Journal
NANO TODAY
Volume 40, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.nantod.2021.101245
Keywords
Phosphorus-rich metal phosphides; Lithium; sodium ion batteries; Hydrogen; oxygen evolution reaction; Theory-composition; structure-performance relationship
Categories
Funding
- National Natural Science Foundation of China [51972075, 51772059]
- Natural Science Foundation of Heilongjiang Province [ZD2019E004]
- China Postdoctoral Science Foundation [2020M681075]
- Fundamental Research Funds for the Central Universities
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Phosphorus-rich metal phosphides (MPs) have emerged as cutting-edge materials in energy storage and conversion, exhibiting significant advantages in various applications. This review summarizes the latest advances in P-rich MPs regarding typical structures, synthetic methods, and performance optimizations. The discussion covers electrochemical reaction mechanisms, composition/structure designs, and desired performance, providing insights into theory-composition/structure-performance relationships and future research directions.
The development of cost-efficient and high-performance electrochemical materials is very important to promote clean energy storage and conversion. Very recently, the phosphorus-rich (P-rich) metal phosphides (MPs) emerge as the cutting-edge materials in energy storage and conversion due to their significant advantages for lithium ion batteries (LIBs), sodium ion batteries (SIBs), hydrogen evolution reaction (HER), oxygen evolution reaction (OER) and solar cells (SCs). This review summarizes the up-to-date advances of P rich MPs in energy storage and conversion from typical structures, main synthetic methods and diversified advanced applications. The corresponding electrochemical reaction mechanism, composition/structure designs and desired performance of P-rich MPs are conjointly discussed to deliver an insightful perspective of the theory-composition/structure-performance relationships and reveal the reasons behind the excellent electrochemical performance. At last, several potential challenges and inspiring outlooks are highlighted to serve guidance for the future research and applications of P-rich MPs. (c) 2021 Elsevier Ltd. All rights reserved.
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