction intermediates. Different design strategies, including the regulation of metal centers, Cu-based single-atom alloy catalysts (SAAs), non-metal SACs, tandem catalysts, and composite catalysts, are also reviewed. Furthermore, the current challenges and future developments of SACs in CO2 RR are summarized.
SCIENCE CHINA-MATERIALS
(2023)
Article
Chemistry, Physical
Naiwrit Karmodak, Sudarshan Vijay, Georg Kastlunger, Karen Chan
Summary: In this study, computational screening and analysis were conducted to investigate the catalytic activity of single and di-atom catalysts on nitrogen-doped graphene for CO2 reduction. The research identified high-efficiency catalysts and studied their behavior and binding motifs.
Article
Chemistry, Multidisciplinary
Youngho Kang, Sungwoo Kang, Seungwu Han
Summary: Based on density functional theory calculations, it was found that in transition metal- and nitrogen-codoped graphene, single Zn atoms do not serve as active sites for CO production in CO2 reduction reactions, while the nearest neighbor C atom (C-NN) exhibits high activity and the Zn atom enhances the catalytic activity of C-NN. The study also revealed that *COOH formation is favorable at the initial electrochemical step on the C-NN site, and each reaction step becomes downhill in energy at small applied potentials, elucidating the origin of the CO2 reduction activity.
Article
Chemistry, Physical
Jian-Chao Jiang, Jun-Chi Chen, Meng-die Zhao, Qi Yu, Yang-Gang Wang, Jun Li
Summary: In this study, a series of Cu-based single-atom alloy catalysts (SAAs) were designed and evaluated for CO2RR. The catalysts showed improved activity for CO2 hydrogenation compared to pure Cu catalysts. The bond angle of adsorbed *CO2 and binding energy of *OH were identified as indicators for CO2 activation ability and CO2RR activity, respectively.
Review
Chemistry, Physical
Shu-Guo Han, Dong-Dong Ma, Qi-Long Zhu
Summary: Carbon-based single-atom catalysts (SACs) have shown significant potential for electrochemical carbon dioxide reduction reaction (CO2RR) by regulating the coordination structures of metal centers and the microenvironments of substrates. This review summarizes recent advances in synthetic strategies and the structure-performance relationship of SACs towards CO2RR, highlighting the challenges and research directions for SACs in the future.
Article
Chemistry, Physical
Yehui Zhang, Bing Wang, Yixin Ouyang, Yipeng Zhou, Qiang Li, Jinlan Wang
Summary: In this study, we propose an adaptive algorithm based on the differential evolution algorithm for structure searching in low-symmetry systems. Our algorithm can not only locate known structures but also discover new stable configurations that were previously unknown. Additionally, we provide frameworks and interfaces for stable structure searching in complex systems.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Chunjin Ren, Shuaihua Lu, Yilei Wu, Yixin Ouyang, Yehui Zhang, Qiang Li, Chongyi Ling, Jinlan Wang
Summary: In this study, a simple and universal descriptor based on inherent atomic properties was proposed for evaluating the complicated interfacial effects on electrochemical reduction reactions. The activity and selectivity trends in CO2 reduction reaction were successfully elucidated, and several potential catalysts with superior activity and selectivity were predicted. Furthermore, the descriptor was also extended to evaluate the activity of dual-atom catalysts for O-2 and N-2 reduction reactions.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Multidisciplinary Sciences
Yan Yang, Jiaju Fu, Yixin Ouyang, Tang Tang, Yun Zhang, Li-Rong Zheng, Qing-Hua Zhang, Xiao-Zhi Liu, Jinlan Wang, Jin-Song Hu
Summary: The electronically asymmetric Cu-Cu/Cu-N-C interface site enhances the adsorption of *CO intermediates and lowers the reaction barrier of C-C coupling in electrochemical CO2 reduction (ECR), enabling efficient C-C coupling at low overpotential. The high-density Cu/CuNC interface sites (ER-Cu/CuNC) catalyst boosts the electrocatalytic CO2-to-ethanol conversion with a Faradaic efficiency toward C2+ of 60.3% (FEethanol of 55%) at a low overpotential of -0.35 V. These findings provide new insights into the efficient conversion of CO2 to C2+ products.
