4.7 Article

Confined tailoring of CoFe2O4/MWCNTs hybrid-architectures to tune electromagnetic parameters and microwave absorption with broadened bandwidth

Journal

CERAMICS INTERNATIONAL
Volume 48, Issue 7, Pages 9569-9578

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.ceramint.2021.12.155

Keywords

MWCNTs; CoFe2O4; Hybrid composite; Reflection loss; Effective absorption bandwidth

Funding

  1. National Science Foundation of China [51572154]

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In this study, cobalt ferrite/multi-walled carbon nanotubes hybrid composite was synthesized using a solvothermal technique. Various analytical techniques were used to investigate the composition, morphological structure, and electromagnetic parameters of the hybrid composite. The results showed that the obtained composite exhibited excellent electromagnetic wave absorption properties, with better reflection loss compared to typical magnetic composite absorbers.
Multi-walled carbon nanotubes (MWCNTs) are highly alluring as an electromagnetic (EM) wave absorber owing to their multi-dimensional structure, high chemical stability, low density, and significant conduction loss, which provide great promises as an excellent EM wave absorber in practical applications. Herein, a simple and controllable solvothermal technique is applied to synthesize cobalt ferrite/MWCNTs (CoFe2O4/MWCNTs) hybrid composite. Various analytical techniques were used to investigate the composition, morphological structure, and electromagnetic parameters of the as-prepared hybrid composite. The obtained results revealed that, a strong network of CoFe(2)O(4)microspheres interweaved with MWCNTs in the prepared hybrid composite. The resultant CoFe2O4/MWCNTs composites achieve a minimum reflection loss (RLmin) of-50.80 dB at a thickness of 4.2 mm and effective absorption bandwidth (EAB) of 3.36 GHz at a thickness of 1.6 mm exhibiting the superior RLmin compared to the typical magnetic composite derived absorbers. This research advocates the precise development and designing of unique MWCNTs-based composites as a high-efficient and lightweight electromagnetic wave absorber.

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