Journal
ELECTROCHIMICA ACTA
Volume 365, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.electacta.2020.137383
Keywords
PEMFC; Vapour transport; Local temperature gradient; Visualisation analysis
Categories
Funding
- Japan Science and Technology Agency (JST), PRESTO [JPMJPR13C1]
- PRESTO network, and Strategic International Research Cooperative Program
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Water management is critical for the function of PEMFC, and the temperature gradient of the cathode GDL plays a significant role. Research has shown that a temperature difference can lead to a drastic decrease in PEMFC performance due to different preferential sites for water condensation.
Water management is critical for the function of the proton exchange membrane fuel cell (PEMFC). The local through-thickness temperature gradient of the cathode gas diffusion layer (GDL) affect water management for a PEMFC. That has been known and been targeted for the discussion for several years. In this study, the effects of temperature gradient inside PEMFC was investigated by controlling it externally with a fine (testing diameter about 30 mu m) and thin (thickness about 6 mu m) thin-film thermocouple (TFTC), which has been developed using micro electromechanical system (MEMS) technology. In addition, X-ray computed tomography (CT) has been chosen as a method to visualise inside of an operating PEMFC. The simultaneously measurement of temperature gradient and liquid water distribution was firstly accomplished. In conclusion, in the case where the temperature of the cathode catalyst coated membrane (CCM) side is higher than that of the channel side, the PEMFC performance drastically decreased. The difference in PEMFC performance was caused by a difference the preferential sites for water condensation. (c) 2020 Elsevier Ltd. All rights reserved.
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