Journal
NANO LETTERS
Volume 20, Issue 7, Pages 5451-5457Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c01939
Keywords
nucleic acid; systems chemistry; endonuclease; DNAzyme; DNA nanotechnology
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Funding
- Israel Science Foundation
- Minerva Center for Biohybrid Complex Systems
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Enzymes (endonucleases) are coupled to constitutional dynamic networks to stimulate the selection of a constituent and cascaded emergence of a new network. This is exemplified with the EcoRI-dictated depletion of a network and selection of a constituent that activates the cascaded emergence of a new network. The new network is further depleted by HindIII to a selected constituent that can be coupled to the cascaded emergence of a dynamic network. In addition, upon subjecting a [3 x 3] constitutional dynamic network to endonucleases EcoRI and HindIII, the programmed hierarchical selection of [2 x 2] constitutional dynamic networks followed by the biocatalytic selection of a constituent for the subsequent emergence of new networks is demonstrated.
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