NATIONAL SCIENCE REVIEW
(2023)
Article
Chemistry, Multidisciplinary
Zhanzhao Fu, Mingliang Wu, Qiang Li, Chongyi Ling, Jinlan Wang
Summary: The performance of supported catalysts is influenced by metal-support interactions, and quantifying the structure-activity relationship remains a challenge. This work constructs a simple descriptor to describe the effect of metal-support interaction on the nitrogen reduction reaction (NRR) activity. The descriptor accurately predicts the limiting potential (U-L) for the NRR without density functional theory calculations. The study also demonstrates the applicability of the descriptor to other materials and successfully selects promising NRR catalysts.
MATERIALS HORIZONS
(2023)
Article
Chemistry, Physical
Yipeng Zhou, Yixin Ouyang, Yehui Zhang, Qiang Li, Jinlan Wang
Summary: This Perspective article summarizes the recent progress and achievements in simulating electrochemical interfaces using machine learning. It discusses the limitations of current machine learning models, such as accurately describing long-range electrostatic interactions and the kinetics of electrochemical reactions at the interface. Finally, it points out future directions for machine learning to expand in the field of electrochemical interfaces.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2023)
Article
Chemistry, Physical
Yixin Ouyang, Li Shi, Xiaowan Bai, Chongyi Ling, Qiang Li, Jinlan Wang
Summary: The mechanism of enhancing ethanol selectivity over modified copper catalysts is clarified in this study by combining explicit solvent models with slow-growth molecular dynamics. Surface-active hydrogen, introduced by guest metals and high-facet atomic arrangements, promotes the kinetics of surface-coupled hydrogenation of intermediates while inhibiting solvent hydrogenation, thereby unlocking the reaction pathway towards ethanol products. This research provides insights into the design of catalytic systems for electrochemical CO2 reduction with desired alcohol products.
Review
Chemistry, Multidisciplinary
Yixin Ouyang, Yipeng Zhou, Yehui Zhang, Qiang Li, Jinlan Wang
Summary: This review discusses the atomic structure characterization of intrinsic defects in two-dimensional layered transition metal dichalcogenides and their impact on the physical and chemical properties of the material. The changes induced by these defects and their effects in various applications are also addressed. Current approaches to filling or passivating defects, as well as methods for in situ synthesis and post-processing to generate defects, are summarized.
TRENDS IN CHEMISTRY
(2022)
Article
Materials Science, Multidisciplinary
Xiaowan Bai, Li Shi, Qiang Li, Chongyi Ling, Yixin Ouyang, Shiyan Wang, Jinlan Wang
Summary: By introducing a second metal and a functional ligand, a design strategy is proposed to achieve high selectivity of C-2 oxygenates and effectively inhibit the HER on the Cu(100) surface. This approach provides a new method to improve the electrocatalytic reduction of CO2.
ENERGY & ENVIRONMENTAL MATERIALS
(2022)
Article
Chemistry, Physical
Yixin Ouyang, Yehui Zhang, Peter S. Rice, Li Shi, Jinlan Wang, P. Hu
Summary: This study compared the electrochemical reduction of carbon dioxide at the aqueous solution/copper interface and polymer electrolyte/copper interface, revealing a fundamental understanding of the superiority of APEECs. Advanced simulations showed that the polymer electrolyte/copper interface exhibited a higher turnover frequency, contributing to an increased conversion current density of APEECs.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Chemistry, Multidisciplinary
Zhanzhao Fu, Qiang Li, Xiaowan Bai, Yuhao Huang, Li Shi, Jinlan Wang
Summary: This study introduces a simple coordination regulation method of the active site to improve the efficiency of CO2 conversion, demonstrates the excellent catalytic performance of NiN3B in CH4 conversion, and highlights the synergistic dual active sites formed between non-metal B and metal Ni atoms in catalysis.
Article
Chemistry, Physical
Shiyan Wang, Xiaowan Bai, Qiang Li, Yixin Ouyang, Li Shi, Jinlan Wang
Summary: It has been demonstrated that two-dimensional Cu2S monolayers are promising photocatalysts for the reduction of CO2 into C2H5OH. The calculations show that these catalysts can greatly enhance the conversion efficiency of C2H5OH, while exhibiting satisfactory visible light absorption and band edge positions.
