4.8 Article

Fast Uncooled Mid-Wavelength Infrared Photodetectors with Heterostructures of van der Waals on Epitaxial HgCdTe

Journal

ADVANCED MATERIALS
Volume 34, Issue 6, Pages -

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202107772

Keywords

mid-wavelength infrared photodetectors; photovoltaic effect; uncooled infrared photodetectors; vdWs-on-MCT

Funding

  1. National Key Research and Development Program of China [2020YFB2009300]
  2. National Natural Science Foundation of China [61725505, 62105349]
  3. Science and Technology Commission of Shanghai Municipality [21JC1406100, 19XD1404100, 21ZR1473400, 21YF1454900]
  4. China Postdoctoral Science Foundation [2020TQ0331, BX2021330]

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Uncooled infrared photodetectors have drawn attention for their low cost and compact detection systems, but typically have slow response times. This study explores a van der Waals heterojunction on epitaxial HgCdTe for uncooled mid-wavelength infrared photodetection, achieving fast response times and high detectivity.
Uncooled infrared photodetectors have evoked widespread interest in basic research and military manufacturing because of their low-cost, compact detection systems. However, existing uncooled infrared photodetectors utilize the photothermoelectric effect of infrared radiation operating at 8-12 mu m, with a slow response time in the millisecond range. Hence, the exploration of new uncooled mid-wavelength infrared (MWIR) heterostructures is conducive to the development of ultrafast and high-performance nano-optoelectronics. This study explores a van der Waals heterojunction on epitaxial HgCdTe (vdWs-on-MCT) as an uncooled MWIR photodetector, which achieves fast response as well as high detectivity for spectral blackbody detection. Specifically, the vdWs-on-MCT photodetector has a fast response time of 13 ns (77 MHz), which is approximately an order of magnitude faster than commercial uncooled MCT photovoltaic photodetectors. Importantly, the device exhibits a photoresponsivity of 2.5 A W-1, quantum efficiency as high as 85%, peak detectivity of 2 x 10(10) cm Hz(1/2) W-1 under blackbody radiation at room temperature, and peak detectivity of up to 10(11) cm Hz(1/2) W-1 at 77 K. Thereby, this work facilitates the effective design of high-speed and high-performance heterojunction uncooled MWIR photodetectors.

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