4.7 Review

An Overview of Cellulose-Based Nanogenerators

Journal

ADVANCED MATERIALS TECHNOLOGIES
Volume 6, Issue 3, Pages -

Publisher

WILEY
DOI: 10.1002/admt.202001164

Keywords

cellulose; nanogenerators; piezoelectricity; pyroelectricity; triboelectric effect

Funding

  1. Advance Queensland Research Fellowship of the Queensland Government
  2. University of Queensland
  3. Creative Research Initiative (CRI) program through the National Research Foundation (NRF) of Korea [2014R1A3A2069102]
  4. Science Research Center (SRC) program through the National Research Foundation (NRF) of Korea [2016R1A5A1009405]

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Nanogenerators utilize the piezoelectric, triboelectric, and pyroelectric effects of materials like cellulose to generate power. These eco-friendly and cost-effective devices demonstrate high output and sustainability through various functionalities and fabrication methods.
Developing nanogenerators (NGs) is achieved by exploiting the piezoelectric, triboelectric, and pyroelectric effects of both organic and inorganic materials. Many exhibit beneficial electrical properties (dielectric, conductive, or insulating) or have surfaces that are polarizable upon friction or physical contact. Recently, biomass-derived materials and recycled materials, whose electrical activity can be induced, are explored for application in the design of more sustainable, cost-effective, biodegradable, disposable NGs, and have demonstrated a wide range of output (microenergy) power densities. Among them, cellulose, the most abundant biopolymer, is found to offer excellent opportunities for designing and manufacturing NGs with multifunctional capacities. Cellulose can be derived into varied forms with multifunctionalities and physical morphologies. This account provides an overview of how cellulose is utilized in creating NGs based on piezoelectric, triboelectric, and pyroelectric effects. Because the mechanical properties of cellulose are tunable, current research trends on NGs originate with the triboelectric effect. The discussion here focuses on design, fabrication methods, achievable electrical power output, and combinations with other materials and devices. Challenges in efficient fabrication and consistent power densities, and opportunities for integrating different technologies and developing more sustainable (in terms of economic, environmental, and ecological) nature-human-machine interfacial devices are also discussed.

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