4.6 Article

Trace Elements From Ocean-Going Vessels in East Asia: Vanadium and Nickel Emissions and Their Impacts on Air Quality

Journal

Publisher

AMER GEOPHYSICAL UNION
DOI: 10.1029/2020JD033984

Keywords

-

Funding

  1. National Natural Science Foundation of China [42077195, 41877506, 41830641]
  2. Key-Area Research and Development Program of Guangdong Province [2020B1111360001]
  3. Major Program of Shanghai Committee of Science and Technology, China [19DZ1205009]

Ask authors/readers for more resources

This study evaluates the impact of vanadium and nickel emissions from shipping on air quality in East Asia in 2015, finding that ship emissions contribute significantly to these trace metals in the region. The research shows an improvement in the model performance of predicting vanadium and nickel concentrations after including shipping emissions. The study highlights the importance of considering shipping traffic in regional air quality assessments, despite the implementation of low-sulfur fuel policies.
Vanadium (V) and nickel (Ni) are considered the most abundant trace metals in ship exhaust burning heavy fuel oils. This study is the first attempt to estimate the impact of V and Ni from shipping on air quality in East Asia for the year 2015. In this study, emission inventories of V and Ni from shipping and land-based sources were constructed and implemented into the revised aerosol module to simulate ambient V and Ni concentrations. Our results showed that ship emissions contributed the majority of vanadium and were important to nickel emissions in most coastal regions in East Asia, with the contributions exceeding 60% and approximately 40% in some regions, respectively. The simulated ambient V and Ni concentrations has been validated by the measurements, and the comparison revealed there was an obvious improvement (reducing the mean bias by 32%-63%) in the model performance of the V and Ni predictions after including shipping emissions. Our study filled the gaps of trace element contributions in coastal regions and implied that the impact of metals from shipping traffic on regional air quality is worthy of attention in East Asia. Although the International Maritime Organization (IMO) low-sulfur fuel policy has been implemented since 2020, the impact of shipping traffic on trace metals with respect to regional air quality is still important given heavy fuel oils being in use. Key Points Emission inventories of vanadium and nickel from shipping and land-based sources were constructed The revised aerosol module was implemented in the Community Multiscale Air Quality to simulate ambient vanadium and nickel concentrations The strongest impact of ship emissions to vanadium and nickel was found in southeastern China, accounting for 88% and 70%, respectively

Authors

I am an author on this paper
Click your name to claim this paper and add it to your profile.

Reviews

Primary Rating

4.6
Not enough ratings

Secondary Ratings

Novelty
-
Significance
-
Scientific rigor
-
Rate this paper

Recommended

Article Environmental Sciences

Impact of dimethylsulfide chemistry on air quality over the Northern Hemisphere

Junri Zhao, Golam Sarwar, Brett Gantt, Kristen Foley, Barron H. Henderson, Havala O. T. Pye, Kathleen M. Fahey, Daiwen Kang, Rohit Mathur, Yan Zhang, Qinyi Li, Alfonso Saiz-Lopez

Summary: The introduction of oceanic dimethylsulfide (DMS) emissions and its atmospheric chemical reactions into the CMAQv53 model has a significant impact on tropospheric composition and air quality over the Northern Hemisphere, increasing sulfate and sulfur dioxide levels while decreasing aerosol nitrate concentration in the lower atmosphere. The effects of DMS chemistry are most pronounced in the summer and least in the fall, with hydroxyl and nitrate radical-initiated pathways oxidizing 75% of the DMS and halogen-initiated pathways oxidizing the remaining 25%. Overall, DMS chemistry leads to more acidic particles over seawater but has a relatively neutral impact on visibility over most of the seawater.

