4.8 Article

Efficient and inexpensive preparation of graphene laminated film with ultrahigh thermal conductivity

Journal

CARBON
Volume 171, Issue -, Pages 639-645

Publisher

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2020.09.039

Keywords

Thermal conductivity; Graphene paper; Low energy cost; Macroscopic; Pilot plant test

Funding

  1. Guangdong Province Key Area RD Program [2019B010933001]
  2. National Natural Science Foundation of China (NSFC), China [21627809, 21501169]
  3. National Natural Science Foundation of China [51725204, 51572179, 21771132, 21471106, 21501126]

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With the rapid development of electronic technology, the demand for thermal management materials is increasing continuously. Graphene paper is considered as a potential material to replace the traditional graphitized polyimide film, but its application is limited due to high energy consumption and heavy metal contamination. A new technology has been developed to produce graphene paper efficiently and cost-effectively, achieving promising results.
With the rapid development of electronic technology, the demand for thermal management materials is increasing continuously. Recent years graphene paper is considered as a potential material to replace the traditional graphitized polyimide film. Although the current route to graphene paper can achieve a high thermal conductivity, the extremely high energy consumption in graphitization procedure and severe heavy metal contamination limit the application of graphene paper. Here we develop a high-efficiency, low-energy cost, and inexpensive technology to produce graphene paper in large quantities. Without graphitization, the thermal conductivity of this graphene laminated film can reach 975 Wm(-1) K-1 when the thickness of film is 65 mm. Based on this easy-operated technology, we have already completed the pilot plant test, attained capacity of 3 kg graphene per reactor in 8 h and 800 mm x 100 m of graphene film each roll which was continuously and macroscopically assembled on our self-made equipment. (C) 2020 Elsevier Ltd. All rights reserved.

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