4.7 Article

Study on the heat transfer reinforcement of glass fiber/epoxy resin composites by grafting and dispersing graphene oxide

Journal

COMPOSITES SCIENCE AND TECHNOLOGY
Volume 216, Issue -, Pages -

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.compscitech.2021.109039

Keywords

Grafting; Dispersion; Graphene oxide; Heat transfer; Composites

Funding

  1. Natural Foundation of Shandong Province [ZR2019BEE068]
  2. Guangdong Basic and Applied Basic Research Foundation [2020A1515111208]

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The research successfully prepared composites by grafting graphene oxide and randomly dispersing graphene oxide on glass fiber. The results showed that under the condition of heating for 60 seconds and containing 0.1% volume of graphene oxide, the thermal conductivity of the dispersed graphene oxide composite increased by 3.48%, while the thermal conductivity of the grafted graphene oxide composite increased by 82.37%.
The grafted-graphene oxide/glass fiber/epoxy resin (grafted-GO/GF/EP) and dispersed-graphene oxide/glass fiber/epoxy resin (dispersed-GO/GF/EP) composites were successfully prepared by grafting graphene oxide (GO) on glass fiber (GF) with coupling agent and random dispersion of GO. A scanning electron microscope (SEM) was employed to characterize the micro structure. The heat transfer RVE models of the grafted-GO/GF/EP and dispersed-GO/GF/EP composites were established respectively. Based on RVE heat transfer simulation model, the heat transfer characteristics of the grafted-GO/GF/EP and dispersed-GO/GF/EP composites were analyzed. The results show that under the condition of 0.1 vol% GO content and heated for 60 s, the thermal conductivities of dispersed-GO/GF/EP and grafted-GO/GF/EP composites are increased by 3.48% and 82.37% respectively. The dispersion of GO increases the heat transfer paths in EP and forms a connected GO-GO heat transfer network. However, with the increasing of GO content, the agglomeration of GO becomes more obvious. The dispersion and interfacial bonding of the GO/GF/EP composites were improved by coupling agent, which effectively reduced the interfacial thermal resistance and significantly improved the thermal conductivity of the composites.

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