Journal
CHINESE JOURNAL OF CHEMICAL PHYSICS
Volume 29, Issue 5, Pages 635-643Publisher
CHINESE PHYSICAL SOC
DOI: 10.1063/1674-0068/29/cjcp1603056
Keywords
Biomass pyrolysis-oil; Bio-hydrogen; Olefins polymerization; Fischer-Tropsch synthesis; Bio-fuels
Categories
Funding
- National Sci-Tech Support Plan [2014BAD02B03]
- Program for Changjiang Scholars and Innovative Research Team in University
- Fundamental Research Funds for the Central Universities [wk2060190040]
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In recent years, production of engine fuels and energy from biomass has drawn much interest. In this work, we conducted a novel integrated process for the preparation of bio-hydrogen and bio-fuels using lignocellulosic biomass pyrolysis-oil (bio-oil). The process includes (i) the production of bio-hydrogen or bio-syngas by the catalytic cracking of bio-oil, (ii) the adjustment of bio-syngas and (iii) the production of bio-fuels by olefinic polymerization (OP) together with Fischer-Tropsch synthesis (FTS). Under the optimal conditions, the yield of bio-hydrogen was 120.9 g H-2/(kg bio-oil). The yield of hydrocarbon bio-fuels reached 526.1 g/(kg bio-syngas) by the coupling of OP and FTS. The main reaction pathways (or chemical processes) were discussed based on the products observed and the catalyst property.
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