Perfluoroalkyl substances (PFASs) in the Ugandan waters of Lake Victoria: Spatial distribution, catchment release and public exposure risk via municipal water consumption

Perfluoroalkyl substances (PFASs) have scarcely been studied in the Lake Victoria Basin and Africa in general. We investigated spatial profiles of PFASs in the Ugandan part of Lake Victoria, their influxes and human exposure via drinking water. We analyzed open lake water, riverine water (Rivers Kagera and Sio), urban drainage water (Nakivubo Channel), over-lake bulk atmospheric deposition and municipal tap water (Kampala, Jinja and Entebbe). The average concentrations (ng/L) for individual target PFASs were in the ranges of 0.08-23.8 (Nakivubo Channel), 0.01-10.8 (Murchison Bay), R. Kagera, >R. Sio > Nakivubo Channel. Perfluorohexanoic acid (PFHxA) and perfluorooctane sulfonic acid (PFOS) had the highest influx and retention estimates, respectively. Perfluoroalkane sulfonates (PFSAs) were mostly associated with urban drainage samples. PFASs were likely recycled from the Nakivubo Channel, through the Murchison Bay, into municipal drinking water. The estimated human exposure to Sigma(11)PFASs via drinking water indicated low risk of adverse health effects. (C) 2021 Elsevier B.V. All rights reserved.

Automated summary

This study investigated the spatial profiles of PFASs in the Ugandan part of Lake Victoria, and found that PFASs were mostly associated with urban drainage samples. The research suggested that PFASs were likely recycled from urban drainage, through the lake, into municipal drinking water, with low risk of adverse health effects from human exposure via drinking water.