ATMOSPHERIC ENVIRONMENT (2021)

Article Environmental Sciences

Change of dominant phytoplankton groups in the eutrophic coastal sea due to atmospheric deposition

Haowen Li, Ying Chen, Shengqian Zhou, Fanghui Wang, Tianjiao Yang, Yucheng Zhu, Qingwei Ma

Summary: This study found that atmospheric deposition, along with phosphate input, can significantly enhance the chlorophyll a (Chl a) concentrations in eutrophic waters, facilitating the growth of diatoms and dinoflagellates. Soluble metals, especially copper, in aerosols were identified as key components affecting phytoplankton composition in the eutrophic sea.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

Article Environmental Sciences

Impact of air emissions from shipping on marine phytoplankton growth

Chao Zhang, Zongbo Shi, Junri Zhao, Yan Zhang, Yang Yu, Yingchun Mu, Xiaohong Yao, Limin Feng, Fan Zhang, Yingjun Chen, Xiaohuan Liu, Jinhui Shi, Huiwang Gao

Summary: This study found that ship-emitted particles have a stimulating effect on phytoplankton growth, particularly through nitrogen fertilization. Nitrogen oxides (NOx) emitted from ships contribute approximately 43% of atmospheric nitrogen deposition in the northwest Pacific Ocean (NWPO) and indirectly enhance the deposition of existing reduced nitrogen in the atmosphere, constituting about 15% of atmospheric nitrogen deposition flux.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

Article Geosciences, Multidisciplinary

Atmospheric Deposition Promotes Relative Abundances of High-Dimethylsulfoniopropionate Producers in the Western North Pacific

Haowen Li, Shengqian Zhou, Yucheng Zhu, Ruifeng Zhang, Fanghui Wang, Yang Bao, Ying Chen

Summary: Research findings suggest that atmospheric deposition may impact the relative abundance of high-DMSP producers in the oceans, potentially contributing to climate change.

GEOPHYSICAL RESEARCH LETTERS (2021)

Article Multidisciplinary Sciences

Predicting the effect of confinement on the COVID-19 spread using machine learning enriched with satellite air pollution observations

Xiaofan Xing, Yuankang Xiong, Ruipu Yang, Rong Wang, Weibing Wang, Haidong Kan, Tun Lu, Dongsheng Li, Junji Cao, Josep Penuelas, Philippe Ciais, Nico Bauer, Olivier Boucher, Yves Balkanski, Didier Hauglustaine, Guy Brasseur, Lidia Morawska, Ivan A. Janssens, Xiangrong Wang, Jordi Sardans, Yijing Wang, Yifei Deng, Lin Wang, Jianmin Chen, Xu Tang, Renhe Zhang

Summary: Satellite observations are used to monitor the reincreasing economic activity associated with the lifting of control measures and its effect on the acceleration of COVID-19 cases. Near-real-time satellite NO2 observations provide a better prediction of the deceleration of COVID-19 cases compared to other predictors, indicating the driving role of NO2 in economic activity reduction.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

Article Multidisciplinary Sciences

Spatially explicit analysis identifies significant potential for bioenergy with carbon capture and storage in China

Xiaofan Xing, Rong Wang, Nico Bauer, Philippe Ciais, Junji Cao, Jianmin Chen, Xu Tang, Lin Wang, Xin Yang, Olivier Boucher, Daniel Goll, Josep Penuelas, Ivan A. Janssens, Yves Balkanski, James Clark, Jianmin Ma, Bo Pan, Shicheng Zhang, Xingnan Ye, Yutao Wang, Qing Li, Gang Luo, Guofeng Shen, Wei Li, Yechen Yang, Siqing Xu

Summary: The study presents a promising option to reduce carbon emissions in China's power sector using BECCS technology, estimating a marginal cost curve and spatially explicit method. Retrofitting 222GW of coal power plants in 2836 counties could potentially abate 1.0 Gt CO2-eq annually, but logistical challenges remain.

NATURE COMMUNICATIONS (2021)

Article Meteorology & Atmospheric Sciences

Non-Marine Sources Contribute to Aerosol Methanesulfonate Over Coastal Seas

Shengqian Zhou, Ying Chen, Adina Paytan, Haowen Li, Fanghui Wang, Yucheng Zhu, Tianjiao Yang, Yan Zhang, Ruifeng Zhang

Summary: The study found that terrestrial sources play a significant role in MSA in the East China Sea, while they are not as important in the Gulf of Aqaba. There is a good correlation between aerosol MSA and air mass exposure to surface phytoplankton biomass, which can help in constructing parameterizations for obtaining the spatiotemporal distributions of marine biogenic aerosol components using satellite ocean color datasets.

