Journal
CHEMELECTROCHEM
Volume 7, Issue 8, Pages 1838-1842Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/celc.202000180
Keywords
cyclo[18]carbon; CO2 electroreduction; carbon catalysis; catalytic mechanism; density functional theory
Categories
Funding
- National Natural Science Foundation of China [21872041, 21373091]
- Science and Technology Project of Guangzhou city [201704030040]
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Cyclo[18]carbon (C-18) as a special molecular allotrope of carbon composed of two-coordinate carbon atoms has recently been manufactured and characterized by atomic manipulation. Herein, we analyze the electrochemical reduction characteristics of carbon dioxide (CO2) on typical carbon materials (graphene, C-60, carbon nanotubes and C-18) using density functional calculations. Encouragingly, C-18 shows excellent CO2 reduction activity compared to other carbon materials.
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