NANOSCALE HORIZONS
(2021)
Article
Chemistry, Physical
Jianxiong Tian, Zhaobo Zhou, Sheng Zhang, Zhixia Li, Li Shi, Qiang Li, Jinlan Wang
Summary: Metal-free photocatalysts based on graphitic carbon nitride (g-C3N4) have shown potential for water oxidation, but their efficiency is often limited by slow reaction rates and fast recombination of electron-hole pairs. This study demonstrates that modifying electronic structures, such as changing the N ratio and doping heteroatoms, can significantly enhance the photocatalytic activity for water oxidation. Specifically, reducing the N ratio and introducing S-doping can improve the OER activity and trap photo-generated holes, leading to enhanced photocatalytic efficiency. Evaluations of band edges, light absorbance, and thermal stability further provide insights for optimizing the performance of carbon nitride based photocatalysts.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Chemistry, Physical
Xianghong Niu, Dazhong Sun, Li Shi, Xiaowan Bai, Qiang Li, Xing'ao Li, Jinlan Wang
Summary: This study proposed a new strategy for N-2 fixation using metal-free boron-decorated diamond clusters, which creates excited states and improves selectivity under light illumination. This approach offers insights for advancing photocatalysis for sustainable NH3 production.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Article
Chemistry, Physical
Mei Gui Vanessa Wee, Amutha Chinnappan, Runxin Shang, Poh Seng Lee, Seeram Ramakrishna
Summary: Cooling processes, from residences to industries, require a lot of energy and are essential. This study introduces MIL-101(Cr), a new desiccant, to heat exchangers for more efficient cooling. By improving the synthesis method and using a special binder, the MIL-101(Cr)-coated heat exchanger shows improved water uptake capacity and lower regeneration temperature.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Ao Zhen, Guanyu Zhang, Ao Wang, Feng Luo, Jiehua Li, Hong Tan, Zhen Li
Summary: In this study, a solvent-free microemulsion method was used to synthesize waterborne polyurethane (WPU) material with high retention of mechanical properties and satisfactory water absorption rates. The material showed excellent biocompatibility and has broad application potential in the field of biomedicine.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Review
Chemistry, Physical
Wensong Ge, Rui Wang, Xiaoyang Zhu, Houchao Zhang, Luanfa Sun, Fei Wang, Hongke Li, Zhenghao Li, Xinyi Du, Huangyu Chen, Fan Zhang, Huifa Shi, Huiqiang Hu, Yongming Xi, Jiankang He, Liang Hu, Hongbo Lan
Summary: This paper reviews the research on the surface tension of eutectic gallium-indium alloys (EGaIn) in the field of stretchable electronics. It covers the principles of oxide layer formation, factors influencing surface tension, and methods for surface modification of liquid metals. The paper also discusses the applications of EGaIn surface modification in different fields and highlights the challenges still faced and the future outlook.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Review
Chemistry, Physical
Xiang Song, Lianghao Jia, Zhengen Wei, Tao Xiang, Shaobing Zhou
Summary: This paper provides an overview of the application, preparation, and role of biomimetic structures in solar evaporators with improved evaporation rate and lifetime.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Wei Yuan, Qian Deng, Dong Pan, Xiang An, Canyang Zhao, Wenjun Su, Zhengmin He, Qiang Sun, Ran Ang
Summary: Optimizing the performance of n-type PbTe thermoelectric materials is crucial for practical applications. Dynamic doping has emerged as an effective method to improve the performance of n-type PbTe by optimizing the carrier concentration. This study demonstrates the significance of Mn alloying in enhancing the performance of Ag-doped n-type PbTe by creating a hierarchical structure to suppress thermal transport and improving the Seebeck coefficient.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Review
Chemistry, Physical
Xiaoyan Wang, Meiqi Geng, Shengjun Sun, Qian Xiang, Shiyuan Dong, Kai Dong, Yongchao Yao, Yan Wang, Yingchun Yang, Yongsong Luo, Dongdong Zheng, Qian Liu, Jianming Hu, Qian Wu, Xuping Sun, Bo Tang
Summary: This review provides a comprehensive analysis of the progress and challenges in the field of bifunctional electrocatalysts and efficient electrolyzers for seawater splitting. It summarizes recent advancements and proposes future perspectives for highly efficient bifunctional electrocatalysts and electrolyzers.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Jason K. Phong, Christopher B. Cooper, Lukas Michalek, Yangju Lin, Yuya Nishio, Yuran Shi, Huaxin Gong, Julian A. Vigil, Jan Ilavsky, Ivan Kuzmenko, Zhenan Bao
