Journal
JOURNAL OF CATALYSIS
Volume 396, Issue -, Pages 324-332Publisher
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcat.2021.02.029
Keywords
Ni3P/gamma-Al2O3; Hydrodeoxygenation; Phenol; Bifunctional; Electroless plating
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Funding
- Natural Science Foundation of China [21972014, 21473017, 21603024, 21872014, U1508205]
- International S&T Cooperation Program of China [2016YFE0109800]
- Fundamental Research Funds for the Central Universities [DUT19GJ205]
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A bifunctional Ni3P/alpha-Al2O3 catalyst prepared by an electroless plating method showed high performance in the hydrodeoxygenation of phenol, and remained structurally stable during a 100-hour run.
A bifunctional Ni3P/alpha-Al2O3 catalyst was prepared by an electroless plating method and characterized by XRD, XPS, N-2 adsorption-desorption, ICP, TEM, CO chemisorption, NH3 TPD, and Py-FTIR. To improve the dispersion of Ni3P on gamma-Al2O3, highly dispersed nickel aluminum oxide hydrate was deposited on gamma-Al2O3 by a deposition-precipitation procedure. The resulting Ni3P nanoparticles (similar to 3.8 nm) were homogeneously dispersed on gamma-Al2O3. The Ni3P/gamma-Al2O3 catalyst exhibited high performance in the hydrodeoxygenation of phenol, in which both hydrogenation and dehydration were involved. The Ni3P/gamma-Al2O3 was remarkably stable both in catalytic performance and in structure during a 100-h run. (C) 2021 Elsevier Inc. All rights reserved.
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