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES (2021)

Article Engineering, Environmental

Stringent Emission Controls Are Needed to Reach Clean Air Targets for Cities in China under a Warming Climate

Rong Wang, Yechen Yang, Xiaofan Xing, Lin Wang, Jianmin Chen, Xu Tang, Junji Cao, Lidia Morawska, Yves Balkanski, Didier Hauglustaine, Philippe Ciais, Jianmin Ma

Summary: By using a statistical model that takes into account both meteorology and primary emissions, the relationship between PM2.5 concentration and climate change can be better understood. This model reduces errors and suggests that climate change may have a greater impact on PM2.5 than previously thought.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

Article Multidisciplinary Sciences

Black carbon health impacts in the Indo-Gangetic plain: Exposures, risks, and mitigation

Shubha Verma, Sanhita Ghosh, Olivier Boucher, Rong Wang, Laurent Menut

Summary: This study evaluates the impact of black carbon (BC) on population exposure, morbidity, and mortality in the Indo-Gangetic plain. The results show a significant population exposure to BC, with more than 60 million people living in high-concentration areas. In terms of cardiovascular disease mortality, 62% of the burden is attributable to BC exposure in the megacity and 49% in the semiurban area. By implementing emission reduction strategies, over 400,000 lives can potentially be saved from cardiovascular disease mortality annually.

SCIENCE ADVANCES (2022)

Article Multidisciplinary Sciences

Delayed use of bioenergy crops might threaten climate and food security

Siqing Xu, Rong Wang, Thomas Gasser, Philippe Ciais, Josep Penuelas, Yves Balkanski, Olivier Boucher, Ivan A. Janssens, Jordi Sardans, James H. Clark, Junji Cao, Xiaofan Xing, Jianmin Chen, Lin Wang, Xu Tang, Renhe Zhang

Summary: The potential of large-scale bioenergy with carbon capture and storage (BECCS) to limit global warming within 2 degrees Celsius may be hindered by the negative effects of climate change on crop yields, which threatens food security. Early mitigation measures, preferably before 2040, are urgently needed to avoid irreversible climate change and serious food crises.

NATURE (2022)

Article Multidisciplinary Sciences

Accelerating the energy transition towards photovoltaic and wind in China

Yijing Wang, Rong Wang, Katsumasa Tanaka, Philippe Ciais, Josep Penuelas, Yves Balkanski, Jordi Sardans, Didier Hauglustaine, Wang Liu, Xiaofan Xing, Jiarong Li, Siqing Xu, Yuankang Xiong, Ruipu Yang, Junji Cao, Jianmin Chen, Lin Wang, Xu Tang, Renhe Zhang

Summary: China aims to achieve carbon neutrality by 2060, requiring a significant increase in the capacity of photovoltaic (PV) and wind power. However, current projections indicate that the capacity will only reach a level of 5-9.5 PWh/year by 2060. Through optimized deployment of PV and wind power plants, coupled with advanced transmission and energy storage technologies, the capacity can be increased to 15 PWh/year, accompanied by a substantial reduction in the cost of carbon abatement. To achieve this, the annual investment in PV and wind power needs to ramp up significantly over the coming decades.

NATURE (2023)

Article Environmental Sciences

Simulating the radiative forcing of oceanic dimetnylsulfide (DMS) in Asia based on machine learning estimates

Junri Zhao, Weichun Ma, Kelsey R. Bilsback, Jeffrey R. Pierce, Shengqian Zhou, Ying Chen, Guipeng Yang, Yan Zhang

Summary: In this study, the researchers estimated the emissions of Dimethylsulfide (DMS) using a machine learning method and simulated its atmospheric chemistry and radiative effects. They evaluated the contributions of DMS to aerosol and cloud condensation nuclei concentrations, as well as its radiative effects over the Asian region. The findings highlight the importance of understanding DMS emissions and their impact on climate.

ATMOSPHERIC CHEMISTRY AND PHYSICS (2022)

No Data Available