4.7 Article

Effects of Proppant Wettability and Size on Transport and Retention of Coal Fines in Saturated Proppant Packs: Experimental and Theoretical Studies

Journal

ENERGY & FUELS
Volume 35, Issue 15, Pages 11976-11991

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.energyfuels.1c01418

Keywords

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Funding

  1. National Natural Science Foundation of China [42002182, 51774307, 52074331]
  2. National Key Research & Development Program of China [2017YFC0307304]
  3. Major Special Project of CNPC, China [ZD2019-184]
  4. Independent Innovation Research Project of China University of Petroleum (East China) [27RA2002016]

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Hydraulic fracturing is the key technique for extracting coalbed methane, but coal fines retention can lead to fracture conductivity impairment. This study investigated the effects of proppant wettability and size on coal fines retention, finding that increasing proppant hydrophilicity and size decreases fines retention. Analysis of forces and torques on coal fines near proppants showed that proppant wettability and size affect fines retention mechanisms.
Hydraulic fracturing is the main stimulation technique that enables the economic production of coalbed methane reservoirs. However, massive invasion and retention of coal fines in proppant packs can clog the pore spaces and lead to an impairment of fracture conductivity. In this study, the effects of proppant wettability and size on retention of coal fines in proppant packs during the dewatering stage were investigated, for their optimization to achieve a long-term and effective control of fines retention. First, a series of transport and retention experiments of coal fines were performed on saturated proppant packs with different proppant sizes and wettabilities. Herein, standard quartz sand was used as the proppant carrier, and its surface wettability was modified to either hydrophobicity or stronger hydrophilicity by treatment with fluorocarbon resin and piranha solution, respectively. The experimental results indicated that both the retained amount and the deposition rate coefficient of coal fines decreased with increasing proppant hydrophilicity (or decreasing proppant hydrophobicity) and size. For the proppants treated with piranha solution, almost no coal fines were retained in proppant packs. Second, the forces/torques acting on coal fines in the vicinity of proppants were analyzed to elucidate the underlying mechanisms responsible for the influence of proppant wettability and size on fines retention. The effective filter surface (EFS) parameter was estimated by analyzing forces/torques to evaluate the filtration performance of proppant packs. Theoretical results illustrated that the EFS value decreased with increasing proppant hydrophilicity and size. The EFS value for proppants treated with piranha solution was near zero, which was due to the chemically unfavorable retention condition induced by piranha solution treatment. The EFS exhibited a similar tendency to the retention of coal fines observed in experiments, which validated the model. Finally, the recommendations on fines retention control in proppant packs were provided.

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