Summary: Dynamic block copolymers (DBCPs) combine the phase separation of traditional block copolymers with the supramolecular self-assembly of periodic dynamic polymers, resulting in the spontaneous self-assembly of high aspect ratio nanofibers with well-ordered PEG and PDMS domains. DBCPs with a periodic block sequence exhibit superior properties compared to those with a random sequence, including delayed onset of terminal flow and higher ionic conductivity values.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Hong Kyu Lee, Yasaswini Oruganti, Jonghyeon Lee, Seunghee Han, Jihan Kim, Dohyun Moon, Min Kim, Dae-Woon Lim, Hoi Ri Moon
Summary: This study reports the moisture-triggered proton-conductivity switching behavior in Zn5FDC MOFs induced by the presence and absence of coordinating solvents, which illustrates the significant role of coordinating solvents in conductivity variation.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Bommaramoni Yadagiri, Sanjay Sandhu, Ashok Kumar Kaliamurthy, Francis Kwaku Asiam, Jongdeok Park, Appiagyei Ewusi Mensah, Jae-Joon Lee
Summary: The molecular engineering of the interface modulator between the perovskite and hole transporting material is crucial for achieving satisfactory performance and stability of perovskite solar cells. In this study, cruciform-shaped dual functional organic materials were employed as surface passivation and hole transporting interfacial layers in perovskite solar cells. The use of these materials significantly improved the power conversion efficiency of the solar cells.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Joaquin Martinez-Ortigosa, Reisel Millan, Jorge Simancas, Manuel Hernandez-Rodriguez, J. Alejandro Vidal-Moya, Jose L. Jorda, Charlotte Martineau-Corcos, Vincent Sarou-Kanian, Mercedes Boronat, Teresa Blasco, Fernando Rey
Summary: This study investigates the synthesis of all-silica RTH zeolites using triisopropyl(methyl)phosphonium as the organic SDA. The results show the formation of two distinct crystalline phases under different synthesis conditions, with fluoride bonding to different silicon sites. It demonstrates the possibility of controlling the placement of fluoride in RTH zeolites through synthesis conditions.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Luyao Zheng, Cong Liu, Wenbiao Zhang, Boxu Gao, Tianlan Yan, Yahong Zhang, Xiaoming Cao, Qingsheng Gao, Yi Tang
Summary: This study successfully improves the efficiency and stability of water splitting by constructing a heterostructured electrocatalyst. The catalyst shows extraordinary performance and could offer an effective approach for the sustainable production of hydrogen.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Carlos A. Campos-Roldan, Raphael Chattot, Frederic Pailloux, Andrea Zitolo, Jacques Roziere, Deborah J. Jones, Sara Cavaliere
Summary: This study systematically evaluated the hydrogen evolution/oxidation reactions on a series of Pt-rare earth nanoalloys in alkaline media, and identified the effect of the lanthanide contraction. The experimental results revealed that the chemical nature of the rare earth modulates the adsorption and mobility of oxygenated-species, enhancing the kinetics of the reactions.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Sara Frank, Mads Folkjaer, Mads L. N. Nielsen, Melissa J. Marks, Henrik S. Jeppesen, Marcel Ceccato, Simon J. L. Billinge, Jacopo Catalano, Nina Lock
Summary: This study investigates the thermal decomposition of ZIF-67 and its correlation with structural evolution and electrocatalytic performance. The researchers used in situ X-ray absorption spectroscopy and total scattering techniques to analyze the process. They found that disorder emerges at lower temperatures and that extending the pyrolysis process can result in materials with superior electrochemical properties.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Zi-Yang Zhang, Hao Tian, Han Jiao, Xin Wang, Lei Bian, Yuan Liu, Nithima Khaorapapong, Yusuke Yamauchi, Zhong-Li Wang
Summary: By constructing Cu-0-Cu+-NH2 composite interfaces with the assistance of SiO2, the electrochemical CO2 reduction reaction (CO2RR) achieves high Faraday efficiency and current density for C2+ production, improving the productivity of carbon cycle.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)
Article
Chemistry, Physical
Ting Wang, Ruijuan Zhang, Pengda Zhai, Mingjie Li, Xinying Liu, Chaoxu Li
Summary: This study successfully exfoliated COFs using a simple electrochemical method, which resulted in improved photocatalytic performance for COFs and enriched the fabrication approach of COF exfoliation.
JOURNAL OF MATERIALS CHEMISTRY A
(2024)