Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 31, Issue 16, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202010483
Keywords
metal hydrides; optical hydrogen sensing; tantalum; thin films; X‐ ray diffraction
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Thin film Ta1-yPdy is an effective optical sensing material for hydrogen detection, with a wide sensing range cover 7 orders of magnitude. The sensing range can be easily tuned by adjusting Pd concentration without sacrificing sensitivity, and with suitable capping layer, sub-second response times can be achieved even at room temperature, faster than any other known thin-film hydrogen sensor.
Hydrogen detection in a reliable, fast, and cost-effective manner is a prerequisite for the large-scale implementation of hydrogen in a green economy. Thin film Ta1-yPdy is presented as an effective optical sensing material with extremely wide sensing ranges covering at least 7 orders of magnitude in hydrogen pressure. Nanoconfinement of the Ta1-yPdy layer suppresses the first-order phase transitions present in bulk and ensures a sensing response free of any hysteresis. Unlike other sensing materials, Ta1-yPdy features the special property that the sensing range can be easily tuned by varying the Pd concentration without a reduction of the sensitivity of the sensing material. Combined with a suitable capping layer, sub-second response times can be achieved even at room temperature, faster than any other known thin-film hydrogen sensor.
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