4.7 Article

Effects of bluff-body cone angle on turbulence-chemistry interaction behaviors in large-scale semicoke and bituminous coal co-combustion

Journal

FUEL PROCESSING TECHNOLOGY
Volume 221, Issue -, Pages -

Publisher

ELSEVIER
DOI: 10.1016/j.fuproc.2021.106915

Keywords

Large-scale semicoke co-combustion; Bluff-body cone angle; Temperature uniformity; Turbulence-chemistry interactions; Damkohler number; Low NOx emissions

Funding

  1. National Key Research and Development Program of China [2017YFB0602002]
  2. National Natural Science Foundation of China [51536002]

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Increasing the bluff-body cone angle contributes to moving the main reaction zone upstream, improving char oxidation reactions and increasing pore structures. A larger cone angle leads to a 27% reduction in NOx emissions at α=34 degrees, enhancing combustion reduction zones and oxygen diffusion rates.
During large-scale semicoke and bituminous coal co-combustion, the behaviors of turbulence-chemistry interactions were experimentally and numerically used to investigate the effects of char burnout and NOx emissions in a pilot-scale bias combustor at different bluff-body cone angles (alpha). The results show that with increasing alpha the main reaction zone moves upstream significantly, and a widened flame and uniform temperature profile are obtained due to enhancing the internal flue gas recirculation. An increase in alpha can improve the char-oxidation reaction, and further results in increased pore structures and char burnout ratios. For all cases, the Da(t) (homogeneous Damkohler number) maximum values are below 0.50. The Da(,O2), Da(,CO2) and Da(,H2O) (heterogeneous Damkohler numbers) values are within 0.670-1.207, 0.004-0.017 and 0.001-0.004, indicating that the char oxidation reaction is dominated by diffusion/kinetics, while the char gasification reactions are controlled by chemical kinetics. However, both reactions tend to be kinetically-controlled with increasing alpha. The NOx emissions decrease by 27% at the alpha = 34 degrees value, because a large cone angle can enlarge the combustion reduction zone and enhance the oxygen diffusion rate. The findings can provide deep insight into the turbulence-chemistry interactions and its effect on NOx emission characteristics of semicoke co-combustion in a bluff-body tangential burner.

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