Journal
CATALYSTS
Volume 10, Issue 12, Pages -Publisher
MDPI
DOI: 10.3390/catal10121421
Keywords
selective catalytic reduction; vanadia-based catalysts; low-temperature activity; reaction mechanism
Categories
Funding
- National Natural Science Foundation of China [21637005, 51822811]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA23010201]
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Selective catalytic reduction of NOx with NH3 (NH3-SCR) has been successfully applied to abate NOx from diesel engines and coal-fired industries on a large scale. Although V2O5-WO3(MoO3)/TiO2 catalysts have been utilized in commercial applications, novel vanadia-based catalysts have been recently developed to meet the increasing requirements for low-temperature catalytic activity. In this article, recent progress on the improvement of the low-temperature activity of vanadia-based catalysts is reviewed, including modification with metal oxides and nonmetal elements and the use of novel supports, different synthesis methods, metal vanadates and specific structures. Investigation of the NH3-SCR reaction mechanism, especially at low temperatures, is also emphasized. Finally, for low-temperature NH3-SCR, some suggestions are given regarding the opportunities and challenges of vanadia-based catalysts in future research.
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